Taming Friedrich-Wintgen Interference in a Resonant Metasurface: Vortex Laser Emitting at an On-Demand Tilted Angle.

Friedrich-Wintgen (FW) interference is an atypical coupling mechanism that grants loss exchange between leaky resonances in non-Hermitian classical and quantum systems. Intriguingly, such a mechanism makes destructive interference possible for scenarios in which a radiating wave becomes a bound state in the continuum (BIC) by giving away all of its losses. Here we propose and demonstrate experimentally an original concept to tailor FW-BICs with polarization singularity at on-demand wavevectors in an optical metasurface. As a proof-of-concept, using hybrid organic-inorganic halide perovskite as an active material, we empower this novel polarization singularity to obtain lasing emission, exhibiting both highly directional emission at oblique angles and a polarization vortex in momentum space. Our results pave the way to steerable coherent emission with a tailored polarization pattern for applications in optical communication/manipulation in free space, high-resolution imaging/focusing, and data storage.

Exploring the benefits of surface analysis techniques to develop double multilayer transfer printing of J-Aggregates cyanine dyes by integrating L-b-L and µCp processes.

Layer-by-layer self-assembly (L-b-L assembly) makes possible to obtain polyelectrolyte multilayers (PEMs) and one of the polyelectrolytes could be replaced by a dye molecule to obtain multilayers which may exhibit optical properties of great interest. On the other hand, µCp has become a routine technique for the preparation of micro- and nanostructured surfaces. In our development in progress of a surface engineering strategy to transfer J-Agg cyanine dyes onto surfaces by integrating L-b-L process and µCp, this contribution highlights how surface analysis imaging techniques can bring valuable information for the development of the process involving a double Multilayers Transfer Printing (MTP) with a Moiré effect. Key parameters sustaining image interpretation are difference in deposit thickness (optical microscopy, atomic force microscopy, scanning electron microscopy), in roughness (atomic force microscopy and scanning electron microscopy), in charge effect (scanning electron microscopy) and the chemical contrast between unprinted and printed areas (time-of-flight secondary ion mass spectrometry).

Selective grating obtained by dye microstructuration based on local photobleaching using a laser writer.

We propose a method to pattern organic optically active materials based on local photobleaching for creating a wavelength-selective grating. Usually, photobleaching is considered a limitation for an organic emitter. Here, this property is exploited to locally suppress dye emission and absorption at the microscale with an abrupt interface and no changes in layer thickness. Periodic patterns were fabricated and exhibit diffraction only at a 590 nm wavelength with a spectral selectivity of 11 nm. Based on laser writer flexibility and efficiency, this study shows the potential of local photobleaching for applications such as wavelength-selective grating fabrication.

Highly efficient singular surface plasmon generation by achiral apertures.

We report a highly efficient generation of singular surface plasmon (SP) fields by an achiral plasmonic structure consisting of Λ-shaped apertures. Our quantitative analysis, based on leakage radiation microscopy (LRM), demonstrates that the induced spin-orbit coupling can be tuned by adjusting the apex angle of the Λ-shaped aperture. Specifically, the array of Λ-shaped apertures with the apex angle 60° is shown to give rise to the directional coupling efficiency. The ring of Λ-shaped apertures with the apex angle 60° was found to generate the maximum extinction ratio (ER=11) for the SP singularities between two different polarization states. This result provides a more efficient way for developing an SP focusing and an SP vortex in the field of nanophotonics such as optical tweezers.

Coherence and aberration effects in surface plasmon polariton imaging.

We study theoretically and experimentally coherent imaging of surface plasmon polaritons using either leakage radiation microscopy through a thin metal film or interference microscopy through a thick metal film. Using a rigorous modal formalism based on scalar Whittaker potentials, we develop a systematic analytical and vectorial method adapted to the analysis of coherent imaging involving surface plasmon polaritons. The study includes geometrical aberrations due index mismatch which played an important role in the interpretation of recent experiments using leakage radiation microscopy. We compare our theory with experiments using classical or quantum near-field scanning optical microscopy probes and show that the approach leads to a full interpretation of the recorded optical images.

Leakage interferences applied to surface plasmon analysis.

We report the experimental combination of leakage radiation microscopy with a Young slit experiment to address the spatial coherence properties of surface waves. We applied this method to measurements of surface plasmon polaritons (SPPs). The relationship between the spatial decay and interference contrast allows us to extract the degree of coherence. In a second step, we investigate the coherence properties of the plasmon in the weak coupling regime between fluorophores and metallic surfaces. Finally, a method is proposed to extract the propagation length of SPPs in a large variety of systems.