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1.
Sensors (Basel) ; 24(13)2024 Jun 21.
Artículo en Inglés | MEDLINE | ID: mdl-39000824

RESUMEN

Quantitative optical gas imaging (QOGI) system can rapidly quantify leaks detected by optical gas imaging (OGI) cameras across the oil and gas supply chain. A comprehensive evaluation of the QOGI system's quantification capability is needed for the successful adoption of the technology. This study conducted single-blind experiments to examine the quantification performance of the FLIR QL320 QOGI system under near-field conditions at a pseudo-realistic, outdoor, controlled testing facility that mimics upstream and midstream natural gas operations. The study completed 357 individual measurements across 26 controlled releases and 71 camera positions for release rates between 0.1 kg Ch4/h and 2.9 kg Ch4/h of compressed natural gas (which accounts for more than 90% of typical component-level leaks in several production facilities). The majority (75%) of measurements were within a quantification factor of 3 (quantification error of -67% to 200%) with individual errors between -90% and 831%, which reduced to -79% to +297% when the mean of estimates of the same controlled release from multiple camera positions was considered. Performance improved with increasing release rate, using clear sky as plume background, and at wind speeds ≤1 mph relative to other measurement conditions.

2.
Environ Sci Technol ; 2024 Feb 05.
Artículo en Inglés | MEDLINE | ID: mdl-38314689

RESUMEN

Most jurisdictions around the globe use leak detection and repair (LDAR) programs to find and fix methane leaks from oil and gas operations. In this work, we empirically evaluate the efficacy of LDAR programs using a large-scale, bottom-up, randomized controlled field experiment across ∼200 oil and gas sites in Red Deer, Canada. We find that tanks are the single largest source of emissions, contributing to nearly 60% of the total emissions. The average number of leaks at treatment sites that underwent repair reduced by ∼50% compared to the control sites. Although control sites did not see a reduction in the number of leaks, emissions reduced by approximately 36%, suggesting potential impact of routine maintenance activities to find and fix large leaks. By tracking tags on leaking equipment over time, we find a high degree of persistence; leaks that are repaired remain fixed in follow-up surveys, while non-repaired leaks remain emitting at a similar rate, suggesting that any increase in observed leak emissions following LDAR surveys are likely from new leaks. Our results show that a focus on equipment and sites that are prone to high emissions, such as tanks and oil sites, is key to cost-effective mitigation.

3.
Environ Sci Technol ; 58(2): 1088-1096, 2024 Jan 16.
Artículo en Inglés | MEDLINE | ID: mdl-38165830

RESUMEN

Methane emissions from oil and gas operations exhibit skewed distributions. New technologies such as aerial-based leak detection surveys promise cost-effective detection of large emitters (greater than 10 kg/h). Recent policies such as the US Environmental Protection Agency (EPA) methane rule that allow the use of new technologies as part of leak detection and repair (LDAR) programs require a demonstration of equivalence with existing optical gas imaging (OGI) based LDAR programs. In this work, we illustrate the impact of emission size distribution on the equivalency condition between the OGI and site-wide survey technologies. Emission size distributions compiled from aerial measurements include significantly more emitters between 1 and 10 kg/h and lower average emission rates for large emitters compared to the emission distribution in the EPA rule. As a result, we find that equivalence may be achieved at lower site-wide survey frequencies when using technologies with detection thresholds below 10 kg/h, compared to the EPA rule. However, equivalence cannot be achieved with a detection threshold of 30 kg/h at any survey frequency, because most emitters across most US basins exhibit emission rates below 30 kg/h. We find that equivalence is a complex tradeoff among technology choice, design of LDAR programs, and survey frequency that can have more than one unique solution set.


Asunto(s)
Contaminantes Atmosféricos , Metano , Estados Unidos , Metano/análisis , Monitoreo del Ambiente/métodos , United States Environmental Protection Agency , Gas Natural/análisis , Contaminantes Atmosféricos/análisis
4.
Environ Sci Technol ; 57(32): 11823-11833, 2023 08 15.
Artículo en Inglés | MEDLINE | ID: mdl-37506319

RESUMEN

Government policies and corporate strategies aimed at reducing methane emissions from the oil and gas sector increasingly rely on measurement-informed, site-level emission inventories, as conventional bottom-up inventories poorly capture temporal variability and the heavy-tailed nature of methane emissions. This work is based on an 11-month methane measurement campaign at oil and gas production sites. We find that operator-level top-down methane measurements are lower during the end-of-project phase than during the baseline phase. However, gaps persist between end-of-project top-down measurements and bottom-up site-level inventories, which we reconcile with high-frequency data from continuous monitoring systems (CMS). Specifically, we use CMS to (i) validate specific snapshot measurements and determine how they relate to the temporal emission profile of a given site and (ii) create a measurement-informed, site-level inventory that can be validated with top-down measurements to update conventional bottom-up inventories. This work presents a real-world demonstration of how to reconcile CMS rate estimates and top-down snapshot measurements jointly with bottom-up inventories at the site level. More broadly, it demonstrates the importance of multiscale measurements when creating measurement-informed, site-level emission inventories, which is a critical aspect of recent regulatory requirements in the Inflation Reduction Act, voluntary methane initiatives such as the Oil and Gas Methane Partnership 2.0, and corporate strategies.


Asunto(s)
Contaminantes Atmosféricos , Metano , Metano/análisis , Gas Natural/análisis , Contaminantes Atmosféricos/análisis
5.
Environ Sci Technol ; 56(20): 14743-14752, 2022 10 18.
Artículo en Inglés | MEDLINE | ID: mdl-36201663

RESUMEN

Methane mitigation from the oil and gas (O&G) sector represents a key near-term global climate action opportunity. Recent legislation in the United States requires updating current methane reporting programs for oil and gas facilities with empirical data. While technological advances have led to improvements in methane emissions measurements and monitoring, the overall effectiveness of mitigation strategies rests on quantifying spatially and temporally varying methane emissions more accurately than the current approaches. In this work, we demonstrate a quantification, monitoring, reporting, and verification framework that pairs snapshot measurements with continuous emissions monitoring systems (CEMS) to reconcile measurements with inventory estimates and account for intermittent emission events. We find that site-level emissions exhibit significant intraday and daily emission variations. Snapshot measurements of methane can span over 3 orders of magnitude and may have limited application in developing annualized inventory estimates at the site level. Consequently, while official inventories underestimate methane emissions on average, emissions at individual facilities can be higher or lower than inventory estimates. Using CEMS, we characterize distributions of frequency and duration of intermittent emission events. Technologies that allow high sampling frequency such as CEMS, paired with a mechanistic understanding of facility-level events, are key to an accurate accounting of short-duration, episodic, and high-volume events that are often missed in snapshot surveys and to scale snapshot measurements to annualized emissions estimates.


Asunto(s)
Contaminantes Atmosféricos , Gas Natural , Contaminantes Atmosféricos/análisis , Metano/análisis , Gas Natural/análisis , Sulfuros , Estados Unidos , United States Environmental Protection Agency
6.
Environ Sci Technol ; 56(20): 14734-14742, 2022 10 18.
Artículo en Inglés | MEDLINE | ID: mdl-36174099

RESUMEN

Coal-to-gas switching in the power sector, as happening in the U.S., has been a key driver of near-term greenhouse gas emissions reductions. Can this success be replicated around the world? Here, we explore the limits of a global, plant-level, coal-to-gas transition arising from pipeline availability constraints. Globally, only 43% of coal capacity is within 14 km of a nearby pipeline, the median distance for recent coal-to-gas conversions. Furthermore, plant-to-pipeline distance distributions vary widely-only 30% of coal capacity in India is within 14 km of a nearby pipeline. Most global coal fleets are in the intermediate space of balancing two competing interests-having a young coal fleet with high "avoided" emissions potential through coal-to-gas switching but without access to low-cost gas resources. A global stocktake based on coal fleet age, pipeline access, and natural gas supply security suggests that a coal-to-gas transition in the power sector is unlikely to be a universal climate solution.


Asunto(s)
Gases de Efecto Invernadero , Gas Natural , Carbón Mineral , Estudios de Factibilidad , India , Gas Natural/análisis , Centrales Eléctricas
7.
Nat Energy ; 7(6): 465-467, 2022.
Artículo en Inglés | MEDLINE | ID: mdl-35637743

RESUMEN

The European Union's plan to phase out Russian natural gas imports by 2027 rests partly on increasing near-term imports of US liquefied natural gas. This will require a coordinated policy response that includes securing supplies from major exporters, global diplomacy, expanding import capacity, and alignment with Europe's climate goals.

8.
Nat Commun ; 12(1): 4715, 2021 08 05.
Artículo en Inglés | MEDLINE | ID: mdl-34354066

RESUMEN

Methane (CH4) emissions from oil and natural gas (O&NG) systems are an important contributor to greenhouse gas emissions. In the United States, recent synthesis studies of field measurements of CH4 emissions at different spatial scales are ~1.5-2× greater compared to official greenhouse gas inventory (GHGI) estimates, with the production-segment as the dominant contributor to this divergence. Based on an updated synthesis of measurements from component-level field studies, we develop a new inventory-based model for CH4 emissions, for the production-segment only, that agrees within error with recent syntheses of site-level field studies and allows for isolation of equipment-level contributions. We find that unintentional emissions from liquid storage tanks and other equipment leaks are the largest contributors to divergence with the GHGI. If our proposed method were adopted in the United States and other jurisdictions, inventory estimates could better guide CH4 mitigation policy priorities.

9.
Environ Sci Technol ; 55(14): 9711-9720, 2021 07 20.
Artículo en Inglés | MEDLINE | ID: mdl-34254796

RESUMEN

Natural gas (NG) produced in Western Canada is a major and growing source of Canada's energy and greenhouse gas (GHG) emissions portfolio. Despite recent progress, there is still only limited understanding of the sources and drivers of Western Canadian greenhouse gas (GHG) emissions. We conduct a case study of a production facility based on Seven Generation Energy Ltd.'s Western Canadian operations and an upstream NG emissions intensity model. The case study upstream emissions intensity is estimated to be 3.1-4.0 gCO2e/MJ NG compared to current best estimates of British Columbia (BC) emissions intensities of 6.2-12 gCO2e/MJ NG and a US average estimate of 15 gCO2e/MJ. The analysis reveals that compared to US studies, public GHG emissions data for Western Canada is insufficient as current public data satisfies only 50% of typical LCA model inputs. Company provided data closes most of these gaps (∼80% of the model inputs). We recommend more detailed data collection and presentation of government reported data such as a breakdown of vented and fugitive methane emissions by source. We propose a data collection template to facilitate improved GHG emissions intensity estimates and insight about potential mitigation strategies.


Asunto(s)
Gases de Efecto Invernadero , Gas Natural , Animales , Colombia Británica , Efecto Invernadero , Estadios del Ciclo de Vida , Gas Natural/análisis
10.
Environ Sci Technol ; 55(13): 9140-9149, 2021 07 06.
Artículo en Inglés | MEDLINE | ID: mdl-34105958

RESUMEN

Reducing methane emissions from oil and gas systems is a central component of US and international climate policy. Leak detection and repair (LDAR) programs using optical gas imaging (OGI)-based surveys are routinely used to mitigate fugitive emissions or leaks. Recently, new technologies and platforms such as planes, drones, and satellites promise more cost-effective mitigation than existing approaches. To be approved for use in LDAR programs, new technologies must demonstrate emissions mitigation equivalent to existing approaches. In this work, we use the FEAST modeling tool to (a) identify cost vs mitigation trade-offs that arise from using new technologies and (b) provide a framework for effective design of alternative LDAR programs. We identify several critical insights. First, LDAR programs can trade sensitivity for speed without sacrificing mitigation outcomes. Second, low sensitivity or high detection threshold technologies have an effective upper bound on achievable mitigation that is independent of the survey frequency. Third, the cost effectiveness of tiered LDAR programs using site-level detection technologies depends on their ability to distinguish leaks from routine venting. Finally, "technology equivalence" based on mitigation outcomes differs across basins and should be evaluated independently. The FEAST model will enable operators and regulators to systematically evaluate new technologies in next-generation LDAR programs.


Asunto(s)
Monitoreo del Ambiente , Metano , Metano/análisis , Políticas
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