Measurements of the absolute gamma-ray emission intensities from the decay of 166Ho.

166Ho (T1/2≈ 26.8 h) is an emerging theragnostic radionuclide of interest in nuclear medicine due to its peculiar decay scheme, featuring high-energy ß- emission (≈ 1.8 MeV) coupled with the main gamma-ray emission (≈ 80.6 keV). Using the new 166Ho activity standard and the well-calibrated, high-energy resolution HPGe detector, both available at ENEA-INMRI, a new determination of several 166Ho gamma-ray emission intensities, Iγ, was performed with low uncertainty. The new Iγ values contributed to the Decay Data Evaluation Project.

Resuming elective surgical activity after the COVID-19 wave: what the patients need to know.

As COVID-19 outbreak enters its second phase of lockdown ease, healthcare plans involve elective surgery re-establishment to provide essential life-saving care. Patients are increasingly requesting information about their facility's readiness for safely performing surgery. This information should be open and transparent including patient's education with objective data regarding the state of the pandemic in the country and the control measures undertaken by the facility.

Efficiency transfer method applied to surface beta contamination measurements.

In this paper, the application of the efficiency transfer method to the evaluation of the surface beta contamination is described. Using efficiency transfer factors, the reference calibration factor of contamination monitors is corrected, to obtain the calibration factor for an actual contamination source. The experimental part of the paper illustrates the applicability of the method to the direct measurement of the surface beta contamination.

99mTc by 99Mo produced at the ENEA-FNG facility of 14MeV neutrons.

A severe supply crisis of 99Mo, precursor of 99mTc a diagnostic radionuclide largely used in Nuclear Medicine, occurred in 2008-2009 due to repeated shut-down of the two main (aged) fission reactors. An alternative route for producing 99Mo by 100Mo(n,2n)99Mo reaction was investigated at ENEA. The experiment, designed according to Monte Carlo simulations performed with the Fluka code, produced 99Mo by irradiating a natural Molybdenum powdered target with 14MeV neutrons produced at the Frascati Neutron Generator. The 99Mo specific activity was measured at metrological level by γ-ray spectrometry.

Comparison of 131I activity measurements at the NCBJ RC POLATOM and the ENEA-INMRI linked to the BIPM SIR system.

A bilateral comparison between ENEA-INMRI (Italy) and NCBJ RC POLATOM (Poland) of 131I-solution activity measurements was organized in the year 2015 and piloted by POLATOM, which provided the sources for the comparison. The 131I master solution was standardized independently at both institutes by using Liquid Scintillation Counting and ionization chamber techniques. The 131I master solution was then sent by POLATOM to the BIPM International Reference System (SIR). The comparison was registered as an EURAMET.RI(II)-K2.I-131 key comparison allowing the ENEA-INMRI result to enter in the SIR database.

A new approach in evaluating the surface beta contamination using the direct method of measurement.

This paper describes a new approach in evaluating the surface beta contamination using the direct method of measurement. It makes use of previous results obtained in numerical modeling of electron transport in planar geometry and is mainly based on the estimation of the efficiency of contamination sources for beta radiation and its standard uncertainty using the available information concerning the component materials of the sources and their main parameters. Experimental results illustrate the appropriateness of the new approach for surface beta contamination measurements.

Modeling the transmission of beta rays through thin foils in planar geometry.

This paper is concerned with the modeling of the transmission of beta rays through thin foils in planar geometry based on the plane source concept, using Monte Carlo simulation of electron transport and least squares fitting. Applications of modeling results for calculating the efficiency of large-area beta sources, transmission coefficient of beta rays through thin foils and the beta detection efficiency of large-area detectors used in surface contamination measurements are also presented.

A novel method for the activity measurement of large-area beta reference sources.

A novel method has been developed for the activity measurement of large-area beta reference sources. It makes use of two emission rate measurements and is based on the weak dependence between the source activity and the activity distribution for a given value of transmission coefficient. The method was checked experimentally by measuring the activity of two ((60)Co and (137)Cs) large-area reference sources constructed from anodized aluminum foils. Measurement results were compared with the activity values measured by gamma spectrometry. For each source, they agree within one standard uncertainty and also agree within the same limits with the certified values of the source activity.

Comparison of (18)F activity measurements at the VNIIM, NPL and the ENEA-INMRI using the SIRTI of the BIPM.

In 2014, the first three comparisons of activity measurements of (18)F were carried out at the VNIIM, NPL and the ENEA-INMRI using the BIPM's Transfer Instrument of the International Reference System. The transfer instrument and the NMIs primary measurement methods are briefly described. The degrees of equivalence with the key comparison reference value defined in the frame of the corresponding SIR comparison have been evaluated. World-wide consistency of activity measurements of (18)F is demonstrated.

Equivalence of computer codes for calculation of coincidence summing correction factors.

The aim of the study was to check for equivalence of computer codes that can perform calculations of true coincidence summing correction factors. All calculations were performed for a set of well-defined detector and sample parameters, without any reference to empirical data. For a p-type detector model the application of different codes resulted in satisfactory agreement in the calculated correction factors. For high-efficiency geometries in combination with an n-type detector and a radionuclide emitting abundant X-rays the results were scattered.

Comparison between two absolute methods used for 177Lu activity measurements and its standardization.

A (177)Lu primary standard was developed at the ENEA-INMRI in the frame of an international comparison organized by BIPM and piloted by NIST (USA). The CIEMAT/NIST method with (3)H standard source as tracer was used for standardizing a solution of (177)Lu. The activity value was compared also with the measurements of the same mother solution carried out by the 4πγ integral counting method. Particular efforts were made to identify and quantify the long-lived (177m)Lu impurity in the mother solution. The results obtained by the two methods are in good agreement within their standard uncertainties. The arithmetic mean of the two values is in good agreement with the Comparison Reference Value (CRV). By the new primary standard two well-type ionization chambers (ICs), one fixed and the other one portable, were calibrated with an uncertainty lower than 2%. These ICs are used for routinely applications in the activity measurements of short-lived radionuclides particularly useful for medical applications.

Intercomparison of methods for coincidence summing corrections in gamma-ray spectrometry--part II (volume sources).

The second part of an intercomparison of the coincidence summing correction methods is presented. This exercise concerned three volume sources, filled with liquid radioactive solution. The same experimental spectra, decay scheme and photon emission intensities were used by all the participants. The results were expressed as coincidence summing corrective factors for several energies of (152)Eu and (134)Cs, and different source-to-detector distances. They are presented and discussed.

Results of an international comparison for the activity measurement of 177Lu.

An international Key Comparison of (177)Lu has recently been carried out. Twelve laboratories performed assays for radioactivity content on aliquots of a common master solution of (177)Lu, leading to eleven results submitted for entry into the Key Comparison Database of the Mutual Recognition Arrangement. A proposed Comparison Reference Value (CRV) was calculated to be 3.288(4)MBq/g using all eleven results. Degrees of equivalence and their uncertainties were calculated for each laboratory based on the CRV. Most of the values reported by the participating laboratories were within 0.6% of the CRV.

Nucleon form factor studies at JLab.

The ratio of the electromagnetic proton elastic form factors, G(p)(E)/G(p)(M), has been measured at Jefferson Lab up to Q(2) approximately 9(GeV/c)(2), by using the CEBAF 6GeV electron beam, and revealing an unexpected and challenging physical behaviour. The 2014 scheduled 12GeV upgrade will allow the measurement of G(p)(E)/G(p)(M) up to Q(2) approximately 15(GeV/c)(2), by taking advantage of the new large-acceptance forward spectrometer Super BigBite (SBS) in Hall A. Measurements of neutron form factors in the region around 10(GeV/c)(2), where quark confinement plays an important role, are expected to show the behaviour already observed in the proton case.

Intercomparison of methods for coincidence summing corrections in gamma-ray spectrometry.

A comparison of the coincidence summing correction methods is presented. Since there are several ways for computing these corrections, each method has advantages and drawbacks that could be compared. This part of the comparison was restricted to point sources. The same experimental spectra, decay scheme and photon emission intensities were used by all the participants. The results were expressed as coincidence summing correction factors for several energies of (152)Eu and (134)Cs, and three source-to-detector distances. They are presented and discussed.

Implementation of a new low cost detector for low intensity light pulses produced by a radioactive gamma-source.

The readout of a cheap scintillating fibre was implemented by means of a new solid-state device (Silicon Photomultiplier, SiPM), able to detect very tiny light pulses. The GEANT3.21 code was adopted to simulate the counting detection efficiency and the energy deposited inside the scintillating fibre due to the radiation of a radioactive gamma source. The results obtained show the capability to detect gamma rays producing as few as 3-4 photoelectrons. The new devices may have many applications in radioactivity metrology.

Simulation of radioactive decay in GEANT Monte Carlo codes: comparison between spectra and efficiencies computed with sch2for and G4RadioactiveDecay.

Two CERN Monte Carlo codes, i.e. GEANT3.21 and GEANT4, were compared. The specific routine (sch2for), implemented in GEANT3.21 to simulate a disintegration process, and the G4RadioactiveDecay class, provided by GEANT4, were used for the computation of the full-energy-peak and total efficiencies of several radionuclides. No reference to experimental data was involved. A level of agreement better than 1% for the total efficiency and a deviation lower than 3.5% for the full-energy-peak efficiencies were found.

Development of a primary standard for calibration of (64)Cu activity measurement systems.

A (64)Cu national primary standard, was developed by the National Institute for Ionising Radiation Metrology (INMRI) of the ENEA (ENEA-INMRI) using the CIEMAT/NIST method of 4pibeta liquid scintillation spectrometry with (3)H-standard efficiency tracing. Relatively short (64)Cu half-life is required for the work to be performed at the production site. It was produced at the Scanditronix MC40 Cyclotron of the Joint Research Centre (JRC) of the European Commission (Ispra, Italy) through the (64)Zn(d,2p) (64)Cu reaction. Significant efforts were made to identify and quantify the impurities of (61)Cu and (65)Zn in the mother solution, which were activated through the (64)Zn(d,alphan) (61)Cu and (64)Zn(d,p) (65)Zn reactions, respectively. To this purpose, a new procedure for the determination of pure beta-emitter impurities by the CIEMAT/NIST method has been applied. A transfer standard portable well-type ionisation chamber was also calibrated with minimum uncertainty.

An intercomparison of Monte Carlo codes used in gamma-ray spectrometry.

In an intercomparison exercise, the Monte Carlo codes most commonly used in gamma-ray spectrometry today were compared with each other in order to gauge the differences between them in terms of typical applications. No reference was made to experimental data; instead, the aim was to confront the codes with each other, as they were applied to the calculation of full-energy-peak and total efficiencies. Surprising differences between the results of different codes were revealed.

Random-summing correction and pile-up rejection in the sum-peak method.

The sum-peak counting method was applied for 125I absolute activity measurement. Count rate-dependent corrections for random summing and dead time effects were experimentally determined at different count rates and in several experimental conditions. Two NaI(Tl) crystals of different volumes were used. They were connected to pulse recording systems with different characteristics, with or without pile-up rejection live-time corrector circuits (PUR/LTC). A theoretical model was proposed to explain the different behaviours found experimentally. It is shown that count rate-dependent effects are drastically reduced by the use of PUR/LTC.