Optical probing of ultrafast laser-induced solid-to-overdense-plasma transitions.

Understanding the solid target dynamics resulting from the interaction with an ultrashort laser pulse is a challenging fundamental multi-physics problem involving atomic and solid-state physics, plasma physics, and laser physics. Knowledge of the initial interplay of the underlying processes is essential to many applications ranging from low-power laser regimes like laser-induced ablation to high-power laser regimes like laser-driven ion acceleration. Accessing the properties of the so-called pre-plasma formed as the laser pulse's rising edge ionizes the target is complicated from the theoretical and experimental point of view, and many aspects of this laser-induced transition from solid to overdense plasma over picosecond timescales are still open questions. On the one hand, laser-driven ion acceleration requires precise control of the pre-plasma because the efficiency of the acceleration process crucially depends on the target properties at the arrival of the relativistic intensity peak of the pulse. On the other hand, efficient laser ablation requires, for example, preventing the so-called "plasma shielding". By capturing the dynamics of the initial stage of the interaction, we report on a detailed visualization of the pre-plasma formation and evolution. Nanometer-thin diamond-like carbon foils are shown to transition from solid to plasma during the laser rising edge with intensities < 1016 W/cm². Single-shot near-infrared probe transmission measurements evidence sub-picosecond dynamics of an expanding plasma with densities above 1023 cm-3 (about 100 times the critical plasma density). The complementarity of a solid-state interaction model and kinetic plasma description provides deep insight into the interplay of initial ionization, collisions, and expansion.

Selecting two-photon sequential ionization pathways in H2 through harmonic filtering.

Recent experiments in gas-phase molecules have shown the versatility of using attosecond pulse trains combined with IR femtosecond pulses to track and control excitation and ionization yields on the attosecond timescale. The interplay between electron and nuclear motions drives the light-induced transitions favoring specific reaction paths, so that the time delay between the pulses can be used as the tracking parameter or as a control knob to manipulate the molecular dynamics. Here, we present ab initio simulations on the hydrogen molecule to demonstrate that by filtering the high harmonics in an attosecond pulse train one can quench or enhance specific quantum paths thus dictating the outcome of the reaction. It is then possible to discriminate the dominant sequential processes in two-photon ionization, as for example molecular excitation followed by ionization or the other way around. More interestingly, frequency filters can be employed to steer the one- and two-photon yields to favor electron emission in a specific direction.