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Phys Rev Lett ; 111(3): 036001, 2013 Jul 19.
Article in English | MEDLINE | ID: mdl-23909338

ABSTRACT

Using discontinuously rate thickening suspensions (DRTS) as a model system, we show that beads-on-a-string morphologies can arise as a result of external viscous drag acting during capillary-driven breakup of a non-Newtonian fluid. To minimize the perturbative effect of gravity, we developed a new experimental test platform in which the filament is supported in a horizontal position at the surface of an immiscible oil bath. We show that the evolution of thin DRTS filaments during the capillary thinning process is well described by a set of one-dimensional slender filament equations. The strongly rate-dependent rheology of the test fluid and the aspect ratio of the filament couple to control the thinning dynamics and lead to a simple criterion describing the localized arrest of the capillary thinning process and the subsequent formation of complex, high aspect ratio beads-on-a-string structures.


Subject(s)
Models, Theoretical , Suspensions/chemistry , Corn Oil/chemistry , Polyethylene Glycols/chemistry , Polystyrenes/chemistry , Viscosity , Water/chemistry
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