Quantum cascade laser-based mid-IR frequency metrology system with ultra-narrow linewidth and 1 × 10⁻¹³-level frequency instability.

We demonstrate a powerful tool for high-resolution mid-IR spectroscopy and frequency metrology with quantum cascade lasers (QCLs). We have implemented frequency stabilization of a QCL to an ultra-low expansion (ULE) reference cavity, via upconversion to the near-IR spectral range, at a level of 1×10(-13). The absolute frequency of the QCL is measured relative to a hydrogen maser, with instability <1×10(-13) and inaccuracy 5×10(-13), using a frequency comb phase stabilized to an independent ultra-stable laser. The QCL linewidth is determined to be 60 Hz, dominated by fiber noise. Active suppression of fiber noise could result in sub-10 Hz linewidth.

Silicon single-crystal cryogenic optical resonator: erratum.

We correct fit formulas from a previous paper [Opt. Lett.39, 3242 (2014)10.1364/OL39.005896OPLEDP0146-9592] for the coefficient of thermal expansion αreson(T).

A compact, robust, and transportable ultra-stable laser with a fractional frequency instability of 1 × 10(-15.).

We present a compact and robust transportable ultra-stable laser system with minimum fractional frequency instability of 1 × 10(-15) at integration times between 1 and 10 s. The system was conceived as a prototype of a subsystem of a microwave-optical local oscillator to be used on the satellite mission Space-Time Explorer and QUantum Equivalence Principle Space Test (STE-QUEST) (http://sci.esa.int/ste-quest/). It was therefore designed to be compact, to sustain accelerations occurring during rocket launch, to exhibit low vibration sensitivity, and to reach a low frequency instability. Overall dimensions of the optical system are 40 cm × 20 cm × 30 cm. The acceleration sensitivities of the optical frequency in the three directions were measured to be 1.7 × 10(-11)/g, 8.0 × 10(-11)/g, and 3.9 × 10(-10)/g, and the absolute frequency instability was determined via a three-cornered hat measurement. Two additional cavity-stabilized lasers were used for this purpose, one of which had an instability σy < 4 × 10(-16) at 1 s integration time. The design is also appropriate and useful for terrestrial applications.

Silicon single-crystal cryogenic optical resonator.

We report on the demonstration and characterization of a silicon optical resonator for laser frequency stabilization, operating in the deep cryogenic regime at temperatures as low as 1.5 K. Robust operation was achieved, with absolute frequency drift less than 20 Hz over 1 h. This stability allowed sensitive measurements of the resonator thermal expansion coefficient (α). We found that α=4.6×10(-13) K(-1) at 1.6 K. At 16.8 K α vanishes, with a derivative equal to -6×10(-10) K(-2). The temperature of the resonator was stabilized to a level below 10 µK for averaging times longer than 20 s. The sensitivity of the resonator frequency to a variation of the laser power was also studied. The corresponding sensitivities and the expected Brownian noise indicate that this system should enable frequency stabilization of lasers at the low-10(-17) level.

Radiation hardness of high-Q silicon nitride microresonators for space compatible integrated optics.

Integrated optics has distinct advantages for applications in space because it integrates many elements onto a monolithic, robust chip. As the development of different building blocks for integrated optics advances, it is of interest to answer the important question of their resistance with respect to ionizing radiation. Here we investigate effects of proton radiation on high-Q (θ(106)) silicon nitride microresonators formed by a waveguide ring. We show that the irradiation with high-energy protons has no lasting effect on the linear optical losses of the microresonators.

Spectrally narrow, long-term stable optical frequency reference based on a Eu3+:Y2SiO5 crystal at cryogenic temperature.

Using an ultrastable continuous-wave laser at 580 nm we performed spectral hole burning of Eu(3+):Y(2)SiO(5) at a very high spectral resolution. The essential parameters determining the usefulness as a macroscopic frequency reference, linewidth, temperature sensitivity, and long-term stability, were characterized using a H-maser stabilized frequency comb. Spectral holes with a linewidth as low as 6 kHz were observed and the upper limit of the drift of the hole frequency was determined to be 5±3 mHz/s. We discuss the necessary requirements for achieving ultrahigh stability in laser frequency stabilization to these spectral holes.

Non-degenerated nonclassical photon pairs in a hot atomic ensemble.

We experimentally demonstrate the generation of non-degenerate nonclassical paired photons in a hot atomic ensemble using off-axis four-wave mixing. The time-resolved second-order correlated function between the Stokes photon and the anti-Stokes photon is given. The two-photon correlation between the photons obtained in this experiment is 1.87+/- 0.04, which leads to the violation of Cauchy-Schwarz inequality by a factor of 1.69+/- 0.14.