Observation of magnetic vortex configuration in non-stoichiometric Fe3O4 nanospheres.

Theoretical and micromagnetic simulation studies of magnetic nanospheres with vortex configurations suggest that such nanostructured materials have technological advantages over conventional nanosystems for applications based on high-power-rate absorption and subsequent emission. However, full experimental evidence of magnetic vortex configurations in spheres of submicrometer size is still lacking. Here, we report the microwave irradiation fabrication of Fe3O4 nanospheres and establish their magnetic vortex configuration based on experimental results, theoretical analysis, and micromagnetic simulations. Detailed magnetic and electrical measurements, together with Mössbauer spectroscopy data, provide evidence of a loss of stoichiometry in vortex nanospheres owing to the presence of a surface oxide layer, defects, and a higher concentration of cation vacancies. The results indicate that the magnetic vortex spin configuration can be established in bulk spherical magnetite materials. This study provides crucial information that can aid the synthesis of magnetic nanospheres with magnetically tailored properties; consequently, they may be promising candidates for future technological applications based on three-dimensional magnetic vortex structures.

Stabilization of Magnetic Skyrmions on Arrays of Self-Assembled Hexagonal Nanodomes for Magnetic Recording Applications.

Magnetic skyrmions are nontrivial spin textures that resist external perturbations, being promising candidates for the next-generation recording devices. Nevertheless, a major challenge in realizing skyrmion-based devices is the stabilization of ordered arrays of these spin textures under ambient conditions and zero applied field. Here, we demonstrate for the first time the formation and stabilization of magnetic skyrmions on the arrays of self-assembled hexagonal nanodomes taking advantage of the intrinsic properties of its curved geometry. Magnetic force microscopy images from the arrays of 100 nm nanodomes showed stable skyrmions at the zero field that are arranged following the topography of the nanostructure. Micromagnetic simulations are compared to the experiments to determine the correlation of the domain textures with the topography of the samples. We propose a simple method to nucleate and annihilate skyrmions, opening the possibility for an ultradense data storage based on the high stability and low energy consumption of the skyrmionic textures.