ABSTRACT
The complex magnetic dipole plasmon couplings in double split-ring resonators are investigated. Two split peaks in the absorption spectrum of these coupled systems are observed, but even the shorter-wavelength resonance peak can be redshifted compared to the peaks of individual rings. The magnetic plasmon fields outside rings are found to play an important role in these strong couplings. Because of them, both bonding and antibonding plasmon hybridizations occur at each split peak. When bonding coupling effects are stronger than those of antibonding ones, this abnormal splitting behavior appears. When the coupling between rings becomes weaker, the splitting phenomenon tends to be normal.
ABSTRACT
We theoretically investigate the plasmon coupling in metallic nanorod dimers. A pronounced dip is found in the extinction spectrum due to plasmonic Fano resonance, which is induced by destructive interference between the bright dipole plasmon of a short nanorod and the dark quadrupole plasmon of a long nanorod. This Fano interference can also be explained as the coupling between the bright and dark modes both supported by the whole dimer. The Fano resonance can be tuned by adjusting the spatial or spectral separation between two nanorods in the dimer.
Subject(s)
Dimerization , Nanotubes/chemistry , Optical PhenomenaABSTRACT
We investigate the optical response of a gold nanorod array coupled with a semicontinuous nanoparticle film. We find that, as the gold nanoparticle film is adjusted to the percolating regime, the nanorod-film hybrids are tuned into plasmonic Fano resonance, characterized by the coherent coupling of discrete plasmonic modes of the nanorod array with the continuum band of the percolating film. Consequently, optical transmission of the percolating film is substantially enhanced. Even more strikingly, electromagnetic fields around the nanorod array become much stronger, as reflected by 2 orders of magnitude enhancement in the avalanche multiphoton luminescence. These findings may prove instrumental in the design of various plasmonic nanodevices.
ABSTRACT
Efficient plasmon-mediated excitation energy transfer between the CdSe/ZnS semiconductor quantum dots (QDs) across the silver nanowire array up to 560 nm in length is observed. The subwavelength imaging and spectral response of the silver nanowire arrays with near-field point-source excitations are revealed by theoretical simulations. Our studies demonstrate three advantages of the nanosystem: efficient exciton-plasmon conversion at the input side of the array through near-field strong coupling, directional waveguidance and resonant transmission via half-wave plasmon modes of the nanowire array, and subwavelength imaging at the output side of the array. These advantages allow a long-range radiative excitation energy transfer with a high efficiency and a good directionality.
Subject(s)
Energy Transfer , Nanotechnology/instrumentation , Nanowires/chemistry , Silver/chemistry , Absorption , Cadmium Compounds/chemistry , Quantum Dots , Selenium Compounds/chemistry , Semiconductors , Sulfides/chemistry , Zinc Compounds/chemistryABSTRACT
We propose the effective dielectric function theory of metal granular composites modified with the metal particle size. The modified theory is used to explain the electrical conductivity, resonant plasmon absorption, and large nonlinear absorption of Au-TiO2 granular composite films with high-density metallic particles and a high electric percolation threshold. It is revealed that the decreasing metal particle size leads to an increasing percolation threshold and large enhancement of optical nonlinearity of the composites.