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1.
Phys Rev Lett ; 122(9): 096401, 2019 Mar 08.
Artículo en Inglés | MEDLINE | ID: mdl-30932511

RESUMEN

We measure the quasiparticle weight in the heavy-fermion compound CeCu_{6-x}Au_{x} (x=0, 0.1) by time-resolved terahertz spectroscopy for temperatures from 2 up to 300 K. This method distinguishes contributions from the heavy Kondo band and from the crystal-electric-field satellite bands by different terahertz response delay times. We find that the formation of heavy bands is controlled by an exponentially enhanced, high-energy Kondo scale once the crystal-electric-field states become thermally occupied. We corroborate these observations by temperature-dependent dynamical mean-field calculations for the multiorbital Anderson lattice model and discuss consequences for quantum-critical scenarios.

2.
J Phys Condens Matter ; 22(16): 164203, 2010 Apr 28.
Artículo en Inglés | MEDLINE | ID: mdl-21386409

RESUMEN

We propose a new criterion for distinguishing the Hertz-Millis (HM) and the local quantum critical (LQC) mechanism in heavy-fermion systems with a magnetic quantum phase transition (QPT). The criterion is based on our finding that the complete spin screening of Kondo ions can be suppressed by the Ruderman-Kittel-Kasuya-Yosida (RKKY) coupling to the surrounding magnetic ions even without magnetic ordering and that, consequently, the signature of this suppression can be observed in spectroscopic measurements above the magnetic ordering temperature. We apply the criterion to high-resolution photoemission measurements on CeCu(6 - x)Au(x) and conclude that the QPT in this system is dominated by the LQC scenario.

3.
Phys Rev Lett ; 101(26): 266404, 2008 Dec 31.
Artículo en Inglés | MEDLINE | ID: mdl-19437657

RESUMEN

A quantum phase transition in a heavy-fermion compound may destroy the Fermi-liquid ground state. However, the conditions for this breakdown have remained obscure. We report the first direct investigation of heavy quasiparticle formation and breakdown in the canonical system CeCu(6-x)Au(x) by ultraviolet photoemission spectroscopy at elevated temperatures without the complications of lattice coherence. Surprisingly, the single-ion Kondo energy scale T(K) exhibits an abrupt step near the quantum critical Au concentration of x(c) = 0.1. We show theoretically that this step is expected from a highly nonlinear renormalization of the local spin coupling at each Ce site, induced by spin fluctuations on neighboring sites. It provides a general high-temperature indicator for heavy-fermion quasiparticle breakdown at a quantum phase transition.

4.
Phys Rev Lett ; 96(1): 019701; discussion 019702, 2006 Jan 13.
Artículo en Inglés | MEDLINE | ID: mdl-16486534
5.
Phys Rev Lett ; 90(7): 076804, 2003 Feb 21.
Artículo en Inglés | MEDLINE | ID: mdl-12633260

RESUMEN

We consider electron transport through a quantum dot described by the Kondo model in the regime of large transport voltage V in the presence of a magnetic field B with max((V,B)>>T(K). The electric current I and the local magnetization M are found to be universal functions of V/T(K) and B/T(K), where T(K) is the equilibrium Kondo temperature. We present a generalization of the perturbative renormali-zation group to frequency dependent coupling functions, as necessitated by the structure of bare perturbation theory. We calculate I and M within a poor man's scaling approach and find excellent agreement with experiment.

6.
Phys Rev Lett ; 89(23): 236402, 2002 Dec 02.
Artículo en Inglés | MEDLINE | ID: mdl-12485023

RESUMEN

How are the properties of a metal changed by strong inelastic scattering? We investigate this question within the two-dimensional t-J model using extended dynamical mean field theory and a generalized noncrossing approximation. Short-ranged antiferromagnetic fluctuations lead to a strongly incoherent single particle dynamics, large entropy, and resistance. Close to the Mott transition at low hole doping a pseudogap opens, accompanied by a drop in resistivity and an increase in the Hall constant for both lower temperatures T and doping levels. The behavior obtained bears surprising similarity to properties of the cuprates.

7.
Phys Rev Lett ; 88(17): 176803, 2002 Apr 29.
Artículo en Inglés | MEDLINE | ID: mdl-12005774

RESUMEN

It is shown that in resistive nanowires out of equilibrium containing either single- or two-channel Kondo impurities the distribution function f(E,U) obeys scaling behavior in terms of the quasiparticle energy E and the bias voltage U. The numerically calculated f(E,U) curves explain quantitatively recent experiments on Cu and Au nanowires. The systematics of the impurity concentration c(imp) extracted from the comparison between theory and results on various Cu and Au samples strongly suggests that in these systems the scaling arises from magnetic Kondo impurities.

8.
Phys Rev Lett ; 87(15): 156802, 2001 Oct 08.
Artículo en Inglés | MEDLINE | ID: mdl-11580717

RESUMEN

We examine the properties of a dc-biased quantum dot in the Coulomb blockade regime. For voltages V that are large compared to the Kondo temperature T(K), the physics is governed by the scales V and gamma, where gamma approximately V/ln(2)(V/T(K)) is the nonequilibrium decoherence rate induced by the voltage-driven current. Based on scaling arguments, self-consistent perturbation theory, and perturbative renormalization group, we argue that due to the large gamma the system can be described by renormalized perturbation theory in 1/ln(V/T(K))<<1. However, in certain variants of the Kondo problem, two-channel Kondo physics is induced by a large voltage V.

9.
Phys Rev Lett ; 87(10): 106401, 2001 Sep 03.
Artículo en Inglés | MEDLINE | ID: mdl-11531493

RESUMEN

We present high-resolution photoemission spectroscopy studies on the Kondo resonance of the strongly correlated Ce system CeCu2Si2. By exploiting the thermal broadening of the Fermi edge we analyze position, spectral weight, and temperature dependence of the low-energy 4f spectral features, whose major weight lies above the Fermi level E(F). We also present theoretical predictions based on the single-impurity Anderson model using an extended noncrossing approximation, including all spin-orbit and crystal field splittings of the 4f states. The excellent agreement between theory and experiment provides strong evidence that the spectral properties of CeCu2Si2 can be described by single-impurity Kondo physics down to T approximately 5 K.

10.
Phys Rev Lett ; 85(12): 2557-60, 2000 Sep 18.
Artículo en Inglés | MEDLINE | ID: mdl-10978106

RESUMEN

The conduction electron density of states nearby single magnetic impurities, as measured recently by scanning tunneling microscopy (STM), is calculated, taking into account tunneling into conduction electron states only. The Kondo effect induces a narrow Fano resonance in the conduction electron density of states. The line shape varies with the distance between STM tip and impurity, in qualitative agreement with experiments, but is very sensitive to details of the band structure. For a Co impurity the experimentally observed width and shift of the Kondo resonance are in accordance with those obtained from a combination of band structure and strongly correlated calculations.

13.
Phys Rev Lett ; 73(14): 1967-1970, 1994 Oct 03.
Artículo en Inglés | MEDLINE | ID: mdl-10056934
15.
Phys Rev B Condens Matter ; 47(17): 11093-11096, 1993 May 01.
Artículo en Inglés | MEDLINE | ID: mdl-10005243
16.
Phys Rev B Condens Matter ; 46(3): 1332-1337, 1992 Jul 15.
Artículo en Inglés | MEDLINE | ID: mdl-10003772
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