RESUMO
A laser-driven quantum electron ratchet nanodevice is proposed. The ratchet consists of a series of disconnected bubble-shaped nanodiode structures with a sharp tip to induce a large field enhancement. A laser pulse is used to create a plasmon oscillation in the vertical direction, and the shape of the bubble funnels the electrons toward the sharp tip leading to net electron transport in the horizontal direction. The electron current carries the fingerprint of the driving laser field. The system is modeled by using the time-dependent orbital free density functional theory with nanostructures containing thousands of atoms.
RESUMO
A dual time propagation approach is introduced to describe electron scattering and ionization. The space is divided into two regions, a central region with a full time-dependent Hamiltonian and an outer region where the kinetic operator and the laser field dominate. The two regions are connected by a source term. Time-dependent density functional theory calculations of wave packet scattering on molecules and photoelectron spectrum due to circularly polarized laser are presented to illustrate the efficiency and applicability of the approach.