Oscillations and Cavity Modes in the Circular Hydraulic Jump.

We report spontaneous oscillations of circular hydraulic jumps created by the impact of a submillimeter water jet on a solid disk. The jet flow rate is shown to condition the occurrence of the oscillations while their period is independent of this parameter. The period, however, varies linearly with the disk radius. This dependency is rationalized by investigating surface gravity wave modes in the cavity formed by the disk. We show that the jump oscillation frequency systematically matches one of the surface wave disk-cavity eigenfrequencies, leading to the conclusion that the oscillations are self-induced by the interaction between the jump and surface wave eigenmodes.

Motion of Long Levitating Drops in Tubes in an Anti-Bretherton Configuration.

In his seminal paper, Bretherton studied the motion of long bubbles in capillary tubes. Here, we unveil the negative configuration wherein a long liquid drop is stably transported in a capillary tube and surrounded by a flow-induced air cushion. These drops are formed when a liquid plug is pushed above a critical velocity sufficient to induce an inversion of the front meniscus with a radius of curvature smaller than the tube radius. The drop shape and lubricating air film thickness is reminiscent of Bretherton's calculation and can be inferred from an adapted analytical theory.

Enhancement of Meniscus Pump by Multiple Particles.

We numerically investigate the behavior of a droplet spreading on a smooth substrate with multiple obstacles. As experimental works have indicated, the macroscopic contact line or the three-phase boundary line of a droplet exhibits significant deformation resulting in a local acceleration by successive interactions with an array of tiny obstacles settled on the substrate (Mu et al., Langmuir 2019, 35). We focus on the menisci formation and the resultant pressure and velocity fields inside a liquid film in a two-spherical-particle system to realize an optimal design for the effective liquid-transport phenomenon. Special attention is paid to the meniscus formation around the second particle, which influences the liquid supply related to the pressure difference around the first particle as a function of the distance between the two particles. We find that the meniscus around the first particle plays an additional role as the reservoir of the liquid supplied toward the second particle, which is found to enhance the total pumping effect.

Pumping effect of heterogeneous meniscus formed around spherical particle.

HYPOTHESIS: A disturbance such as a microparticle on the pathway of a spreading droplet has shown the tremendous ability to accelerate locally the motion of the macroscopic contact line (Mu et al., 2017). Although this ability has been linked to the particle-liquid interaction, the physical mechanisms behind it are still poorly understood despite its academic interest and the scope of numerous industrial applications in need of fast wetting. EXPERIMENTS: In order to better understand the mechanisms behind the particle-liquid interaction, we numerically investigate the pressure and velocity fields in the liquid film. The results are compared to experiments assessing the temporal shape variation of the liquid-film meniscus from which pressure difference around the particle is evaluated. FINDINGS: The particle-induced acceleration of the film front depends both on the shape of the meniscus that forms around the particle foot and the liquid "reservoir" in the film that can be pumped thanks to the presence of the particle. The study validates the presence of three stages of pressure difference between the upstream and downstream regions of the meniscus around the particle, which leads to the local acceleration/deceleration of the macroscopic contact line. We indicate that asymmetric meniscus around the particle foot produces a net pressure force driving liquid and accelerating the liquid-film front.

Evaluation of the hydrophobic properties of latex microspheres and Bacillus spores. Influence of the particle size on the data obtained by the MATH method (microbial adhesion to hydrocarbons).

The current experimental study investigates the influence of latex microsphere particles' size on the assessment of their hydrophilic/hydrophobic character, using the method known as "Microbial Adhesion to Hydrocarbons" (MATH). Since bacteria surfaces often change according to the environment in which they find themselves, most of the experiments here were carried out using the calibrated latex microspheres Polybeads® and Yellow-green Fluoresbrite® (Polyscience) microspheres with diameters between 0.2 µm and 4.5 µm. All the beads had a density of ˜1.05 g/cm3. The first set of experiments was performed to adapt the procedure for measurements of water contact angles to microsphere lawns. It was found that all the microspheres tested were hydrophobic, when using a water contact angle of around 110-118°. However, wide differences were observed using the MATH method. The smaller microspheres (0.2 µm, 0.5 µm +/- 0.75 µm) exhibited a poor affinity to hexadecane, even after long contact times, suggesting a hydrophilic character. In contrast, larger microspheres quickly adhered to hexadecane, which is consistent with the values obtained for the water contact angles observed. These results suggest that, at least where hydrophobic particles are concerned, the MATH method is not suitable for the assessment of the hydrophobic character of particles with diameters of less than 1.0 µm. We lastly investigated whether the data obtained for Bacillus spores could also be affected by spore size. The hydrophobicity of spores of eight Bacillus strains was analysed by both MATH and contact angle. Some discrepancies were observed between both methods but could not be related their size (length or width).

Quick Liquid Propagation on a Linear Array of Micropillars.

The wetting process of a high energy surface can be accelerated locally through the capillary interaction of a liquid advancing front with a micro-object introduced to the surface (Mu et al., J. Fluid Mech, 2017, 830, R1). We demonstrate that a linear array of micropillars embedded in a fully wettable substrate can produce quick propagation of liquid along the array. It is observed that multiple interactions of a liquid front with pillars can induce the motion of liquid a hundred times faster than in the absence of pillars.

Inverse Saffman-Taylor Experiments with Particles Lead to Capillarity Driven Fingering Instabilities.

Using air to displace a viscous fluid contained in a Hele-Shaw cell can create a fingering pattern at the interface between the fluids if the capillary number exceeds a critical value. This Saffman-Taylor instability is revisited for the inverse case of a viscous fluid displacing air when partially wettable hydrophilic particles are lying on the walls. Though the inverse case is otherwise stable, the presence of the particles results in a fingering instability at low capillary number. This capillary-driven instability is driven by the integration of particles into the interface which results from the minimization of the interfacial energy. Both axisymmetric and rectangular geometries are considered in order to quantify this phenomenon.

Increased resistance to detachment of adherent microspheres and Bacillus spores subjected to a drying step.

In various environments, including that of food processing, adherent bacteria are often subjected to drying conditions. These conditions have been shown to result in changes in the ability of biofilms to cross-contaminate food in contact with them. In this study, we investigated the consequences of a drying step on the further ability of adherent bacterial spores to resist detachment. An initial series of experiment was set up with latex microspheres as a model. A microsphere suspension was deposited on a glass slide and incubated at 25, 35 and 50°C for times ranging from 1h to 48h. By subjecting the dried slides to increasing water flow rates, we showed that both time and temperature affected the ease of microsphere detachment. Similar observations were made for three Bacillus spores despite differences in their surface properties, especially regarding their surface physicochemistry. The differences in ease of adherent spore detachment could not be clearly linked to the minor changes in spore morphology, observed after drying in various environmental conditions. In order to explain the increased interaction between spheres or spores and glass slides, the authors made several assumptions regarding the possible underlying mechanisms: the shape of the liquid bridge between the sphere and the substratum, which is greatly influenced by the hydrophilic/hydrophobic characters of both surfaces; the accumulation of soil at the liquid/air interface; the presence of trapped nano-bubbles around and/or under the sphere.

Capillary tube wetting induced by particles: towards armoured bubbles tailoring.

In this paper, we report on the strongly modified dynamics of a liquid finger pushed inside a capillary tube, when partially wettable particles are lying on the walls. Particles promote the appearance of new regimes and enable the tailored synthesis of bubbles encapsulated in a monolayer of particles (so-called "armoured bubbles"). This remarkable behavior arises due to the collection of particles at the air-liquid interface, which modify the global energy balance and stabilize the interface. Armoured-bubbles are of primary interest in industrial processes since they display increased stability, interfacial rigidity and can even sustain non-spherical shapes. This work opens perspective for a low cost bubbles-on-demand technology enabling the synthesis of armoured bubbles with specific sizes, shapes and composition.

Mixing generated by Faraday instability between miscible liquids.

The mixing between two miscible liquids subject to vertical vibrations is studied by way of experiments and a two-dimensional numerical model. The experimental setup consisted of a rectangular cell in which the lighter fluid was placed above the denser one. The diffuse interface was then visualized by a high-speed camera. After an initial period of diffusion growth, the interface becomes unstable with a defined wavelength, which depends on the amplitude and frequency of the acceleration. The waviness of the interfacial region disappears once the mixing of the two fluids takes place. The mixing is characterized by a mixing layer thickness (MLT) which measures the thickness of the mixed region between the two pure fluid domains. We find that the MLT shows an exponential growth with time due to an initial fingering that appears at the interface and then a growth with a defined slope after the mixing takes place. The MLT also increases with amplitude of driving motion. Experimentally determined MLTs are always greater than those determined by computations since the latter assume a jump discontinuity between the fluids prior to shaking, whereas in an experiment an initial diffusive region establishes itself prior to shaking and this is destabilizing. In addition, it is found from computations that mixing is best for low gravity levels at earlier times and high gravity levels at longer times. Explanations are advanced for each of these observations.

Enhancement of biosensing performance in a droplet-based bioreactor by in situ microstreaming.

A droplet-based micro-total-analysis system involving biosensor performance enhancement by integrated surface-acoustic-wave (SAW) microstreaming is shown. The bioreactor consists of an encapsulated droplet with a biosensor on its periphery, with in situ streaming induced by SAW. This paper highlights the characterization by particle image tracking of the speed distribution inside the droplet. The analyte-biosensor interaction is then evaluated by finite element simulation with different streaming conditions. Calculation of the biosensing enhancement shows an optimum in the biosensor response. These results confirm that the evaluation of the Damköhler and Peclet numbers is of primary importance when designing biosensors enhanced by streaming.