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A highly enantioselective allylic amination reaction using a commercially available chiral rhodium catalyst: resolution of racemic allylic carbonates.
Vrieze, Derek C; Hoge, Garrett S; Hoerter, Perrine Z; Van Haitsma, Jared T; Samas, Brian M.
Org Lett ; 11(14): 3140-2, 2009 Jul 16.
Article in English | MEDLINE | ID: mdl-19527001

ABSTRACT

A novel method for the kinetic resolution of unsymmetrical acyclic allylic carbonates and the concurrent synthesis of enantioenriched secondary amines using a commercially available chiral catalyst is disclosed.


Subject(s)
Allyl Compounds/chemistry , Amines/chemical synthesis , Carbonates/chemistry , Rhodium/chemistry , Amines/chemistry , Catalysis , Molecular Structure , Stereoisomerism
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