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We report superconducting anisotropy measurements in the electron-doped high-Tc superconductors (HTSCs) Pr(2-x)Ce(x)C(u)O(4-y) (PCCO, x = 0.15 and 0.17) with an applied magnetic field (H0) up to 28 T. Our results show that the upper critical field [H(c2)(T)] of PCCO is highly anisotropic and as the temperature T â 0, the value of it at H0 ⥠c [H(c2,â¥c)(0)] is far less than the Pauli limit. The low temperature anisotropic character of PCCO is found to be rather similar to that of hole-doped cuprate HTSCs, but apparently larger than that of typical Fe-based superconductors. This study also proves a new sensitive probe of detecting rich properties of unconventional superconductors with the use of the resonant frequency of an NMR probe circuit.
RESUMEN
In contrast with the simultaneous structural and magnetic first order phase transition T0 previously reported, our detailed investigation on an underdoped Ba(0.84)K(0.16)Fe2As2 single crystal unambiguously revealed that the transitions are not concomitant. The tetragonal (τ: I4/mmm)-orthorhombic (Ï: Fmmm) structural transition occurs at T(S)≃110 K, followed by an adjacent long-range antiferromagnetic (AFM) transition at T(N)≃102 K. Hysteresis and coexistence of the τ and Ï phases over a finite temperature range observed by NMR experiments confirm the first order character of the τ-Ï transition and provide evidence that both T(S) and T(N) are strongly correlated. Our data also show that superconductivity develops in the Ï phase below T(c)=20 K and coexists with AFM. This new observation, T(S)≠T(N), firmly establishes another similarity between the hole-doped BaFe2As2 and the electron-doped iron-arsenide superconductors.
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The transition metal (TM) chalcogenides of the form TMX(2) (X = S or Se) have been studied for decades due to their interesting electronic and magnetic properties such as metamagnetism and metal-insulator transitions. In particular, the Co(1-x)Fe(x)S(2) alloys were the subject of investigation in the 1970s due to general interest in itinerant ferromagnetism. In recent years (2000-present) it has been shown, both by electronic structure calculations and detailed experimental investigations, that Co(1-x)Fe(x)S(2) is a model system for the investigation of highly spin polarized ferromagnetism. The radically different electronic properties of the two endpoint compounds (CoS(2) is a narrow bandwidth ferromagnetic metal, while FeS(2) is a diamagnetic semiconductor), in a system forming a substitutional solid solution allows for composition control of the Fermi level relative to the spin split bands, and therefore composition-controlled conduction electron spin polarization. In essence, the recent work has shown that the concept of 'band engineering' can be applied to half-metallic ferromagnets and that high spin polarization can be deliberately engineered. Experiments reveal tunability in both sign and magnitude of the spin polarization at the Fermi level, with maximum values obtained to date of 85% at low temperatures. In this paper we review the properties of Co(1-x)Fe(x)S(2) alloys, with an emphasis on properties of relevance to half-metallicity. Crystal structure, electronic structure, synthesis, magnetic properties, transport properties, direct probes of the spin polarization, and measurements of the total density of states at the Fermi level are all discussed. We conclude with a discussion of the factors that influence, or even limit, the spin polarization, along with a discussion of opportunities and problems for future investigation, particularly with regard to fundamental studies of spintronic devices.
RESUMEN
Highly spin polarized (SP) and half-metallic ferromagnetic systems are of considerable current interest and of potential importance for spintronic applications. Recent work has demonstrated that Co1-xFexS2 is a highly polarized ferromagnet (FM) where the spin polarization can be tuned by alloy composition. Using 59Co FM-NMR as a probe, we have measured the low-temperature spin relaxation in this system in magnetic fields from 0 to 1.0 T for 0
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A resistively detected NMR technique was used to probe the two-dimensional electron gas in a GaAs/AlGaAs quantum well. The spin-lattice relaxation rate (1/T(1)) was extracted at near complete filling of the first Landau level by electrons. The nuclear spin of (75)As is found to relax much more efficiently with T --> 0 and when a well developed quantum Hall state with R(xx) approximately 0 occurs. The data show a remarkable correlation between the nuclear spin relaxation and localization. This suggests that the magnetic ground state near complete filling of the first Landau level may contain a lattice of topological spin texture, i.e., a Skyrmion crystal.
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59Co NMR measurements on La1-xSrxCoO3 reported here establish unequivocally, for the first time, the coexistence of ferromagnetic regions, spin-glass regions, and hole-poor low spin regions at all x values from 0.1 to 0.5. A zero external field NMR spectrum, which is assigned to the ferromagnetic regions, has a spectral shape that is nearly x independent at 1.9 K, as are the relaxation times, T1 and T2. The integrated spectral area increases rapidly with x up to x = 0.2 and then decreases slightly for larger x. In a field of 9.97 T, a narrow NMR line is observed at 102 MHz, identical to that found in x = 0 samples in previous work. The integrated intensity of this spectrum decreases rapidly with increasing x, and is ascribed to hole-poor low spin regions. Beneath this spectrum, a third broad line, with a peak at 100 MHz, is assigned to a spin- or cluster-glass-like phase.
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We report the spin Knight shift (K(s)) and the nuclear spin-lattice relaxation rate (1/T1) in the vortex state as a function of magnetic field (H) up to 28 T in the high-Tc superconductor TlSr2CaCu2O6.8 (Tc = 68 K). At low temperatures well below Tc, both K(s) and 1/T1 measured around the middle point between the two nearest vortices (saddle point) increase substantially with increasing field, which indicate that the quasiparticle states with an ungapped spectrum are extended outside the vortex cores in a d-wave superconductor. The density of states (DOS) around the saddle point is found to be kappaN(0)square root[H/H(c2)], with kappa = 0.5-0.7 and N0 being the normal-state DOS.
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Puzzling aspects of high-transition-temperature (high-Tc) superconductors include the prevalence of magnetism in the normal state and the persistence of superconductivity in high magnetic fields. Superconductivity and magnetism generally are thought to be incompatible, based on what is known about conventional superconductors. Recent results, however, indicate that antiferromagnetism can appear in the superconducting state of a high-Tc superconductor in the presence of an applied magnetic field. Magnetic fields penetrate a superconductor in the form of quantized flux lines, each of which represents a vortex of supercurrents. Superconductivity is suppressed in the core of the vortex and it has been suggested that antiferromagnetism might develop there. Here we report the results of a high-field nuclear-magnetic-resonance (NMR) imaging experiment in which we spatially resolve the electronic structure of near-optimally doped YBa2Cu3O7-delta inside and outside vortex cores. Outside the cores, we find strong antiferromagnetic fluctuations, whereas inside we detect electronic states that are rather different from those found in conventional superconductors.