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Chemistry ; 24(50): 13306-13310, 2018 Sep 06.
Article in English | MEDLINE | ID: mdl-29989264

ABSTRACT

A novel catalytic enantioselective methodology based on synergistic catalysis for the synthesis of chiral 2-acyl pyridines and pyrazines is reported. The strategy involves the metal-Lewis acid activation of acetyl aza-arenes and the secondary-amine activation of enals. The proposed mechanism is supported by DFT calculations.

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