Migration behavior of radiostrontium and radiocesium in arid-region soil.

The time-dependent of the average migration, depths and migration rates of radiostrontium and radiocesium were experimentally determined in sandy soil in Kuwait. The study aimed to describe the behavior of these radionuclides in typical soil types in Kuwait. Custom-made large-diameter lysimeters (30 cm) were constructed to hold about 70 kg of undisturbed soil. The top surface soil was contaminated with known activity concentrations of 85Sr and 134Cs radionuclides. The topsoil was wetted with 1 L of water weekly using a rain simulator tool. Gamma scanning of the lysimeters in a step of 5 cm from three sides was performed at three measurement times by a high-resolution portable gamma spectrometry system. The vertical distribution pattern of 85Sr and 134Cs concentration exhibited an exponential trend. The average migration depth and migration rates were calculated, and 90% of the 85Sr and 134Cs were situated at 10.38 and 5.73 cm in the topsoil layer, respectively. The average vertical migration rate of 85Sr varied from 2.2 to 4.4 cm y-1, and 134Cs was from 0.3 to 0.9 cm y-1. It was demonstrated that the mobility of the 85 Sr and 134 Cs in the sandy soil could be attributed to the physicochemical properties of the radionuclide, in particular the distribution coefficient (Kd). The obtained results could be adopted by the regions of similar climatological conditions, especially, the gulf countries region when the radiological risk assessment of contaminated sites and dose estimation is required.

Activity size distributions of radioactive airborne particles in an arid environment: a case study of Kuwait.

Atmospheric radioactive airborne released from several natural and artificial sources can travel for long distances and disperse in different directions. Both the physical and chemical characteristics of the atmospheric aerosols control this movement. The concentrations of 210Pb, 210Po, 7Be, 40K and 137Cs radionuclides in the ground surface air were determined in three particle sizes (2.4-10.2, 0.73-2.4 and less than 0.73 µm). High-volume air samples were collected from five different locations representing the five governorates of Kuwait using high-volume air samplers connected to a five-stage cascade impactor. The radioactivity concentrations of almost all fallout radionuclides were concentrated on the fine particle size fractions. The cosmogenic 7Be radioactivity level in all locations was relatively comparable and varied between 1.16 and 18.38 mBq/m3, with a geometric mean value of 6.80 mBq/m3. 137Cs was infrequently recorded with concentration varied between 4 and 14.3 µBq/m3. The geometric mean levels of the 210Po and 210Pb were 0.899 mBq/m3 and 1.03 mBq/m3, respectively, indicating that anthropogenic sources likely enrich 210Po. 40K was concentrated on large particle size fractions with a geometric mean value of 2.34 mBq/m3, reflecting the effects of the local dust sources. It was concluded that the radiological hazards due to airborne radioactive inhalation are low and can be negligible, where the annual estimated effective dose is about 64.0 µSv. The radioactive airborne measurements compose the base of estimating the aerosols residence time, resuspension rate of dust, soil redistribution and source apportionment, particularly the 210Pb and 210Po radionuclides.