Anthropogenic accumulation based on chemometrics of the radionuclide K-40 in tropical soils in the northeast Brazil.

The continuous use of fertilizers can increase the radionuclides levels in soils, and their accumulation and concentration are related to their characteristics and the various processes of use and soil occupation. Analyzing data from radiometric and pedological measurements often demands the use of more robust tools for better integration of results. This work presents the results of a study to evaluate the accumulation of 40K, in an area of the Zona da Mata region in Pernambuco, Northeastern Brazil, due to the contribution of natural or artificial sources. 40K activity concentration was measured by high resolution gamma spectrometry in 108 soil samples, as well the organic matter content and particle size distribution. Results showed the 40K activity ranged from 103 to 1843 Bq.Kg-1, with the arable soils showing levels above the world average value (420 Bq.Kg-1). A higher prevalence of 40K was observed on arable soils, regardless of soil type, organic matter content, depth or texture. Agricultural activities increased of 40K levels in different degrees, depending on the type of crop used, with an accumulation factor of up to 4 times greater compared to soils not impacted by agricultural activities. The radiochemometric diagnosis maded it possible to draw up a strategic management plan to improve the management practices of family farming in order to maximize production efficiency, and promote the conservation of natural resources and environmental preservation.

Risk survey for the population of Recife and neighboring cities due to the occurrence of radium in groundwater.

The Metropolitan Region of Recife and its surroundings are heavily exploited to capture water for public supply through tubular wells. However, a survey of the levels of natural radionuclides from these sources had never been carried out, even though part of this region contains a phosphate deposit that has a high concentration of natural uranium. In this context, this research aimed to identify 228Ra and 226Ra levels in groundwater in the coastal region of Pernambuco, Brazil. About 110 points (wells) of drinking water for public supply were identified and studies were carried out to estimate the level of ingestion and subsequent risk due to the presence of this radionuclide. The average concentration of combined radium was 104 mBq.L-1. For 228Ra an effective dose of 0.46, 0.11, 0.12 and 0.0276 mSv.y-1 for infants, children aged 1 and 10 and adults, respectively, were obtained. Although doses above those recommended by WHO were found, the equivalent dose and the induction of bone sarcoma did not indicate a risk to the population. Groundwater with higher dose values is influenced by local geology.

ENVIRONMENTAL IONIZING RADIATION DOSE OUTDOOR IN AN INHABITED AREA WITH A HIGH CONCENTRATION OF URANO-PHOSPHATE IN NORTHEAST OF BRAZIL.

A marine phosphorus region with high concentrations of phosphate, coastwise of Pernambuco, Northeast of Brazil, is densely inhabited. Rock phosphate deposits naturally contain uranium ore that produces ionizing radiation from it and its natural descendants, furthermore, its thorium and potassium concentrations are comparable to those usually found in soils. Radiological monitoring of this environment is important to verify the occurrence of harmful effective doses for the adjacent population. This study aimed at the in situ radiometric monitoring in four cities of the north of the Metropolitan Region of Recife-Pernambuco, estimating the effective environmental dose to which the local population is subject. In total, 91 points were monitored with a discriminator-type detector. The outdoor environmental effective dose rates ranged from 1.99 ± 0.09 to 7.59 ± 0.36 mSv y-1, with an average of 2.60 ± 0.69 mSv y-1.

INVESTIGATION OF NATURAL RADIOACTIVITY AS A POSSIBLE DRIVER OF CANCER INCIDENCE IN PARAÍBA, NORTHEASTERN BRAZIL.

An increase of health problems has been reported in the city of Triunfo, Paraíba, NE Brazil. This pattern has been attributed to environmental radiation since there are uranium deposits in the neighboring municipalities. The present study aimed to carry a radiometric survey in Triunfo to determine effective dose from external outdoor radiation exposure. The results were obtained through 'in situ' measurements using a gamma spectrometry system. The results ranged from 0.06 to 0.38 mSv/y, mean of 0.20 mSv/y. Due to the low value of the effective dose rate, we concluded that the area is characterized by low background radiation. Therefore, natural radioactivity is probably not directly influencing the increase in cancer incidence in the region. However, there is a need for complementary studies in this area to evaluate the dose from potential exposure to ingested and inhaled natural radionuclides from natural radioactivity in soil, rocks, vegetation and water.

Natural radionuclides in electronic waste: an initial approach.

Some radionuclides are present in trace amount in the raw material of electronic devices that suffer obsolescence and are improperly disposed of. Obsolete personal computers become electronic waste and may contain potential environmental contaminants. Furthermore, there may be an additional concern: the ionizing radiation emission. This study aimed to assess qualitatively the possibility of alpha and beta particles and gamma rays reaching somehow workers involved in the handling of such wastes. Using gamma spectrometry method, we analyzed a set of 10 microprocessors randomly taken from motherboards incorrectly discarded. The analysis resulted in the occurrence of primordial radioisotopes in the microchips.

Analysis of the 40K levels in soil using gamma spectrometry

Potassium-40 was determined in soil in an area with 40,000 m² situated in the western State of Pernambuco, Brazil. For radiometric measurements, the gamma spectrometry method with a high purity germanium (HPGe) detector was used. Sampling of 78 soil samples has been performed at intervals of 25 m. The specific activities of 40K were calculated based on the photopeak of 1.46 MeV. Values from 541 to 3,572 Bq kg-1 were obtained (mean of 1,827 Bq kg-1). These values allowed the determination of the elemental concentrations as well as the absorbed dose rates in air, 1 m above the ground. The values varied from 1.7 to 11.5 percent (mean of 6 percent) and from 23.4 to 154.3 nGy h-1 (mean of 79 nGy h-1), respectively.

A radioatividade do 40K foi determinada em solo em uma área de aproximadamente 40.000 m² localizada no Estado de Pernambuco, Brasil. Para as medidas radiométricas foi usado o método de espectrometria gama com detector de germânio de alta pureza (HPGe). A amostragem perfaz um total de setenta e oito amostras de solo coletadas em intervalos de 25 m. As atividades específicas do 40K foram calculadas com base no fotopico gama de 1,46 MeV. Foram obtidos valores que variaram de 541 a 3.572 Bq kg-1 (média aritmética de 1.827 Bq kg-1). Com base nestes cálculos, obteve-se concentrações elementares e doses absorvidas no ar a 1 m, derivadas da contribuição do 40K no solo, onde os valores obtidos variaram respectivamente de 1,7 a 11,5 por cento (média 6 por cento) e 23,4 a 154,3 nGy h-1 (média 79 nGy h-1).

Intake of uranium and radium-226 due to food crops consumption in the phosphate region of Pernambuco--Brazil.

The phosphate region located in the Northeast of Brazil covers an area of approximately 150 km long with an average width of 4 km, along the coast of the states of Pernambuco and Paraíba. The inhabitants of this area are exposed to natural radioactivity levels higher than the background values recorded in the literature, mainly due to the presence of uranium and its decay products in the phosphatic sediments. The main aim of this study was to determine the activity concentration of uranium and (226)Ra in foodstuffs cultivated in this area, where the phosphate mineral has been extracted. The activity concentrations found for uranium and (226)Ra in the foodstuffs analyzed varied from 13 to 186 mBq kg(-1) (wet weight), with a mean value of 46 mBq kg(-1) and from 43 to 2209 mBq kg(-1) (wet weight), with a mean value of 358 mBq kg(-1), respectively. The annual intake of these radionuclides, for rural residents, was 7.45 Bq for uranium and 69.3 Bq for (226)Ra.