Two-quantum magnetic resonance driven by a comb-like rf field.

We report a new method for excitation of magnetic resonance in an optically aligned atomic ensemble. It employs a comb-like rf field acting on the end sublevels of the Fg=1 state separated by the doubled Zeeman frequency. This approach provides a resonance without substructures associated with the quadratic Zeeman shift. A theoretical explanation of the effect is given in terms of the two-quantum transition |Fg=1,mFg=-1⟩⇆|Fg=1,mFg=1⟩ and is corroborated by an experiment with 87Rb atoms. Possible advantages of the approach and its range of applicability are discussed.

Mass selective laser cooling of 229Th3+ in a multisectional linear Paul trap loaded with a mixture of thorium isotopes.

We consider an experiment on trapping and laser cooling of 229Th3+ ions in a linear Paul trap in the presence of undesirable impurities such as ions of the radioactive isotope 228Th3+. We suggest a method of separating these impurities by means of selective laser cooling utilizing the isotope shift of cooling transitions in 229Th3+ and 228Th3+ ions. According to our estimation, the isotope shift is equal to 3.4 GHZ and makes laser separation of these isotopes possible.

Loading of mass spectrometry ion trap with Th ions by laser ablation for nuclear frequency standard application.

We describe an original multisectional quadrupole ion trap aimed to realize nuclear frequency standard based on the unique isomer transition in thorium nucleus. It is shown that the system effectively operates on Th+, Th2+ and Th3+ ions produced by laser ablation of metallic thorium-232 target. Laser intensity used for ablation is about 6 GW/cm2. Via applying a bias potential to every control voltage including the RF one, we are able not only to manipulate ions within the energy range as wide as 1-500 eV but to specially adjust trap potentials in order to work mainly with ions that belong to energy distribution maximum and therefore to effectively enhance the number of trapped ions. Measurement of energy distributions of 232Th+, 232Th2+, 232Th3+ ions obtained by laser ablation allows us to define optimal potential values for trapping process. Observed number of ions inside trap in dependence on trapping time is found to obey an unusually slow - logarithmic decay law that needs more careful study.