2-µm Brillouin laser based on infrared nonlinear glass fibers.

Infrared fiber materials such as chalcogenide, tellurite, and heavily germanium-doped silica glasses are attractive materials for many applications based on nonlinear optical effects such as Kerr, Raman, and Brillouin processes. Here, we experimentally demonstrate a close-to-single-frequency Brillouin fiber laser in the 2-µm wavelength region either based on tellurite (TeO2) glass or on heavily germanium-doped silica glass. Our results reveal a strong enhancement of the Brillouin gain efficiency at 2 µm of more than 50 times that of standard silica optical fibers. A lasing threshold and narrow linewidth of 98 mW and 48 kHz, respectively, have been demonstrated in the tellurite fiber-based laser. This simple Brillouin laser source configuration confirms the potential applications of such fibers for the development of nonlinear photonic devices in the important 2-µm spectral range.

Core-clad phosphate glass fibers for biosensing.

Recently, a phosphate glass with composition 20 CaO-20 SrO-10 Na2O-50 P2O5 (mol%) was found to have good potential as a biomaterial and to possess thermal properties suitable for fiber drawing. This study opened the path towards the development of fully bioresorbable fibers promising for biosensing. In the past, this phosphate glass with CeO2 was found to increase the refractive index and the glass stability. Therefore, a new SrO-containing glass was prepared with 1 mol% of CeO2 and core fibers were drawn from it. A core-clad fiber was also processed, where the core was a Ce-doped glass and the clad undoped, to allow for total internal reflection. The mechanical properties of the core and core-clad fibers are discussed as a function of immersion time in TRIS-buffer solution. Finally, a sensing region was created, in the core-clad fiber, by etching the cladding using phosphoric acid. Then, the change in light transmission, upon immersion in TRIS-buffer solution, was quantified to assess the potential use of the novel core-clad fiber as a biosensor. Upon immersion in TRIS, the core-clad fiber was found to guide light effectively and to maintain a tensile strength of ~150-200 MPa up to 6 weeks in TRIS, clearly showing that this fiber has potential as a biosensing device.

Impact of optical and structural aging in As2S3 microstructured optical fibers on mid-infrared supercontinuum generation.

We analyze optical and structural aging in As2S3 microstructured optical fibers (MOFs) that may have an impact on mid-infrared supercontinuum generation. A strong alteration of optical transparency at the fundamental OH absorption peak is measured for high-purity As2S3 MOF stored in atmospheric conditions. The surface evolution and inherent deviation of corresponding chemical composition confirm that the optical and chemical properties of MOFs degrade upon exposure to ambient conditions because of counteractive surface process. This phenomenon substantially reduces the optical quality of the MOFs and therefore restrains the spectral expansion of generated supercontinuum. This aging process is well confirmed by the good matching between previous experimental results and the reported numerical simulations based on the generalized nonlinear Schrödinger equation.

Multioctave midinfrared supercontinuum generation in suspended-core chalcogenide fibers.

An As2S3 fiber-based supercontinuum source that covers 3500 nm, extending from near visible to the midinfrared, is successfully reported by using a 200-fs-pulsed pump with nJ-level energy at 2.5 µm. The main features of our fiber-based source are two-fold. On the one hand, a low-loss As2S3 microstructured optical fiber has been fabricated, with typical attenuation below 2 dB/m in the 1-4 µm wavelength range. On the other hand, a 20-mm-long microstructured fiber sample is sufficient to enable a spectral broadening, spreading from 0.6 to 4.1 µm in a 40 dB dynamic range.

Mid-infrared 2000-nm bandwidth supercontinuum generation in suspended-core microstructured sulfide and tellurite optical fibers.

In this work, we report the experimental observation of supercontinua generation in two kinds of suspended-core microstructured soft-glass optical fibers. Low loss, highly nonlinear, tellurite and As2S3 chalcogenide fibers have been fabricated and pumped close to their zero-dispersion wavelength in the femtosecond regime by means of an optical parametric oscillator pumped by a Ti:Sapphire laser. When coupled into the fibers, the femtosecond pulses result in 2000-nm bandwidth supercontinua reaching the Mid-Infrared region and extending from 750 nm to 2.8 µm in tellurite fibers and 1 µm to 3.2 µm in chalcogenide fibers, respectively.

Fourth-order cascaded Raman shift in AsSe chalcogenide suspended-core fiber pumped at 2 µm.

Cascaded Raman wavelength shifting up to the fourth order ranging from 2092 to 2450 nm is demonstrated using a nanosecond pump at 1995 nm in a low-loss As(38)Se(62) suspended-core microstructured fiber. These four Stokes shifts are obtained with a low peak power of 11 W, and only 3 W are required to obtain three shifts. The Raman gain coefficient for the fiber is estimated to (1.6±0.5)×10(-11) m/W at 1995 nm. The positions and the amplitudes of the Raman peaks are well reproduced by the numerical simulations of the nonlinear propagation.

Suppression of the frequency drift of modulational instability sidebands by means of a fiber system associated with a photon reservoir.

We analyze fiber systems where the linear losses act as a strong perturbation, causing a frequency drift of the modulational instability sidebands. We achieve the total suppression of this frequency drift by means of a technique based on the concept of a photon reservoir, which feeds in situ the process of modulational instability by continually supplying it the amount of photons absorbed by the fiber.

Low loss microstructured chalcogenide fibers for large non linear effects at 1995 nm.

Microstructured optical fibers (MOFs) are traditionally prepared using the stack and draw technique. In order to avoid the interfaces problems observed in chalcogenide glasses, we have developed a new casting method to prepare the chalcogenide preform. This method allows to reach optical losses around 0.4 dB/m at 1.55 µm and less than 0.05 dB/m in the mid IR. Various As(38)Se(62) chalcogenide microstructured fibers have been prepared in order to combine large non linear index of these glasses with the mode control offered by MOF structures. Small core fibers have been drawn to enhance the non linearities. In one of these, three Stokes order have been generated by Raman scattering in a suspended core MOF pumped at 1995 nm.

Microstructured chalcogenide optical fibers from As(2)S(3) glass: towards new IR broadband sources.

The aim of this paper is to present an overview of the recent achievements of our group in the fabrication and optical characterizations of As(2)S(3) microstructured optical fibers (MOFs). Firstly, we study the synthesis of high purity arsenic sulfide glasses. Then we describe the use of a versatile process using mechanical drilling for the preparation of preforms and then the drawing of MOFs including suspended core fibers. Low losses MOFs are obtained by this way, with background level of losses reaching less than 0.5 dB/m. Optical characterizations of these fibers are then reported, especially dispersion measurements. The feasibility of all-optical regeneration based on a Mamyshev regenerator is investigated, and the generation of a broadband spectrum between 1 µm and 2.6 µm by femto second pumping around 1.5 µm is presented.

Strong infrared spectral broadening in low-loss As-S chalcogenide suspended core microstructured optical fibers.

We report the fabrication and characterization of the first guiding chalcogenide As(2)S(3) microstructured optical fibers (MOFs) with a suspended core. At 1.55 microm, the measured losses are approximately 0.7 dB/m or 0.35 dB/m according to the MOF core size. The fibers have been designed to present a zero dispersion wavelength (ZDW) around 2 microm. By pumping the fibers at 1.55 microm, strong spectral broadenings are obtained in both 1.8 and 45-m-long fibers by using a picosecond fiber laser.

Experimental investigation of Brillouin and Raman scattering in a 2SG sulfide glass microstructured chalcogenide fiber.

In this work, we investigate the Brillouin and Raman scattering properties of a Ge15Sb20S65 chalcogenide glass microstructured single mode fiber around 1.55 microm. Through a fair comparison between a 2-m long chalcogenide fiber and a 7.9-km long classical single mode silica fiber, we have found a Brillouin and Raman gain coefficients 100 and 180 larger than fused silica, respectively.

Second-harmonic generation of thermally poled chalcogenide glass.

Second harmonic generation (SHG) has been obtained in a sample of Ga5Ge20Sb10S65 glass submitted to a thermal poling treatment. An original characterization method is used for the determination of the induced second-order nonlinear profile. A reproducible chi(2) susceptibility of 4.4 +/- 0.4 pm/Volt was achieved for specific poling conditions.