Final amplifier of an ultra-intense all-OPCPA system with 13-J output signal energy and 41% pump-to-signal conversion efficiency.

Optical parametric chirped-pulse amplification (OPCPA) using high-energy Nd:glass lasers has the potential to produce ultra-intense pulses (>1023 W/cm2). We report on the performance of the final high-efficiency amplifier in an OPCPA system based on large-aperture (63 × 63-mm2) partially deuterated potassium dihydrogen phosphate (DKDP) crystals. The seed beam (180-nm bandwidth, 110 mJ) was provided by the preceding OPCPA stages. A maximum pump-to-signal conversion efficiency of 41% and signal energy up to 13 J were achieved with a 52-mm-long DKDP crystal due to the flattop super-Gaussian pump beam profile and flat-in-time pulse shape.

Design and characterization of "flow-cell" integrated-flow active cooling for high-average-power ceramic optics.

We used COMSOL Multiphysics to design a prototype actively cooled "flow-cell" substrate targeted at high-average-power applications, fabricated the prototype from cordierite ceramic, and tested the substrate under load in our thermal loading test stand. Sub-aperture testing revealed average-power handling up to 3.88-W/cm2 absorbed power density, in excellent agreement with model predictions. Gratings fabricated on 2-in.-diam cordierite coupons were subjected to laser-damage testing and showed a damage threshold of 250 mJ/cm2.

High-efficiency, fifth-harmonic generation of a joule-level neodymium laser in a large-aperture ammonium dihydrogen phosphate crystal.

High-energy deep ultraviolet (UV) sources are required for high-density plasma diagnostics. The fifth-harmonic generation of large-aperture neodymium lasers in ammonium dihydrogen phosphate (ADP) can significantly increase UV energies due to the availability of large ADP crystals. Noncritical phase matching in ADP for (ω + 4ω) was achieved by cooling a 65 × 65-mm crystal in a two-chamber cryostat to 200 K. The crystal chamber used helium as the thermally conductive medium between the crystal and the crystal chamber, which was surrounded by a high-vacuum chamber with a liquid nitrogen reservoir. A temperature variation of 0.2 K across the crystal aperture was obtained. The total conversion efficiency from the fundamental to the fifth harmonic at 211 nm was 26%.

Advanced laser development and plasma-physics studies on the multiterawatt laser.

The multiterawatt (MTW) laser, built initially as the prototype front end for a petawatt laser system, is a 1053 nm hybrid system with gain from optical parametric chirped-pulse amplification (OPCPA) and Nd:glass. Compressors and target chambers were added, making MTW a complete laser facility (output energy up to 120 J, pulse duration from 20 fs to 2.8 ns) for studying high-energy-density physics and developing short-pulse laser technologies and target diagnostics. Further extensions of the laser support ultrahigh-intensity laser development of an all-OPCPA system and a Raman plasma amplifier. A short summary of the variety of scientific experiments conducted on MTW is also presented.

Direct-drive laser fusion: status, plans and future.

Laser-direct drive (LDD), along with laser indirect (X-ray) drive (LID) and magnetic drive with pulsed power, is one of the three viable inertial confinement fusion approaches to achieving fusion ignition and gain in the laboratory. The LDD programme is primarily being executed at both the Omega Laser Facility at the Laboratory for Laser Energetics and at the National Ignition Facility (NIF) at Lawrence Livermore National Laboratory. LDD research at Omega includes cryogenic implosions, fundamental physics including material properties, hydrodynamics and laser-plasma interaction physics. LDD research on the NIF is focused on energy coupling and laser-plasma interactions physics at ignition-scale plasmas. Limited implosions on the NIF in the 'polar-drive' configuration, where the irradiation geometry is configured for LID, are also a feature of LDD research. The ability to conduct research over a large range of energy, power and scale size using both Omega and the NIF is a major positive aspect of LDD research that reduces the risk in scaling from OMEGA to megajoule-class lasers. The paper will summarize the present status of LDD research and plans for the future with the goal of ultimately achieving a burning plasma in the laboratory. This article is part of a discussion meeting issue 'Prospects for high gain inertial fusion energy (part 2)'.

High-energy parametric amplification of spectrally incoherent broadband pulses.

We study and demonstrate the efficient parametric amplification of spectrally incoherent broadband nanosecond pulses to high energies. Signals composed of mutually incoherent monochromatic lines or amplified spontaneous emission are amplified in a sequence of optical parametric amplifiers pumped at 526.5 nm, with the last amplifier set in a collinear geometry. This configuration results in 70% conversion efficiency from the pump to the combined signal and idler, with a combined energy reaching 400 mJ and an optical spectrum extending over 60 nm around 1053 nm. The spatial, spectral, and temporal properties of the amplified waves are investigated. The demonstrated high conversion efficiency, spectral incoherence, and large bandwidth open the way to a new generation of high-energy, solid-state laser drivers that mitigate laser-plasma instabilities and laser-beam imprint via enhanced spectral bandwidth.

The Dynamic Compression Sector laser: A 100-J UV laser for dynamic compression research.

The Dynamic Compression Sector (DCS) laser is a 100-J ultraviolet Nd:glass system designed and built by the Laboratory for Laser Energetics for experimental research at the DCS located at the Advanced Photon Source (Argonne National Laboratory). Its purpose is to serve as a shock driver to study materials under extreme dynamic pressures. It was designed to deposit energy within a uniformly illuminated 500-µm spot on target, with additional optics provided to implement spot sizes of 250 and 1000 µm. Designed after larger-scale glass lasers such as OMEGA and the National Ignition Facility, the laser consists of a fiber front end with interferometer-based pulse shaping, a Nd:glass regenerative amplifier, a four-pass rod amplifier, and a 15-cm glass disk amplifier, through which six passes are made in a bowtie geometry. The output is frequency tripled from 1053 to 351 nm by using a pair of type-II phase-matched KDP crystals, with a third to increase conversion bandwidth. The super-Gaussian spot in the far field is achieved with a distributed phase plate and a 1-m aspherical focusing lens. Beam smoothing is achieved by smoothing by spectral dispersion and polarization smoothing, resulting in a root-mean-square variation in intensity on target of ±8.7%.

Tripled yield in direct-drive laser fusion through statistical modelling.

Focusing laser light onto a very small target can produce the conditions for laboratory-scale nuclear fusion of hydrogen isotopes. The lack of accurate predictive models, which are essential for the design of high-performance laser-fusion experiments, is a major obstacle to achieving thermonuclear ignition. Here we report a statistical approach that was used to design and quantitatively predict the results of implosions of solid deuterium-tritium targets carried out with the 30-kilojoule OMEGA laser system, leading to tripling of the fusion yield to its highest value so far for direct-drive laser fusion. When scaled to the laser energies of the National Ignition Facility (1.9 megajoules), these targets are predicted to produce a fusion energy output of about 500 kilojoules-several times larger than the fusion yields currently achieved at that facility. This approach could guide the exploration of the vast parameter space of thermonuclear ignition conditions and enhance our understanding of laser-fusion physics.

Chirped-pulse-amplification seed source through direct phase modulation.

This work presents integration of a directly chirped laser source (DCLS) into a high-energy optical parametric chirped-pulse-amplification (OPCPA) system. DCLS is an all-fiber, chirped laser source that produces nanosecond, linearly chirped laser pulses at 1053 nm for seeding high-energy chirped-pulse-amplification systems. DCLS produces a frequency chirp on an optical pulse through direct temporal phase modulation. A 1-ns, linearly chirped pulse with a 3-nm bandwidth is produced by applying an ~1000-rad (300π) quadratic temporal phase. The chirped pulse is amplified to 76 mJ in an OPCPA system and compressed to close to its Fourier transform limit, producing an intensity autocorrelation trace with a 1.5-ps width.

Record fifth-harmonic-generation efficiency producing 211 nm, joule-level pulses using cesium lithium borate.

The fifth harmonic of a pulsed Nd:YLF laser has been realized in a cascade of nonlinear crystals with a record efficiency of 30%. Cesium lithium borate is used in a Type-I configuration for sum-frequency mixing of 1053 and 266 nm, producing 211 nm pulses. Flat-topped beam profiles and pulse shapes optimize efficiency. The energies of the fifth harmonic up to 335 mJ in 2.4 ns pulses were demonstrated.

First Observation of Cross-Beam Energy Transfer Mitigation for Direct-Drive Inertial Confinement Fusion Implosions Using Wavelength Detuning at the National Ignition Facility.

Cross-beam energy transfer (CBET) results from two-beam energy exchange via seeded stimulated Brillouin scattering, which detrimentally reduces ablation pressure and implosion velocity in direct-drive inertial confinement fusion. Mitigating CBET is demonstrated for the first time in inertial-confinement implosions at the National Ignition Facility by detuning the laser-source wavelengths (±2.3 Å UV) of the interacting beams. We show that, in polar direct-drive, wavelength detuning increases the equatorial region velocity experimentally by 16% and alters the in-flight shell morphology. These experimental observations are consistent with design predictions of radiation-hydrodynamic simulations that indicate a 10% increase in the average ablation pressure.

Thermal effects in an ultrafast BiB3O6 optical parametric oscillator at high average powers.

An ultrafast, high-average-power, extended-cavity, femtosecond BiB3O6 optical parametric oscillator was constructed as a test bed for investigating the scalability of infrared parametric devices. Despite the high pulse energies achieved by this system, the reduction in slope efficiency near the maximum-available pump power prompted the investigation of thermal effects in the crystal during operation. The local heating effects in the crystal were used to determine the impact on both phase matching and thermal lensing to understand limitations that must be overcome to achieve microjoule-level pulse energies at high repetition rates.

High-average-power, 2-µm femtosecond optical parametric oscillator synchronously pumped by a thin-disk, mode-locked laser.

A high-energy, extended-cavity femtosecond BiBO optical parametric oscillator synchronously pumped by a 1.0-ps, 1030-nm Yb:YAG, thin-disk pump laser is presented. The oscillator operated near degeneracy in a noncollinear interaction geometry, producing signal wavelength tunability from 1.99 to 2.20 µm. The signal pulses have an average power exceeding 2 W, producing 455-fs pulses at 7.08 MHz with energies up to 350 nJ, showing increased potential for tunable sources of scalable ultrafast pulses in the infrared.

Self-phase modulation compensation in a regenerative amplifier using cascaded second-order nonlinearities.

Self-phase modulation limits the amplification of short optical pulses because of spatial self-focusing and spectral broadening. Cascaded nonlinearities are theoretically and experimentally investigated for intracavity nonlinearity compensation in a neodymium-doped yttrium-lithium-fluoride (Nd:YLF) regenerative amplifier. Experimental results are in good agreement with simulations. Spectral broadening is significantly reduced, allowing for efficient amplification in a Nd:YLF power amplifier.

X-ray streak camera cathode development and timing accuracy of the 4ω ultraviolet fiducial system at the National Ignition Facility.

The convergent ablator experiments at the National Ignition Facility (NIF) are designed to measure the peak velocity and remaining ablator mass of an indirectly driven imploding capsule. Such a measurement can be performed using an x-ray source to backlight the capsule and an x-ray streak camera to record the capsule as it implodes. The ultimate goal of this experiment is to achieve an accuracy of 2% in the velocity measurement, which translates to a ±2 ps temporal accuracy over any 300 ps interval for the streak camera. In order to achieve this, a 4ω (263 nm) temporal fiducial system has been implemented for the x-ray streak camera at NIF. Aluminum, titanium, gold, and silver photocathode materials have been tested. Aluminum showed the highest relative quantum efficiency, with five times more peak signal counts per fiducial pulse when compared to Gold. The fiducial pulse data were analyzed to determine the centroiding statistical accuracy for incident laser pulse energies of 1 and 10 nJ, showing an accuracy of ±1.6 ps and ±0.7 ps, respectively.

Time-resolved measurements of hot-electron equilibration dynamics in high-intensity laser interactions with thin-foil solid targets.

Time-resolved K(α) spectroscopy has been used to infer the hot-electron equilibration dynamics in high-intensity laser interactions with picosecond pulses and thin-foil solid targets. The measured K(α)-emission pulse width increases from ~3 to 6 ps for laser intensities from ~10(18) to 10(19) W/cm(2). Collisional energy-transfer model calculations suggest that hot electrons with mean energies from ~0.8 to 2 MeV are contained inside the target. The inferred mean hot-electron energies are broadly consistent with ponderomotive scaling over the relevant intensity range.

Analysis and suppression of parasitic processes in noncollinear optical parametric amplifiers.

The influence of parasitic processes on the performance of ultra-broadband noncollinear optical parametric amplifiers (NOPA's) is investigated for walk-off and non-walk-off compensating configurations. Experimental results with a white-light-seeded NOPA agree well with numerical simulations. The same model shows that 10% of the output energy of an amplified signal can be transferred into a parasitic second harmonic of the signal. These findings are supported by quantitative measurements on a few-cycle NOPA, where a few percent of the signal energy is converted to its second harmonic in the walk-off compensating case. This effect is reduced by an order of magnitude in the non-walk-off compensating configuration. A detailed study of the phase-matching conditions of the most common nonlinear crystals provides guidelines for designing NOPA systems.

Amplifying nanosecond optical pulses at 1053 nm with an all-fiber regenerative amplifier.

Nanosecond, 1053 nm optical pulses are amplified from 15 pJ to 240 nJ by a Yb-doped all-fiber regenerative amplifier (AFRA), achieving an overall gain of 42 dB. To the best of our knowledge, this is the highest output-pulse energy from an AFRA ever reported. Techniques for suppressing amplified spontaneous emission are employed to favor the signal gain 23 nm off the gain peak of the Yb-doped fiber. Numerical simulations show that increasing the number of round trips and operating the AFRA at saturation will increase the output level and improve the output stability. This is currently limited by the onset of bifurcation instability, which can be avoided at low repetition rates.

All-fiber optical isolator based on Faraday rotation in highly terbium-doped fiber.

An all-fiber isolator with 17 dB optical isolation is demonstrated. The fiber Faraday rotator uses 56 wt. % terbium (Tb)-doped silicate fiber, and the fiber polarizers are Corning SP1060 single-polarization fiber. The effective Verdet constant of the Tb-doped fiber is measured to be -24.5+/-1.0 rad/(Tm) at 1053 nm, which is 20 times larger than silica fiber and 22% larger than previously reported results.

Scaling hot-electron generation to high-power, kilojoule-class laser-solid interactions.

Thin-foil targets were irradiated with high-power (1 ≤ P(L) ≤ 210 TW), 10-ps pulses focused to intensities of I>10(18) W/cm(2) and studied with K-photon spectroscopy. Comparing the energy emitted in K photons to target-heating calculations shows a laser-energy-coupling efficiency to hot electrons of η(L-e) = 20 ± 10%. Time-resolved x-ray emission measurements suggest that laser energy is coupled to hot electrons over the entire duration of the incident laser drive. Comparison of the K-photon emission data to previous data at similar laser intensities shows that η(L-e) is independent of laser-pulse duration from 1 ≤ τ(p) ≤ 10 ps.