Origin and percolation times of Milandre Cave drip water determined by tritium time series and beryllium-7 data from Switzerland.

Early observations of the tritium (3H) activity in precipitation from Switzerland started in 1967 in Bern and a monitoring program with improved analytical techniques was carried out between 1971 and 2009. Between 2012 and 2015, we performed tritium analyses on daily precipitation samples from north-western Switzerland to better constrain the tritium variability. We also collected waters dripping inside Milandre Cave (Jura Mountains) with a 4-6 months' resolution in order to estimate the age of the drip water, which is mandatory to interpret the high-resolution speleothem (cave carbonate deposits) records. Over the monitoring period, the mean tritium concentration in the daily precipitation samples was approximately 8.7 ± 4.7 TU with distinct seasonality showing higher values in spring and summer (from April-May to August-September). The similarity in trends with the other cosmogenic radionuclide beryllium-7 (7Be) suggests that, for the study site, tritium in precipitation essentially originates from stratospheric input in spring. In winter, precipitation dynamics with increasing moisture originating from the Atlantic and diluted during transport contribute to low values close to the Atlantic background. In cave drip water, the depleted activity level of tritium indicates a relatively long percolation time from the surface to the cave of several years. A residual superimposed short tritium variability provides evidence for the occurrence of fast flowing water paths. The contribution from both components were quantified based on a two-component lumped parameter-mixing model. Finally, we show that tritium concentrations in cave drip water are linked to the moisture origin and atmospheric transport pathways.

Central Europe temperature constrained by speleothem fluid inclusion water isotopes over the past 14,000 years.

The reasons for the early Holocene temperature discrepancy between northern hemispheric model simulations and paleoclimate reconstructions-known as the Holocene temperature conundrum-remain unclear. Using hydrogen isotopes of fluid inclusion water extracted from stalagmites from the Milandre Cave in Switzerland, we established a mid-latitude European mean annual temperature reconstruction for the past 14,000 years. Our Milandre Cave fluid inclusion temperature record (MC-FIT) resembles Greenland and Mediterranean sea surface temperature trends but differs from recent reconstructions obtained from biogenic proxies and climate models. The water isotopes are further synchronized with tropical precipitation records, stressing the Northern Hemisphere signature. Our results support the existence of a European Holocene Thermal Maximum and data-model temperature discrepancies. Moreover, data-data comparison reveals a significant latitudinal temperature gradient within Europe. Last, the MC-FIT record suggests that seasonal biases in the proxies are not the primary cause of the Holocene temperature conundrum.