An ultra-narrow linewidth solution-processed organic laser.

Optically pumped lasers based on solution-processed thin-film gain media have recently emerged as low-cost, broadly tunable, and versatile active photonics components that can fit any substrate and are useful for, e.g., chemo- or biosensing or visible spectroscopy. Although single-mode operation has been demonstrated in various resonator architectures with a large variety of gain media-including dye-doped polymers, organic semiconductors, and, more recently, hybrid perovskites-the reported linewidths are typically on the order of a fraction of a nanometer or broader, i.e., the coherence lengths are no longer than a few millimeters, which does not enable high-resolution spectroscopy or coherent sensing. The linewidth is fundamentally constrained by the short photon cavity lifetime in the standard resonator geometries. We demonstrate here a novel structure for an organic thin-film solid-state laser that is based on a vertical external cavity, wherein a holographic volume Bragg grating ensures both spectral selection and output coupling in an otherwise very compact (∼cm3) design. Under short-pulse (0.4 ns) pumping, Fourier-transform-limited laser pulses are obtained, with a full width at half-maximum linewidth of 900 MHz (1.25 pm). Using 20-ns-long pump pulses, the linewidth can be further reduced to 200 MHz (0.26 pm), which is four times above the Fourier limit and corresponds to an unprecedented coherence length of 1 m. The concept is potentially transferrable to any type of thin-film laser and can be ultimately made tunable; it also represents a very compact alternative to bulky grating systems in dye lasers.

Thermal effects in thin-film organic solid-state lasers.

With the recent development of organic solid-state lasers (OSSLs) architectures enabling power scaling and progresses towards continuous-wave operation, the question of thermal effects now arises in OSSLs. In this paper, a Rhodamine 640-PMMA based vertical external cavity surface emitting organic laser is investigated. A thermal microscope is used to record temperature maps at the organic thin film surface during laser action; those maps are compared with time-resolved finite element thermal simulations. The measured and simulated peak temperature rises are in good accordance and are shown to remain below 10 K in standard operating conditions, showing a negligible impact on performance. The validated model is used to investigate typical OSSL structures from the literature, in a virtual high average power regime, and up to the CW regime. It is shown that whenever true CW organic lasing will be realized, significant thermal effects will have to be considered and properly managed.

Implementation of PT symmetric devices using plasmonics: principle and applications.

The so-called PT symmetric devices, which feature ε((-x)) = ε((x))* associated with parity-time symmetry, incorporate both gain and loss and can present a singular eigenvalue behaviour around a critical transition point. The scheme, typically based on co-directional coupled waveguides, is here transposed to the case of variable gain on one arm with fixed losses on the other arm. In this configuration, the scheme exploits the full potential of plasmonics by making a beneficial use of their losses to attain a critical regime that makes switching possible with much lowered gain excursions. Practical implementations are discussed based on existing attempts to elaborate coupled waveguide in plasmonics, and based also on the recently proposed hybrid plasmonics waveguide structure with a small low-index gap, the PIROW (Plasmonic Inverse-Rib Optical Waveguide).

Highly efficient, diffraction-limited laser emission from a vertical external-cavity surface-emitting organic laser.

We report on a solid-state laser structure functioning as the organic counterpart of a vertical external-cavity surface-emitting laser (VECSEL) design. The gain medium is a poly(methyl methacrylate) film doped with Rhodamine 640, spin casted onto the high-reflectivity mirror of a plano-concave resonator. Upon pumping by 7 ns pulses at 532 nm, a diffraction-limited beam (M(2)=1) was obtained, with a conversion efficiency of 43%; higher peak powers (2 kW) could be attained when resorting to shorter (0.5 ns) pump pulses. The spectrum was controlled by the thickness of the active layer playing the role of an intracavity etalon; tunability is demonstrated at over and up to 20 nm.