Observation of mode-mixing in the spatial eigenmodes of an optical microcavity.

We present a method to determine the complex coupling parameter of a two-coupled-modes system by directly measuring the coupled eigenmodes rather than their eigenvalues. This method is useful because mode-mixing can be observed even if frequency shifts can not be measured. It also allows to determine the complex coupling parameter, from which we conclude that the observed coupling is mainly conservative. We observe mode-mixing in an optical microcavity, where the modes couple primarily at the mirror surface, as confirmed by AFM measurements. The presented method is general and can be applied to other systems to measure mode coupling more accurately and to determine the nature of the coupling.

Microcavity resonance condition, quality factor, and mode volume are determined by different penetration depths.

The penetration depth in a distributed Bragg reflector (DBR) co-determines the resonance condition, quality factor, and mode volume of DBR-based microcavities. Recent studies have used an incomplete description of the penetration depth and incorrect equations. We present a complete analysis that involves three different penetration depths. We also present a series of experiments on microcavities to accurately determine the frequency and modal penetration depth of our DBRs and compare these results with theoretical predictions. The obtained results are relevant for anyone who models a DBR as an effective hard mirror if lengths of the order of the wavelength are relevant, as is the case for microcavities.

Observation of the Unconventional Photon Blockade.

We observe the unconventional photon blockade effect in quantum dot cavity QED, which, in contrast to the conventional photon blockade, operates in the weak coupling regime. A single quantum dot transition is simultaneously coupled to two orthogonally polarized optical cavity modes, and by careful tuning of the input and output state of polarization, the unconventional photon blockade effect is observed. We find a minimum second-order correlation g^{(2)}(0)≈0.37, which corresponds to g^{(2)}(0)≈0.005 when corrected for detector jitter, and observe the expected polarization dependency and photon bunching and antibunching; close by in parameter space, which indicates the abrupt change from phase to amplitude squeezing.

Scattering media characterization with phase-only wavefront modulation.

A new experimental approach is demonstrated to probe the scattering properties of complex media. Using phase-only modulation of the light illuminating a random scattering sample, we induce and record fluctuations in the reflected speckle patterns. Using predictions from diffusion theory, we obtain the scattering and absorption coefficients of the sample from the average change in the speckle amplitude. Our approach, which is based on interference, is in principle able to give better signal to noise ratio as compared to an intensity modulation approach. We compare our results with those obtained from a knife-edge illumination method and enhanced back-scattering cone. Our work can find application in the non-invasive study of biological specimens as well as the study of light propagation in random scattering devices like solar cells or LEDs.

Two-mode surface plasmon lasing in hexagonal arrays.

We demonstrate surface-plasmon lasing in hexagonal metal hole arrays with a semiconductor gain medium. The device can be tuned between two laser modes, with distinct wavelengths, spatial distributions, and polarization patterns, by changing the size of the optically pumped area. One of the modes exhibits a six-fold polarization pattern, while the mode observed for larger pump spots has a rotationally symmetric polarization pattern. We explain the mode tuning by the differences of in-plane and radiative out-of-plane losses of the modes. The spatial and polarization properties of the modes are conveniently described by a sum of vectorial orbital angular momentum beams with orbital, spin, and total angular momentum j=ℓ+s.

Angle resolved transmission through metal hole gratings.

We present the first angle resolved measurements of extraordinary optical transmission (EOT) through hole array gratings in a gold film. Varying the lattice spacing of the arrays and looking at higher diffraction orders, we retrieve the angular emission pattern of the constituent holes with better signal to noise ratio than with single-hole experiments. We present a method to determine separately the angular dependence of the direct and resonant contribution to EOT by using the spectral features of the diffraction orders together with an established model. The comparison of our results with the known angular transmission of a single hole in a metal film yields a good agreement for s-polarized light. Deviations are found for illumination with p-polarized light and we address the discrepancy with Coupled Mode Model calculations and Finite Difference Time Domain simulations. These measured deviations are currently not fully understood.

Purification of a single-photon nonlinearity.

Single photon nonlinearities based on a semiconductor quantum dot in an optical microcavity are a promising candidate for integrated optical quantum information processing nodes. In practice, however, the finite quantum dot lifetime and cavity-quantum dot coupling lead to reduced fidelity. Here we show that, with a nearly polarization degenerate microcavity in the weak coupling regime, polarization pre- and postselection can be used to restore high fidelity. The two orthogonally polarized transmission amplitudes interfere at the output polarizer; for special polarization angles, which depend only on the device cooperativity, this enables cancellation of light that did not interact with the quantum dot. With this, we can transform incident coherent light into a stream of strongly correlated photons with a second-order correlation value up to 40, larger than previous experimental results, even in the strong-coupling regime. This purification technique might also be useful to improve the fidelity of quantum dot based logic gates.

Surface plasmon dispersion in hexagonal, honeycomb and kagome plasmonic crystals.

We present a systematic experimental study on the optical properties of plasmonic crystals (PlC) with hexagonal symmetry. We compare the dispersion and avoided crossings of surface plasmon modes around the Γ-point of Au-metal hole arrays with a hexagonal, honeycomb and kagome lattice. Symmetry arguments and group theory are used to label the six modes and understand their radiative and dispersive properties. Plasmon-plasmon interaction are accurately described by a coupled mode model, that contains effective scattering amplitudes of surface plasmons on a lattice of air holes under 60°, 120°, and 180°. We determine these rates in the experiment and find that they are dominated by the hole-density and not on the complexity of the unit-cell. Our analysis shows that the observed angle-dependent scattering can be explained by a single-hole model based on electric and magnetic dipoles.

Scattering of guided light by a single hole in a dielectric slab.

We study the scattering of waveguided light by a single hole in a dielectric slab with FDTD simulations and investigate two scattering processes: two dimensional (2D) scattering into slab modes and three-dimensional (3D) scattering into the surroundings. We find that 2D scattering typically dominates over the 3D losses. We find important quantitative differences between the single hole scattering and the case of scattering from an infinite Mie cylinder. Additionally, we find that a hole cannot be simply modelled as a dipolar object even in the limit of small scatterers (Rayleigh approximation). This is visible from the angular dependence of the 2D scattered intensity. We discuss the relevance of our findings in the modeling of two dimensional random scattering media.

Position-Dependent Local Detection Efficiency in a Nanowire Superconducting Single-Photon Detector.

We probe the local detection efficiency in a nanowire superconducting single-photon detector along the cross-section of the wire with a far subwavelength resolution. We experimentally find a strong variation in the local detection efficiency of the device. We demonstrate that this effect explains previously observed variations in NbN detector efficiency as a function of device geometry.

Rayleigh scattering of surface plasmons by sub-wavelength holes.

We study the scattering of surface plasmons from sub-wavelength holes and find that it exhibits a stronger wavelength dependence than the traditional λ(-4) scaling found for Rayleigh scattering of light from small particles. This experimental observation is consistent with recent theoretical work and linked to the two-dimensional nature of the surface plasmon and the wavelength dependence of its spatial extent in the third dimension. The scattering cross sections are obtained with a frequency-correlation technique, which compares intensity speckle patterns observed behind various random structures of holes and recorded at different wavelengths. This powerful technique even allows us to distinguish between scattering of surface plasmons into photons and scattering into other surface plasmons.

Experimental test of theories of the detection mechanism in a nanowire superconducting single photon detector.

We report an experimental test of the photodetection mechanism in a nanowire superconducting single photon detector. Detector tomography allows us to explore the 0.8-8 eV energy range via multiphoton excitations. High accuracy results enable a detailed comparison of the experimental data with theories for the mechanism of photon detection. We show that the temperature dependence of the efficiency of the superconducting single photon detector is determined not by the critical current but by the current associated with vortex unbinding. We find that both quasiparticle diffusion and vortices play a role in the detection event.

The role of spatial and temporal modes in pulsed parametric down-conversion.

We explore spatial correlations created by stimulated pair emission in frequency degenerate parametric down-conversion from a periodically poled KTP crystal pumped by ∼2 ps duration laser pulses. The ratio of stimulated pairs over spontaneous pairs reaches as high 0.8 in the experiment. This ratio is a direct measure of the total number of modes relevant to the down-conversion process. We identify a universal curve for this ratio that accounts for the effect of the focused pump, introducing a coherence diameter r(0) related to the diffraction limited size of the pump beam in the far-field. Measurements of the spatial correlations of the PDC light for longer crystals and tight focusing conditions show that the description given in terms of a universal curve is surprisingly robust and breaks down only for a laser beam focussed to a waist smaller than 40 µm in a 2 mm long PPKTP crystal.

Surface plasmon dispersion in metal hole array lasers.

We experimentally study surface plasmon lasing in a series of metal hole arrays on a gold-semiconductor interface. The sub-wavelength holes are arranged in square arrays of which we systematically vary the lattice constant and hole size. The semiconductor medium is optically pumped and operates at telecom wavelengths (λ ~ 1.5 µm). For all 9 studied arrays, we observe surface plasmon (SP) lasing close to normal incidence, where different lasers operate in different plasmonic bands and at different wavelengths. Angle- and frequency-resolved measurements of the spontaneous emission visualizes these bands over the relevant (ω, k||) range. The observed bands are accurately described by a simple coupled-wave model, which enables us to quantify the backwards and right-angle scattering of SPs at the holes in the metal film.

Instability of higher-order optical vortices analyzed with a multi-pinhole interferometer.

Higher-order optical vortices are inherently unstable in the sense that they tend to split up in a series of vortices with unity charge. We demonstrate this vortex-splitting phenomenon in beams produced with holograms and spatial light modulators and discuss its generic and practically unavoidable nature. To analyze the splitting phenomena in detail, we use a multi-pinhole interferometer to map the combined amplitude and phase profile of the optical field. This technique, which is based on the analysis of the far-field interference pattern observed behind an opaque screen perforated with multiple pinholes, turns out to be very robust and can among others be used to study very 'dark' regions of electromagnetic fields. Furthermore, the vortex splitting provides an ultra-sensitive measurement method of unwanted scattering from holograms and other phase-changing optical elements.

Modified detector tomography technique applied to a superconducting multiphoton nanodetector.

We present an experimental method to characterize multi-photon detectors with a small overall detection efficiency. We do this by separating the nonlinear action of the multiphoton detection event from linear losses in the detector. Such a characterization is a necessary step for quantum information protocols with single and multiphoton detectors and can provide quantitative information to understand the underlying physics of a given detector. This characterization is applied to a superconducting multiphoton nanodetector, consisting of an NbN nanowire with a bowtie-shaped subwavelength constriction. Depending on the bias current, this detector has regimes with single and multiphoton sensitivity. We present the first full experimental characterization of such a detector.

Transmission processes in random patterns of subwavelength holes.

The optical transmission of random patterns of holes is believed to depend on the transmission of the independent holes only. By comparing the transmission spectra of random patterns with different densities, we show that the quasi-cylindrical wave plays an important role in the transmission of samples with large hole densities. Furthermore, we report on a speckle pattern seen in the transmission of these arrays. By studying the degree of depolarization in this speckle pattern, as a function of hole density, we are able to quantify the role of surface plasmons to the transmission.

Search for Hermite-Gauss mode rotation in cholesteric liquid crystals.

In theory, there are analogous transformations of light's spin and orbital angular momentum [Allen and Padgett, J. Mod. Opt. 54, 487 (2007)]; however, none have been observed experimentally yet. In particular, it is unknown if there exists for the orbital angular momentum of light an effect analogous to the spin angular momentum-based optical rotation; this would manifest itself as a rotation of the corresponding Hermite-Gauss mode. Here we report an experimental search for this effect in a cholesteric liquid crystal polymer, using strongly focussed, spin-orbit coupled light. We find that the relative phase velocities of the orbital modes constituting the Hermite-Gauss mode agree to within 10(-5).

Measurements of spatial coherence of partially coherent light with and without orbital angular momentum.

We study the spatial coherence of a partially coherent beam before and after being transmitted through a spiral phase plate that changes the overall orbital angular momentum of the field. The two-point coherence function is measured and directly visualized on a CCD through interference in a Mach-Zehnder interferometer equipped with an image rotator. We show, in particular, how the coherence singularities associated with Airy rings are strongly affected by the spiral phase plate.

Observation of two-photon speckle patterns.

We report the observation of speckle patterns in quantum correlations within light that is scattered by a disordered medium. The random medium is illuminated with spatially entangled photon pairs, and fourth-order speckle patterns are spatially resolved by two independently scanning detectors. Spatial entanglement gives two-photon speckle a much richer structure than ordinary one-photon speckle. Our experiments demonstrate that two-photon speckle from a surface scatterer and a volume scatterer look entirely different.