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Carbohydr Polym ; 251: 116987, 2021 Jan 01.
Article in English | MEDLINE | ID: mdl-33142559

ABSTRACT

The kinetics of thermal degradation of ß-chitin extracted from Dosidicus gigas squid pen, was studied at normal conditions as well as after being subjected to the action of high-pressure impact of 9.7 GPa. The integral iso-conversional procedure of Kissinger-Akahira-Sunose (KAS) recommended by the ICTAC kinetics committee was applied to the non-isothermal data obtained from thermogravimetry (TGA). Lifetimes were predicted without assumption of any reaction model. Heating rates of ß = 10, 15, 20 and 25 °C/min under nitrogen atmosphere were used from room temperature to 1300 °C. A comparative study with α-chitin was performed. All the samples were structurally and chemically characterized by several techniques. The extracted ß-chitin was found to be in the monohydrate form; while with the action of high-pressure impact, it was transformed into ß-chitin dehydrate showing slightly higher stability. Reliable prediction for lifetimes considering working temperatures over 425 K was found for α and ß-chitin.


Subject(s)
Chitin/chemistry , Decapodiformes/chemistry , Animals , Atmospheric Pressure , Biodegradation, Environmental , Carbohydrate Conformation , Crystallization , Kinetics , Microscopy, Electron, Scanning , Powder Diffraction , Spectroscopy, Fourier Transform Infrared , Temperature , Thermogravimetry , X-Ray Diffraction
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