Plasmonic nanoparticle chain in a light field: a resonant optical sail.

Optical trapping and driving of small objects has become a topic of increasing interest in multidisciplinary sciences. We propose to use a chain made of metallic nanoparticles as a resonant light sail, attached by one end point to a transparent object and propelling it by the use of electromagnetic radiation. Driving forces exerted on the chain are theoretically studied as a function of radiation's wavelength and chain's alignments with respect to the direction of radiation. Interestingly, there is a window in the frequency spectrum in which null-torque equilibrium configuration, with minimum geometric cross section, corresponds to a maximum in the driving force.

Light control of silver nanoparticle's diffusion.

The diffusion of silver nanoparticles in water at 298K inside an optical vortex lattice is analyzed in detail by numerical simulations. At power densities of the order of those used to trap nanoparticles with optical tweezers, the dynamic response shows three different regimes depending on the light wavelength. In the first one particles get trapped inside the light vortices following almost closed trajectories. In the second one, around the plasmon resonance, the diffusion constant is dramatically enhanced with respect to the Brownian motion. In the third one, at longer wavelengths, nanoparticles are confined during a few seconds in quasi-one-dimensional optical traps.

Giant enhanced diffusion of gold nanoparticles in optical vortex fields.

We study the diffusion of a metal nanoparticle in the nonconservative force field of an optical vortex lattice. Radiation pressure in the vortex array is shown to induce a giant enhancement over the free thermal diffusion. Langevin dynamics simulations show that the diffusion coefficient of (50 nm radius) gold particles at room temperature is enhanced by 2 orders of magnitude at power densities of the order or smaller than those used to trap nanoparticles with optical tweezers.

Scattering forces from the curl of the spin angular momentum of a light field.

Light forces on small (Rayleigh) particles are usually described as the sum of two terms: the dipolar or gradient force and the scattering or radiation pressure force. The scattering force is traditionally considered proportional to the Poynting vector, which gives the direction and magnitude of the momentum flow. However, as we will show, there is an additional nonconservative contribution to the scattering force arising in a light field with nonuniform helicity. This force is shown to be proportional to the curl of the spin angular momentum of the light field. The relevance of the spin force is illustrated in the simple case of a 2D field geometry arising in the intersection region of two standing waves.

Optical resonances in one-dimensional dielectric nanorod arrays: field-induced fluorescence enhancement.

Arrays of transparent dielectric nanorods are shown to produce very large local field enhancements at specific resonant conditions. These structures would lead to enhancement of molecular fluorescence signals without quenching. The resonant angular width and field enhancements are analytically derived as a function of wavelength, grating period, rod radius, and dielectric constant.