Ultrahigh-order wave mixing in noncollinear high harmonic generation.

We show that noncollinear high harmonic generation (HHG) can be fully understood in terms of nonlinear optical wave mixing. We demonstrate this by superposing on the fundamental ω1 field its second harmonic ω2 of variable intensity in a noncollinear geometry. It allows us to identify, by momentum conservation, each field's contribution (n1,n2) to the extreme ultraviolet emission at frequency Ω = n1ω1 + n2ω2. We observe that the photon (Ω) yield follows an n2 power law on the ω2 intensity, before saturation. It demonstrates that, although HHG is a highly nonperturbative process, a perturbation theory can still be developed around it.

Enhanced propagation for relativistic laser pulses in inhomogeneous plasmas using hollow channels.

The influence of long (several millimeters) and hollow channels, bored in inhomogeneous ionized plasma by using a long pulse laser beam, on the propagation of short, ultraintense laser pulses has been studied. Compared to the case without a channel, propagation in channels significantly improves beam transmission and maintains a beam quality close to propagation in vacuum. In addition, the growth of the forward-Raman instability is strongly reduced. These results are beneficial for the direct scheme of the fast ignitor concept of inertial confinement fusion as we demonstrate, in fast-ignition-relevant conditions, that with such channels laser energy can be carried through increasingly dense plasmas close to the fuel core with minimal losses.

Wavelength scaling of high harmonic generation efficiency.

Using longer wavelength laser drivers for high harmonic generation is desirable because the highest extreme ultraviolet frequency scales as the square of the wavelength. Recent numerical studies predict that high harmonic efficiency falls dramatically with increasing wavelength, with a very unfavorable lambda(-(5-6)) scaling. We performed an experimental study of the high harmonic yield over a wavelength range of 800-1850 nm. A thin gas jet was employed to minimize phase matching effects, and the laser intensity and focal spot size were kept constant as the wavelength was changed. Ion yield was simultaneously measured so that the total number of emitting atoms was known. We found that the scaling at constant laser intensity is lambda(-6.3+/-1.1) in Xe and lambda(-6.5+/-1.1) in Kr over the wavelength range of 800-1850 nm, somewhat worse than the theoretical predictions.

Dynamic two-center interference in high-order harmonic generation from molecules with attosecond nuclear motion.

We report a new dynamic two-center interference effect in high-harmonic generation from H2, in which the attosecond nuclear motion of H2+ initiated at ionization causes interference to be observed at lower harmonic orders than would be the case for static nuclei. To enable this measurement we utilize a recently developed technique for probing the attosecond nuclear dynamics of small molecules. The experimental results are reproduced by a theoretical analysis based upon the strong-field approximation which incorporates the temporally dependent two-center interference term.

Laser-induced electron tunneling and diffraction.

Molecular structure is usually determined by measuring the diffraction pattern the molecule impresses on x-rays or electrons. We used a laser field to extract electrons from the molecule itself, accelerate them, and in some cases force them to recollide with and diffract from the parent ion, all within a fraction of a laser period. Here, we show that the momentum distribution of the extracted electron carries the fingerprint of the highest occupied molecular orbital, whereas the elastically scattered electrons reveal the position of the nuclear components of the molecule. Thus, in one comprehensive technology, the photoelectrons give detailed information about the electronic orbital and the position of the nuclei.

Generation of 1.5 microJ single-cycle terahertz pulses by optical rectification from a large aperture ZnTe crystal.

We demonstrate the generation muJ-level, single-cycle terahertz pulses by optical rectification from a large-aperture ZnTe single crystal wafer. Energies up to 1.5 muJ per pulse and a spectral range extending to 3 THz were obtained using a 100 Hz Ti:sapphire laser source and a 75-mmdiameter, 0.5-mm-thick, (110) ZnTe crystal, corresponding to an average power of 150 muW and an energy conversion efficiency of 3.1 x 10(-5). We also demonstrate real-time imaging of the focused terahertz beam using a pyroelectric infrared camera.

Thomson-scattering study of the subharmonic decay of ion-acoustic waves driven by the Brillouin instability.

Thomson scattering (TS) has been used to investigate the two-ion decay instability of ion acoustic waves generated by stimulated Brillouin scattering in an underdense CH plasma. Two complementary TS diagnostics, spectrally and spatially resolved, demonstrate the occurrence of the subharmonic decay of the primary ion acoustic wave into two secondary waves. The study of the laser intensity dependence shows that the secondary ion acoustic waves are correlated with the SBS reflectivity saturation, at a level of a few percent.

Strong reduction of the degree of spatial coherence of a laser beam propagating through a preformed plasma.

A strong reduction of the spatial coherence of a laser beam after its propagation through a plasma has been measured using a Fresnel biprism interferometer. The laser beam was diffraction limited; the coherence width was reduced from 40 mm in vacuum down to a few mm with the plasma. Numerical results based on a paraxial model exhibit a coherence degree close to the experimental one; they also prove the importance of taking into account the nonlocal transport effects in numerical simulations for such plasma conditions.

Observation of ion acoustic waves associated with plasma-induced incoherence of laser beams using Thomson scattering.

We have carried out experiments to investigate the physical processes responsible for the recently discovered phenomenon of plasma-induced incoherence (PII) of a laser beam. Using a Thomson scattering diagnostic, we have observed ion acoustic waves (IAW) having wave vectors transverse to the interaction beam spectral and temporal characteristics of which show a clear correlation with other signatures of PII for various conditions of plasma density and laser intensity. These results support the recent theoretical interpretation for which the IAW result from the coupling between forward stimulated Brillouin scattering and self-focusing of the laser light in PII mechanisms.

Reduction of the coherence time of an intense laser pulse propagating through a plasma.

We present direct measurements of the coherence time of a laser beam after propagation through an underdense plasma. At an intensity of 10(14) W/cm(2), a large decrease of the coherence time is observed, from 300 ps to a few picoseconds. This decrease is larger as the plasma density is increased or as the light is scattered at larger angles. The amount of temporal decorrelation as well as the effect of the plasma density, laser intensity, and scattering angle all coincide with trends observed in recent numerical simulations.

Experimental evidence of electric inhibition in fast electron penetration and of electric-field-limited fast electron transport in dense matter

Fast electron generation and propagation were studied in the interaction of a green laser with solids. The experiment, carried out with the LULI TW laser (350 fs, 15 J), used K(alpha) emission from buried fluorescent layers to measure electron transport. Results for conductors (Al) and insulators (plastic) are compared with simulations: in plastic, inhibition in the propagation of fast electrons is observed, due to electric fields which become the dominant factor in electron transport.