Low-temperature laser-stimulated controllable generation of micro-bubbles in a water suspension of absorptive colloid particles.

A method is described for the generation of micrometer-sized vapor-gas bubbles in a water suspension containing absorptive pigment nanoparticles. The diluted suspension (mean interparticle distance 20 µm) absorbs the continuous laser radiation (wavelength 808 nm), and each particle in the best illuminated volume (~10 × 10 × 200 µm3) serves as a bubble-nucleation center. The suspension heating is inessential (several degrees above the room temperature) and the bubbles are formed mainly of the air gases dissolved in water. The bubbles can stably exist within or near the illuminated area where their location is governed by the competition between thermal and optical forces and can be controlled via the laser beam parameters. The method enables controllable creation, support, prescribed transportation, and destruction of the bubbles. This can be useful in applications aimed at precise sorting, transportation, and delivery of species in nano- and micro-engineering as well as for biomedical studies.

Controllable generation and manipulation of micro-bubbles in water with absorptive colloid particles by CW laser radiation.

Micrometer-sized vapor-gas bubbles are formed due to local heating of a water suspension containing absorptive pigment particles of 100 nm diameter. The heating is performed by CW near-infrared (980 nm) laser radiation with controllable power, focused into a 100 µm spot within a 2 mm suspension layer. By changing the laser power, four regimes are realized: (1) bubble generation; (2) stable growth of the existing bubbles; (3) stationary existence of the bubbles and (4) the bubbles' shrinkage and collapse. This behavior is interpreted based on the temperature conditions. The generation and evolution of single bubbles and ensembles of bubbles with controllable sizes and numbers is demonstrated. The bubbles are grouped within the laser-illuminated region and form quasi-ordered structures. They can easily be moved and transported controlled by the focal spot. The results are useful for applications associated with the precise manipulation, sorting and specific delivery in nano- and micro-engineering problems.

Measurement of small light absorption in microparticles by means of optically induced rotation.

The absorption parameters of micro-particles have been associated with the induced spin exerted upon the particle, when embedded in a circularly polarized coherent field. The induced rotational speed is theoretically analyzed, showing the influence of the beam parameters, the parameters of the particle and the tribological parameters of the surrounding fluid. The theoretical findings have been adequately confirmed in experiments.

Self-action of continuous laser radiation and Pearcey diffraction in a water suspension with light-absorbing particles.

Water suspension of light-absorbing nano-sized particles is an example of a medium in which non-linear effects are present at moderate light intensities favorable for optical treatment of organic and biological objects. We study experimentally the phenomena emerging in a thin layer of such a medium under the action of inhomogeneous light field formed due to the Pearcey diffraction pattern near a microlens focus. In this high-gradient field, the light energy absorbed by the particles induces inhomogeneous distribution of the medium refraction index, which results in observable self-diffraction of the incident light, here being strongly sensitive to the medium position with respect to the focus. This technique, based on the complex spatial structure of both the incident and the diffracted fields, can be employed for the detection and measurement of weak non-linearities.

Self-diffraction of continuous laser radiation in a disperse medium with absorbing particles.

We study the self-action of light in a water suspension of absorbing subwavelength particles. Due to efficient accumulation of the light energy, this medium shows distinct non-linear properties even at moderate radiation power. In particular, by means of interference of two obliquely incident beams, it is possible to create controllable phase and amplitude gratings whose contrast, spatial and temporal parameters depend on the beams' coherence and power as well as the interference geometry. The grating characteristics are investigated via the beams' self-diffraction. The main mechanism of the grating formation is shown to be thermal, which leads to the phase grating; a weak amplitude grating also emerges due to the particles' displacements caused by the light-induced gradient and photophoretic forces. These forces, together with the Brownian motion of the particles, are responsible for the grating dynamics and degradation. The results and approaches can be used for investigation of the thermal relaxation and kinetic processes in liquid suspensions.

Circular motion of particles suspended in a Gaussian beam with circular polarization validates the spin part of the internal energy flow.

Non-spherical dielectric microparticles were suspended in a water-filled cell and exposed to a coherent Gaussian light beam with controlled state of polarization. When the beam polarization is linear, the particles were trapped at certain off-axial position within the beam cross section. After switching to the right (left) circular polarization, the particles performed spinning motion in agreement with the angular momentum imparted by the field, but they were involved in an orbital rotation around the beam axis as well, which in previous works [Y. Zhao et al, Phys. Rev. Lett. 99, 073901 (2007)] was treated as evidence for the spin-to orbital angular momentum conversion. Since in our realization the moderate focusing of the beam excluded the possibility for such a conversion, we consider the observed particle behavior as a demonstration of the macroscopic "spin energy flow" predicted by the theory of inhomogeneously polarized paraxial beams [A. Bekshaev et al, J. Opt. 13, 053001 (2011)].

Orbital rotation without orbital angular momentum: mechanical action of the spin part of the internal energy flow in light beams.

The internal energy flow in a light beam can be divided into the "orbital" and "spin" parts, associated with the spatial and polarization degrees of freedom of light. In contrast to the orbital one, experimental observation of the spin flow seems problematic because it is converted into an orbital flow upon tight focusing of the beam, usually applied for energy flow detection by means of the mechanical action upon probe particles. We propose a two-beam interference technique that results in an appreciable level of spin flow in moderately focused beams and detection of the orbital motion of probe particles within a field where the transverse energy circulation is associated exclusively with the spin flow. This result can be treated as the first demonstration of mechanical action of the spin flow of a light field.

Centrifugal transformation of the transverse structure of freely propagating paraxial light beams.

Superpositions of coaxial Laguerre-Gaussian modes with common waists and the same Gaussian envelopes are known to form beams whose transverse structures experience the self-similar transformation during free beam propagation: the beam shape remains the same except for the divergence and rotation around the propagation axis. We show that under certain conditions this transformation can be represented as if every point of the beam cross section performs a centrifugal straight-line fly off.

Optical vortex symmetry breakdown and decomposition of the orbital angular momentum of light beams.

Two forms of the transverse energy circulation within plane-polarized paraxial light beams are specified: one inherent in wave-front singularities (optical vortices) and the other peculiar to astigmatism and asymmetry of beams with a smooth wave front. As quantitative measures of these energy flow components, the concepts of vortex and asymmetry parts of a beam's orbital angular momentum are introduced and their definitions are proposed on the basis of beam intensity moments. The properties and physical meaning of these concepts are analyzed, and their use for the study of transformations of optical vortices is demonstrated.

Manifestation of the rotational Doppler effect by use of an off-axis optical vortex beam.

We report what is to our knowledge the first all-optical detection of the frequency beats between Gaussian and Laguerre-Gaussian LG0(1) modes in their axial superposition, caused by the rotational Doppler effect. The relation between the observable off-axis optical vortex rotation and the rotational frequency shift of the Laguerre-Gaussian component is ascertained. The results can be used as a physical basis for recognition of Laguerre-Gaussian mode spectra along their orbital angular momenta.