Creation and characterization of free-standing cryogenic targets for laser-driven ion acceleration.

A technique for the creation of free-standing cryogenic targets for laser-driven ion acceleration is presented, which allows us to create solid state targets consisting of initially gaseous materials. In particular, the use of deuterium and the methods for its preparation as a target material for laser-driven ion acceleration are discussed. Moving in the phase diagram through the liquid phase leads to the substance covering an aperture on a cooled copper frame where it is solidified through further cooling. An account of characterization techniques for target thickness is given, with a focus on deducing thickness values from distance values delivered by chromatic confocal sensors.

Pre-plasma formation in experiments using petawatt lasers.

We used time-resolved shadowgraphy to characterize the pre-plasma formation in solid-target interaction experiments with micrometer-scale accuracy. We performed quantitative measurements of the plasma density for amplified spontaneous emission (ASE) levels ranging from 2 · 10(-7) to 10(-10) backed with 2-dimensional hydrodynamic simulations. We find that ASE levels above 10(-9) are able to create a significant pre-plasma plume that features a plasma canal driving a self-focusing of the laser beam. For ASE levels of 10(-10), no ASE pre-plasma could be detected.

Structure and dynamics in protic ionic liquids: a combined optical Kerr-effect and dielectric relaxation spectroscopy study.

The structure and dynamics of ionic liquids (ILs) are unusual due to the strong interactions between the ions and counter ions. These microscopic properties determine the bulk transport properties critical to applications of ILs such as advanced fuel cells. The terahertz dynamics and slower relaxations of simple alkylammonium nitrate protic ionic liquids (PILs) are here studied using femtosecond optical Kerr-effect spectroscopy, dielectric relaxation spectroscopy, and terahertz time-domain spectroscopy. The observed dynamics give insight into more general liquid behaviour while comparison with glass-forming liquids reveals an underlying power-law decay and relaxation rates suggest supramolecular structure and nanoscale segregation.

Terahertz near-field microscopy of complementary planar metamaterials: Babinet's principle.

Using terahertz near-field imaging we experimentally investigate the resonant electromagnetic field distributions behind a split-ring resonator and its complementary structure with sub-wavelength spatial resolution. For the out-of-plane components we experimentally verify complementarity of electric and magnetic fields as predicted by Babinet's principle. This duality of near-fields can be used to indirectly map resonant magnetic fields close to metallic microstructures by measuring the electric fields close to their complementary analogues which is particularly useful since magnetic near-fields are still extremely difficult to access in the THz regime. We find excellent agreement between the results from theory, simulation and two different experimental near-field techniques.

Terahertz near-field microscopy with subwavelength spatial resolution based on photoconductive antennas.

Imaging and sensing applications based on pulsed terahertz radiation have opened new possibilities for scientific and industrial applications. Many exploit the unique features of the terahertz (THz) spectral region, where common packaging materials are transparent and many chemical compounds show characteristic absorptions. Because of their diffraction limit, THz far-field imaging techniques lack microscopic resolution and, if subwavelength features have to be resolved, near-field techniques are required. Here, we present a THz near-field microscopy approach based on photoconductive antennas as the THz emitter and as a near-field probe. Our system allows us to measure amplitude, phase, and polarization of the electric fields in the vicinity of a sample with a spatial resolution on the micrometer scale (approximately lambda/20). Using a dielectric (plant leaf) and a metallic structure (microwire) as examples, we demonstrate the capabilities of our approach.

Chemical sensing and imaging with pulsed terahertz radiation.

Over the past decade, terahertz spectroscopy has evolved into a versatile tool for chemically selective sensing and imaging applications. In particular, the potential to coherently generate and detect short, and hence, broadband terahertz pulses led to the development of efficient and compact spectrometers for this interesting part of the electromagnetic spectrum, where common packaging materials are transparent and many chemical compounds show characteristic absorptions. Although early proof-of-principle demonstrations have shown the great potential of terahertz spectroscopy for sensing and imaging, the technology still often lacks the required sensitivity and suffers from its intrinsically poor spatial resolution. In this review we discuss the current potential of terahertz pulse spectroscopy and highlight recent technological advances geared towards both enhancing spectral sensitivity and increasing spatial resolution.