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Highly enantioselective zinc/amino alcohol-catalyzed alkynylation of aldehydes.
Zhong, Jiang-Chun; Hou, Shi-Cong; Bian, Qing-Hua; Yin, Min-Min; Na, Ri-Song; Zheng, Bing; Li, Zhi-Yuan; Liu, Shang-Zhong; Wang, Min.
Chemistry ; 15(13): 3069-71, 2009.
Article in English | MEDLINE | ID: mdl-19219869

ABSTRACT

Meeting the challenge: The zinc/amino alcohol catalyzed enantioselective addition of terminal alkynes to aldehydes is effective with both phenylacetylene and methyl propiolate, leading to chiral secondary propargyl alcohols with very high enantioselectivity (see scheme).


Subject(s)
Aldehydes/chemistry , Alkynes/chemistry , Amino Alcohols/chemistry , Propanols/chemical synthesis , Zinc/chemistry , Alkynes/chemical synthesis , Catalysis , Combinatorial Chemistry Techniques , Cyclopropanes/chemistry , Models, Chemical , Molecular Structure , Stereoisomerism
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