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1.
Sci Total Environ ; 869: 161743, 2023 Apr 15.
Artigo em Inglês | MEDLINE | ID: mdl-36690102

RESUMO

Vapour intrusion (VI) is the process through which volatile organic compounds migrate from the subsurface source to the soil predominantly by diffusion, entering the overlying buildings through joints, cracks or other openings. This activity poses potentially serious health hazards for the occupants. Because of these health risks, recommendations for site closure are often made by quantifying the VI risks using mathematical models known as 'vapour intrusion models' (VIM). Most of these VIMs seem to overlook the role of preferred pathways like utility lines, high conductivity zones of soil or rocks, etc., which act as the path of least resistance for vapour transport thereby increasing vapour intrusion risks. This study presents a two-dimensional (2-D) chlorinated vapour intrusion (CVI) model which seeks to estimate the source-to-indoor air concentration attenuation. It takes into account the effects of a highly permeable utility line embedment as a preferential pathway. The transport of 2-D soil gas is described using the finite difference method where advection serves as the dominant transport mechanism in the preferential pathway layer, while diffusion applies to the rest of the vadose zone. The model returned results comparable with other models for the same input parameters, and was found to closely replicate the results of 3-D models. The simulations indicate that the presence of highly permeable utility line embedment and backfill layers do trigger a higher indoor air concentration compared to a no preferential pathway scenario.

2.
J Environ Manage ; 299: 113654, 2021 Dec 01.
Artigo em Inglês | MEDLINE | ID: mdl-34482107

RESUMO

Despite the increasing use of chemical additives in construction and their potential threat to the environment and human health, many C&DW studies lack a comprehensive view of chemicals of concern (COC) in C&DW. This study systematically reviewed published studies from 2010 to August 2021 using a keyword search methodology to explore COC in C&DW fine residues based on 73 articles identified from 5 prominent databases. Results show that trace/heavy metals (As, Cr, Cu, Cd, and Pb) as well as high concentrations of toxic gasses (methane, hydrogen sulphide and mercury vapour) have been reported in landfills. Besides, organic chemicals such as polycyclic aromatic hydrocarbons, polychlorinated biphenyls, and brominated flame retardants have been found in landfill leachates in the Netherlands and widely detected in landfill leachates in Sweden, Japan, and Canada. The potential of these contaminants to cause health complications has also been reported. Carcinogenicity, liver and kidney damage, cumulative damage, neurological disorders and foetal damage were reported as associated health implications of exposure to COC from C&DW. A waste disposal lens was used to explore the factors that influence the environment and human health impacts (pH, gypsum and organic content, size fraction, atmospheric exposure and liquid infiltration rate). Despite environmental and health issues relating to C&DW fine residues, the ultimate destination for C&DW fine residues remains in general landfills. Although significant efforts in managing C&DW have been implemented at various levels, those specifically targeting C&DW fine residues remain sparse.


Assuntos
Retardadores de Chama , Eliminação de Resíduos , Poluentes Químicos da Água , Monitoramento Ambiental , Retardadores de Chama/análise , Humanos , Instalações de Eliminação de Resíduos , Poluentes Químicos da Água/análise
3.
Sci Total Environ ; 796: 148885, 2021 Nov 20.
Artigo em Inglês | MEDLINE | ID: mdl-34265614

RESUMO

Vapour intrusion (VI) is the phenomenon by which volatile organic compounds (VOCs) migrate from the subsurface source through the soil and enter into the overlying buildings, affecting the indoor air quality and ultimately causing health hazards to the occupants. Health risk assessments associated with hydrocarbon contaminated sites and recommendations of site closure are often made by quantifying the VI risks using mathematical models known as 'vapour intrusion models' (VIM). In order to predict the health risk, various factors such as the lithological and geochemical conditions of the subsurface, environmental conditions, building operational conditions etc. are commonly evaluated using VIMs. Use of these models can overlook the role of preferential pathways like highly permeable subsurface layers and utility lines which act as the path of least resistance for vapour transport, which can increase the VI risks. The extensive networks of utility lines and sanitary sewer systems in urban areas can significantly exacerbate the uncertainty of VI investigations. The backfill materials like sand and gravel surrounding the utility lines can allow the vapours to easily pass through due to their high porosity as compared to natural formations. Hence, failure to understand the role of preferential pathways on the fate and transport of VOC in the vadose zone can result in more conservative predictions of indoor air vapour concentrations and wrong clean up approaches. This comprehensive review outlines the vapour transport mechanisms, factors influencing VI, VIMs and the role of preferential pathways in predicting indoor air vapour concentrations.


Assuntos
Poluição do Ar em Ambientes Fechados , Compostos Orgânicos Voláteis , Poluição do Ar em Ambientes Fechados/análise , Gases , Hidrocarbonetos/análise , Solo
4.
J Environ Sci (China) ; 88: 31-45, 2020 Feb.
Artigo em Inglês | MEDLINE | ID: mdl-31862072

RESUMO

Since the early 1980's there have been several different strategies designed and applied to the remediation of subsurface environment including physical, chemical and biological approaches. They have had varying degrees of success in remediating contaminants from subsurface soils and groundwater. The objective of this review is to examine the range of technologies for the remediation of contaminants, particularly petroleum hydrocarbons, in subsurfaces with a specific focus on bioremediation and electrokinetic remediation. Further, this review examines the efficiency of remediation carried out by combining bioremediation and electrokinetic remediation. Surfactants, which are slowly becoming the selected chemicals for mobilizing contaminants, are also considered in this review. The current knowledge gaps of these technologies and techniques identified which could lead to development of more efficient ways of utilizing these technologies or development of a completely new technology.


Assuntos
Recuperação e Remediação Ambiental , Petróleo , Poluentes do Solo , Biodegradação Ambiental , Hidrocarbonetos , Solo
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