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1.
Sci Rep ; 7: 46296, 2017 04 10.
Article in English | MEDLINE | ID: mdl-28393931

ABSTRACT

In search of novel, improved materials for magnetic data storage and spintronic devices, compounds that allow a tailoring of magnetic domain shapes and sizes are essential. Good candidates are materials with intrinsic anisotropies or competing interactions, as they are prone to host various domain phases that can be easily and precisely selected by external tuning parameters such as temperature and magnetic field. Here, we utilize vector magnetic fields to visualize directly the magnetic anisotropy in the uniaxial ferromagnet CeRu2Ga2B. We demonstrate a feasible control both globally and locally of domain shapes and sizes by the external field as well as a smooth transition from single stripe to bubble domains, which opens the door to future applications based on magnetic domain tailoring.

2.
Phys Rev Lett ; 110(11): 117204, 2013 Mar 15.
Article in English | MEDLINE | ID: mdl-25166571

ABSTRACT

In the spin ladder compound BiCu(2)PO(6), there exists a decisive dynamics of spin excitations that we classify and characterize using inelastic light scattering. We observe an interladder singlet bound mode at 24 cm(-1) and two intraladder bound states at 62 and 108 cm(-1) in the leg (bb) and the rung (cc) polarization as well as a broad triplon continuum extending from 36 cm(-1) to 700 cm(-1). Though isolated spin ladder physics can roughly account for the observed excitations at high energies, frustration and interladder interactions need to be considered to fully describe the spectral distribution and scattering selection rules at low and intermediate energies. In addition, we attribute the rich spectrum of singlet bound modes to a melting of a dimer crystal. Our study provides evidence for a Z(2) quantum phase transition from a dimer to a resonating valence bond state driven by singlet fluctuations.

3.
J Phys Condens Matter ; 24(18): 185602, 2012 May 09.
Article in English | MEDLINE | ID: mdl-22508934

ABSTRACT

Despite the conceptional importance of realizing spin liquids in solid states only few compounds are known. On the other hand the effect of lattice distortions and anisotropies on the magnetic exchange topology and the fluctuation spectrum is an interesting problem. We compare the excitation spectra of the two s = 1/2 kagome lattice compounds, volborthite and vesignieite, using Raman scattering. We demonstrate that even small modifications of the crystal structure may have a huge effect on the phonon spectrum and low-temperature properties.

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