Small footprint cholesteric liquid crystal laser.

We demonstrate a small optical bench footprint laser assembly based on the small pulsed Nd:YAG laser head SSY-1 for pumping cholesteric liquid crystal (CLC) lasers and illustrate its performance using low molecular weight CLC samples doped with the fluorescent dye PM597. A low lasing threshold, narrow laser line, and far-field interference patterns of the CLC laser were observed using the SSY-1-based laser assembly as the pump. The emission characteristics of the CLC laser are similar to those observed with comparable CLC materials pumped by an order of magnitude physically larger and many orders of magnitude more expensive commercial Nd:YAG laser systems. The small footprint CLC laser demonstrated in this work provides an opportunity for significant size and cost reduction of CLC lasers and fostering their practical applications.

Topology-commanded optical properties of bistable electric-field-induced torons in cholesteric bubble domains.

Nowadays, complicated topological defects enable many experimental manipulations and configurational simulations of active soft matter for optical and photonic applications. Investigation of topological defects in soft anisotropic materials enables one to better understand three-dimensional orientation fields in cholesteric liquid crystals. Here, we describe optical properties of bistable bubble domain (BD) texture torons in a thin layer of cholesteric liquid crystal (CLC), frustrated by homeotropic anchoring conditions, and reliably switchable by a random process. The control of macroscopic optical density and diffraction efficiency of the BD texture is demonstrated by a selection of a confinement ratio of the CLC. Experimentally reconstructed CLC director profile reveals the topology of BD torons allowing consideration of naturally occurring BD texture for applications in optical and photonic devices, which are bistably switchable between active and transparent optical states.

Command Electro-Optical Switching of Photoaligned Liquid Crystal on Photopatterned Graphene.

We report command electro-optical switching on photolithographically-patterned graphene into a high-density electrode pattern for a high-transmission in-plane-switching (IPS) liquid crystal device. A highly-effective liquid crystal photoalignment method is used to maximize the field-driven optical contrast of a prototyped device. A non-contact and low-temperature photoalignment allows delicate surface treatment required for successful processing of graphene layer into an IPS electrode structure. Electro-optic performance of the graphene-based single pixel laboratory IPS prototype demonstrates the application potential of graphene for liquid crystal electro-optic devices with complex and high-definition electrode patterns.

Giant Flexoelectro-optic Effect with Liquid Crystal Dimer CB7CB.

We demonstrate a giant flexoelectro-optic behavior of liquid crystal dimer CB7CB. Flexoelectric properties of CB7CB experimentally characterized by measured angle of an in-plane rotation of helical axis (HA) in polymer stabilized uniform lying helix cholesteric liquid crystal. The 45° rotation of HA providing full intensity modulation of transmitted through a pair of crossed polarizers light, is achieved with 4.5 V/µm with a sub-millisecond electro-optic switching time. Reported properties enable application of CB7CB in applications of the flexoelectric effect in fast switching photonic and electro-optic devices.

Electrically tunable laser based on oblique heliconical cholesteric liquid crystal.

A cholesteric liquid crystal (CLC) formed by chiral molecules represents a self-assembled one-dimensionally periodic helical structure with pitch [Formula: see text] in the submicrometer and micrometer range. Because of the spatial periodicity of the dielectric permittivity, a CLC doped with a fluorescent dye and pumped optically is capable of mirrorless lasing. An attractive feature of a CLC laser is that the pitch [Formula: see text] and thus the wavelength of lasing [Formula: see text] can be tuned, for example, by chemical composition. However, the most desired mode to tune the laser, by an electric field, has so far been elusive. Here we present the realization of an electrically tunable laser with [Formula: see text] spanning an extraordinarily broad range (>100 nm) of the visible spectrum. The effect is achieved by using an electric-field-induced oblique helicoidal (OH) state in which the molecules form an acute angle with the helicoidal axis rather than align perpendicularly to it as in a field-free CLC. The principal advantage of the electrically controlled CLCOH laser is that the electric field is applied parallel to the helical axis and thus changes the pitch but preserves the single-harmonic structure. The preserved single-harmonic structure ensures efficiency of lasing in the entire tunable range of emission. The broad tuning range of CLCOH lasers, coupled with their microscopic size and narrow line widths, may enable new applications in areas such as diagnostics, sensing, microscopy, displays, and holography.

Tunable lasing in cholesteric liquid crystal elastomers with accurate measurements of strain.

We report wide range and reversible tuning of the selective reflection band of a single crystal cholesteric liquid crystal elastomer (CLCE). The tuning is the result of mechanical shortening of the helical pitch achieved by imposing a uniform uniaxial strain along the helical axis. On doping the CLCE sample with a laser dye, we observe lasing from the CLCE in both glassy and rubbery states. By changing the cholesteric pitch, mechanical compression provides tuning of the laser emission from the dye doped CLCE over a significant part of the fluorescence band of the laser dye. In this work we demonstrate for the first time that both the CLCE pitch and the lasing wavelength are linearly dependent on the strain imposed on the CLCE film.

Photoswitchable and dye-doped bubble domain texture of cholesteric liquid crystals.

We demonstrate control of the transmittance of the naturally formed bubble domain (BD) texture of cholesteric liquid crystals (CLC) with negative dielectric anisotropy confined into a cell with homeotropic surface anchoring. By using a photosensitive chiral dopant with variable helical twisting power under light irradiation, control of packing density of bubbles, spatial patterning, and all optical switching between bistable states with different optical densities is achieved. By introducing dichroic dye into the CLC mixture, a bistable and switchable by applied electric field guest-host system is obtained. The light dimming properties of dye-doped BD CLC systems may lead to development of a wide range of applications.