Photon Pathways and the Nonperturbative Scaling Law of High Harmonic Generation.

High harmonic generation (HHG) has become a core pillar of attosecond science. Traditionally described with field-based models, HHG can also be viewed in a parametric picture, which predicts all properties of the emitted photons, but not the nonperturbative efficiency of the process. Driving HHG with two noncollinear beams and deriving analytically the corresponding yield scaling laws for any intensity ratio, we herein reconcile the two interpretations, introducing a generalized photonic description of HHG. It is in full agreement with field-based simulations and experimental data, opening the route to smart engineering of HHG with multiple driving beams.

Ultrafast Hidden Spin Polarization Dynamics of Bright and Dark Excitons in 2H-WSe_{2}.

We performed spin-, time- and angle-resolved extreme ultraviolet photoemission spectroscopy of excitons prepared by photoexcitation of inversion-symmetric 2H-WSe_{2} with circularly polarized light. The very short probing depth of XUV photoemission permits selective measurement of photoelectrons originating from the top-most WSe_{2} layer, allowing for direct measurement of hidden spin polarization of bright and momentum-forbidden dark excitons. Our results reveal efficient chiroptical control of bright excitons' hidden spin polarization. Following optical photoexcitation, intervalley scattering between nonequivalent K-K^{'} valleys leads to a decay of bright excitons' hidden spin polarization. Conversely, the ultrafast formation of momentum-forbidden dark excitons acts as a local spin polarization reservoir, which could be used for spin injection in van der Waals heterostructures involving multilayer transition metal dichalcogenides.

Observation of Magnetic Helicoidal Dichroism with Extreme Ultraviolet Light Vortices.

We report on the experimental evidence of magnetic helicoidal dichroism, observed in the interaction of an extreme ultraviolet vortex beam carrying orbital angular momentum with a magnetic vortex. Numerical simulations based on classical electromagnetic theory show that this dichroism is based on the interference of light modes with different orbital angular momenta, which are populated after the interaction between light and the magnetic topology. This observation gives insight into the interplay between orbital angular momentum and magnetism and sets the framework for the development of new analytical tools to investigate ultrafast magnetization dynamics.

Anisotropic dynamics of two-photon ionization: An attosecond movie of photoemission.

Imaging in real time the complete dynamics of a process as fundamental as photoemission has long been out of reach because of the difficulty of combining attosecond temporal resolution with fine spectral and angular resolutions. Here, we achieve full decoding of the intricate angle-dependent dynamics of a photoemission process in helium, spectrally and anisotropically structured by two-photon transitions through intermediate bound states. Using spectrally and angularly resolved attosecond electron interferometry, we characterize the complex-valued transition probability amplitude toward the photoelectron quantum state. This allows reconstructing in space, time, and energy the complete formation of the photoionized wave packet.