Ultracompact meta-pixels for high colour depth generation using a bi-layered hybrid metasurface.

Nano-structural colour pixels have attracted much attention as promising solutions for compact display devices. However, it is difficult to miniaturize and integrate conventional transmissive colour filtering components for high resolution pixels within subwavelength scale without sacrificing colour depth. Here, we propose a novel colour pixel structure using bi-layered hybrid metasurfaces that are composed of aluminum nanograting and amorphous silicon nanorod layers. The independent high-contrast control of resonance intensity and spectral position is achieved by anisotropic Mie resonances and cavity effect between stacked two metasurfaces. Moreover, the proposed structures permit the wide colour gamut through the novel physical principles. In addition, a meta-pixel which can provide gradual tuning of colour is demonstrated to obtain high colour depth. The proposed structures are expected to be fruitful for the development of next generation display and imaging systems.

Kinetics of lipid raft formation at lipid monolayer-bilayer junction probed by surface plasmon resonance.

A label-free, non-dispruptive, and real-time analytical device to monitor the dynamic features of biomolecules and their interactions with neighboring molecules is an essential prerequisite for biochip- and diagonostic assays. To explore one of the central questions on the lipid-lipid interactions in the course of the liquid-ordered (lo) domain formation, called rafts, we developed a method of reconstituting continuous but spatially heterogeneous lipid membrane platforms with molayer-bilayer juntions (MBJs) that enable to form the lo domains in a spatiotemporally controlled manner. This allows us to detect the time-lapse dynamics of the lipid-lipid interactions during raft formation and resultant membrane phase changes together with the raft-associated receptor-ligand binding through the surface plasmon resonance (SPR). For cross-validation, using epifluorescence microscopy, we demonstrated the underlying mechanisms for raft formations that the infiltration of cholesterols into the sphingolipid-enriched domains plays a crucial roles in the membrane phase-separation. Our membrane platform, being capable of monitoring dynamic interactions among lipids and performing the systematic optical analysis, will unveil physiological roles of cholesterols in a variety of biological events.

Plasmonic metasurface cavity for simultaneous enhancement of optical electric and magnetic fields in deep subwavelength volume.

It has been hard to achieve simultaneous plasmonic enhancement of nanoscale light-matter interactions in terms of both electric and magnetic manners with easily reproducible fabrication method and systematic theoretical design rule. In this paper, a novel concept of a flat nanofocusing device is proposed for simultaneously squeezing both electric and magnetic fields in deep-subwavelength volume (~λ3/538) in a large area. Based on the funneled unit cell structures and surface plasmon-assisted coherent interactions between them, the array of rectangular nanocavity connected to a tapered nanoantenna, plasmonic metasurface cavity, is constructed by periodic arrangement of the unit cell. The average enhancement factors of electric and magnetic field intensities reach about 60 and 22 in nanocavities, respectively. The proposed outstanding performance of the device is verified numerically and experimentally. We expect that this work would expand methodologies involving optical near-field manipulations in large areas and related potential applications including nanophotonic sensors, nonlinear responses, and quantum interactions.

Huygens' optical vector wave field synthesis via in-plane electric dipole metasurface.

We investigate Huygens' optical vector wave field synthesis scheme for electric dipole metasurfaces with the capability of modulating in-plane polarization and complex amplitude and discuss the practical issues involved in realizing multi-modulation metasurfaces. The proposed Huygens' vector wave field synthesis scheme identifies the vector Airy disk as a synthetic unit element and creates a designed vector optical field by integrating polarization-controlled and complex-modulated Airy disks. The metasurface structure for the proposed vector field synthesis is analyzed in terms of the signal-to-noise ratio of the synthesized field distribution. The design of practical metasurface structures with true vector modulation capability is possible through the analysis of the light field modulation characteristics of various complex modulated geometric phase metasurfaces. It is shown that the regularization of meta-atoms is a key factor that needs to be considered in field synthesis, given that it is essential for a wide range of optical field synthetic applications, including holographic displays, microscopy, and optical lithography.

Complete amplitude and phase control of light using broadband holographic metasurfaces.

Reconstruction of light profiles with amplitude and phase information, called holography, is an attractive optical technology with various significant applications such as three-dimensional imaging and optical data storage. Subwavelength spatial control of both amplitude and phase of light is an essential requirement for an ideal hologram. However, traditional holographic devices suffer from their restricted capabilities of incomplete modulation in both amplitude and phase of visible light; this results in sacrifice of optical information and undesirable occurrences of critical noises in holographic images. Herein, we have proposed a novel metasurface that is capable of completely controlling both the amplitude and phase profiles of visible light independently with subwavelength spatial resolution. The full, continuous, and broadband control of both amplitude and phase was achieved using X-shaped meta-atoms based on the expanded concept of the Pancharatnam-Berry phase. The first experimental demonstrations of the complete complex-amplitude holograms with subwavelength definition at visible wavelengths were achieved, and excellent performances with a remarkable signal-to-noise ratio as compared to those of traditional phase-only holograms were obtained. Extraordinary control capability with versatile advantages of our metasurface paves a way to an ideal holography, which is expected to be a significant advancement in the field of optical holography and metasurfaces.

Broadband efficient modulation of light transmission with high contrast using reconfigurable VO2 diffraction grating.

Ultra-compact dynamically reconfigurable modulation of optical transmission has been widely studied by using subwavelength-spaced resonant metasurface structures containing reconfigurable optical materials. However, it has been difficult to achieve high transmissivity, large modulation depth, and broad bandwidth simultaneously with the conventional resonance-based metasurface schemes. Here, we propose a reconfigurable phase-transition diffractive grating, made of thick VO2 ridge waveguides, for achieving the above-mentioned three goals simultaneously in the near-infrared range. Based on the large dielectric-to-plasmonic transition characteristic of VO2 in the near-infrared range, diffraction directivity of dual-VO2 ridge waveguide is designed to be tuned by thermally driven phase transition of VO2 for transverse electrically polarized illumination. Then, the diffractive VO2 ridge waveguide grating composed of the periodically arranged dual VO2 ridge waveguides is designed with on-state efficiency around 0.3 and minimum modulation depth about 0.35 over a broad bandwidth of 550 nm (1100-1650 nm). The working principle and excellent modulation performance are thoroughly verified through numerical and experimental studies.

Broadband ultrathin circular polarizer at visible and near-infrared wavelengths using a non-resonant characteristic in helically stacked nano-gratings.

Modern imaging and spectroscopy systems require to implement diverse functionalities with thin thickness and wide wavelength ranges. In order to meet this demand, polarization-resolved imaging has been widely investigated with integrated circular polarizers. However, the circular polarizers which operate at the entire visible wavelengths and have a thickness of several tens of nanometers have not been developed yet. Here, a circular polarizer, operating at the entire visible wavelength range, is demonstrated using helically stacked aluminum nano-grating layers. High extinction ratio and broad operation bandwidth are simultaneously achieved by using non-resonant anisotropic characteristics of the nano-grating. It is theoretically verified that the averaged extinction ratio becomes up to 8 over the entire visible wavelength range while having a thickness of 390 nm. Also, the feasibility of the proposed structure and circular polarization selectivity at the visible wavelength range are experimentally verified. It is expected that the proposed structure will lead to extreme miniaturization of a circular polarizer and contribute greatly to the development of mobile/wearable imaging systems such as virtual reality and augmented reality displays.

Active directional switching of surface plasmon polaritons using a phase transition material.

Active switching of near-field directivity, which is an essential functionality for compact integrated photonics and small optoelectronic elements, has been challenging due to small modulation depth and complicated fabrication methods for devices including active optical materials. Here, we theoretically and experimentally realize a nanoscale active directional switching of surface plasmon polaritons (SPPs) using a phase transition material for the first time. The SPP switching device with noticeable distinction is demonstrated based on the phase transition of vanadium dioxide (VO2) at the telecom wavelength. As the insulator-to-metal phase transition (IMT) of VO2 induces the large change of VO2 permittivity at telecom wavelengths, the plasmonic response of a nanoantenna made of VO2 can be largely tuned by external thermal stimuli. The VO2-insulator-metal (VIM) nanoantenna and its periodic array, the VIM metagrating, are suggested as optical switches. The directional power distinction ratio is designed to change from 8.13:1 to 1:10.56 by the IMT and it is experimentally verified that the ratio changes from 3.725:1 to 1:3.132 as the VIM metagratings are heated up to 90 °C. With an electro-thermally controllable configuration and an optimized resonant design, we expect potential applications of the active switching mechanism for integrable active plasmonic elements and reconfigurable imaging.

Triple-slit nanoaperture for transmission enhancement of a cavity-aperture.

A cavity-aperture has a problem of low transmission efficiency due to its nano-sized aperture despite its potential for plasmonic color filters. In this study, a triple-slit aperture is proposed as the nanoaperture in the center of the cavity-aperture to improve the transmittance. It provides one centered nanoslit and two symmetric wedge structures to each of three cavities corresponding to incident polarization, and induces the strong confinement and transmission of electric fields due to plasmonic resonances at the two types of nanostructures. The transmittance of the triple-slit aperture is theoretically five times and experimentally two times higher than that of a circular aperture. Furthermore, expansive studies on polarization-insensitive nanoapertures with six-fold rotational symmetry will contribute to the development of plasmonic color filters and imaging devices.

Interferometric control of plasmonic resonator based on polarization-sensitive excitation of surface plasmon polaritons.

A plasmonic resonator is proposed whose electromagnetic energy density can be tuned by the polarization state of the incident light. Counter-propagating surface plasmon polaritons, which are excited by polarization-sensitive subwavelength apertures, give tunability. Stored energy density in the resonator varies from the minimum to the maximum when the orientation angle of the incoming electric field rotates by 90 degrees. After optimizing a rectangular cavity and periodic gratings, the on/off ratio is calculated as 430 and measured as 1.55. Based on our scheme, interferometric control is executed simply by rotation of a polarizer. The proposed plasmonic resonator can be utilized in all-optically controlled active plasmonic devices, coherent network elements, particle trapping systems, and polarimeters.

Near-field focus steering along arbitrary trajectory via multi-lined distributed nanoslits.

The modulation of near-field signals has recently attracted considerable interest because of demands for the development of nano-scale optical devices that are capable of overcoming the diffraction limit of light. In this paper, we propose a new type of tuneable plasmonic lens that permits the foci of surface plasmon polariton (SPP) signals to be continuously steered by adjusting the input polarization state. The proposed structure consists of multi-lined nanoslit arrays, in which each array is tilted at a different angle to provide polarization sensitivity and the nanoslit size is adjusted to balance the relative amplitudes of the excited SPPs from each line. The nanoslits of each line are designed to focus SPPs at different positions; hence, the SPP focal length can be tuned by modifying the incident polarization state. Unlike in previously reported studies, our method enables plasmonic foci to be continuously varied with a smooth change in the incident linear polarization state. The proposed structures provide a novel degree of freedom in the multiplexing of near fields. Such characteristics are expected to enable the realization of active SPP modulation that can be applied in near-field imaging, optical tweezing systems, and integrated nano-devices.

Plasmonic cavity-apertures as dynamic pixels for the simultaneous control of colour and intensity.

Despite steady technological progress, displays are still subject to inherent limitations in resolution improvement and pixel miniaturization because a series of colours is generally expressed by a combination of at least three primary colour pixels. Here we propose a structure comprising a metal cavity and a nanoaperture, which we refer to as a cavity-aperture, to simultaneously control the colour and intensity of transmitted light in a single pixel. The metal cavity constructs plasmonic standing waves to organize the spatial distribution of amplitudes according to wavelength, and the nanoaperture permits light with a specific wavelength and amplitude to pass through it, depending on the nanoaperature's relative position in the cavity and the polarization state of the incident light. Therefore, the cavity-aperture has the potential to function as a dynamic colour pixel. This design method may be helpful in developing various photonic devices, such as micro-imaging systems and multiplexed sensors.

Hybrid states of propagating and localized surface plasmons at silver core/silica shell nanocubes on a thin silver layer.

Hybrid characteristics of propagating surface plasmons (PSPs) and localized surface plasmons (LSPs) appear at a combined structure of a thin silver (Ag) layer and silver core/silica shell nanocubes (AgNC@SiO(2)s) in the Kretschmann configuration, because the resonant condition of PSPs on the thin Ag layer is significantly modified by LSPs of the AgNC@SiO(2)s. We investigate theoretically and experimentally that due to the hybrid property, the slope and position of the minimum reflectance band can be controlled on a graph of incident angle versus wavelength of reflected light, by changing structural parameters. The hybrid properties of PSPs and LSPs have a potential to simultaneously detect surface plasmon resonance signals and fluorescence images.

Switchable beaming from a nanoslit with metallic gratings controlled by the phase difference between incident beams.

We propose a switching method for optical beaming generated from a metal slit surrounded by surface gratings. The principle of the method is based on the interference of diffracted surface plasmon polaritons from the gratings which are controlled by the relative phases of two oblique incident beams that are illuminated on the metal slit. By adjusting the relative position of the interference pattern of the incident beams with respect to the metal slit, beaming from the proposed structure can be switched from the on- to the off-mode by virtue of the change in the symmetry of the generated surface plasmon polaritons. An experimental demonstration of the method is presented in which an electrically controlled interferometric configuration is used.

Intermediate plasmonic characteristics in a quasi-continuous metallic monolayer.

There has been a significant interest on plasmonics in a metallic structure with very narrow gaps for studies of nanophotonics. However, little attention has been paid to the behavior of surface plasmons (SPs) in quasi-continuous metallic structures. This study observes and analyzes intermediate characteristics between propagating SPs (PSPs) and localized SPs (LSPs) in a quasi-continuous metallic monolayer of core-shell nanocubes. We reveal that, in a very narrow region of few-nanometer gaps among the nanocubes, the intrinsic energy bands of PSPs and LSPs intersect each other to generate two hybrid bands and an anti-crossing. Using a self-assembly method instead of the lithographic techniques which have several limitations as of now, we materialize the quasi-continuous metallic layer with plenty of nano-gaps that exhibit intermediate plasmonic characteristics. The intermediate plasmonic characteristics observed in this study will lead to interesting subjects, such as band engineering and slow SPs, in nanophotonics.

Site-selective synthesis of silver nanoparticles in pre-patterned trenches and their localized surface plasmon resonances.

A method for depositing silver nanoparticles in a pre-patterned trench by site-selective synthesis is described. In the trench patterns with various shapes, silver nanoparticles can be selectively nucleated and grown only on polyvinylpyrrolidone (PVP) domains by attraction (or repulsion) between silver ions and the hydrophilic PVP island domains in a silica matrix of the trench (or the hydrophobic fluorosilane layer). Regarding the silver nanoparticles in the trench, localized surface plasmon resonance (LSPR) could be excited by obliquely incident light, reradiating the enhanced electromagnetic field in the far- and near-fields. Even in the case of a large angle incidence in total internal reflection (TIR), the patterned silver nanoparticle clusters underwent strong scattering with a high intensity, due to the LSPR effect.