Time/frequency-domain characterization of a mid-IR DFG frequency comb via two-photon and heterodyne detection.

Mid-infrared frequency combs are nowadays well-appreciated sources for spectroscopy and frequency metrology. Here, a comprehensive approach for characterizing a difference-frequency-generated mid-infrared frequency comb (DFG-comb) both in the time and in the frequency domain is presented. An autocorrelation scheme exploiting mid-infrared two-photon detection is used for characterizing the pulse width and to verify the optimal compression of the generated pulses reaching a pulse duration (FWHM) as low as 196 fs. A second scheme based on mid-infrared heterodyne detection employing two independent narrow-linewidth quantum cascade lasers (QCLs) is used for frequency-narrowing the modes of the DFG-comb down to 9.4 kHz on a 5-ms timescale.

Direct imaging of molecular symmetry by coherent anti-stokes Raman scattering.

Nonlinear optical methods, such as coherent anti-Stokes Raman scattering and stimulated Raman scattering, are able to perform label-free imaging, with chemical bonds specificity. Here we demonstrate that the use of circularly polarized light allows to retrieve not only the chemical nature but also the symmetry of the probed sample, in a single measurement. Our symmetry-resolved scheme offers simple access to the local organization of vibrational bonds and as a result provides enhanced image contrast for anisotropic samples, as well as an improved chemical selectivity. We quantify the local organization of vibrational bonds on crystalline and biological samples, thus providing information not accessible by spontaneous Raman and stimulated Raman scattering techniques. This work stands for a symmetry-resolved contrast in vibrational microscopy, with potential application in biological diagnostic.

Interferometric background reduction for femtosecond stimulated Raman scattering loss spectroscopy.

We present a purely optical method for background suppression in nonlinear spectroscopy based on linear interferometry. Employing an unbalanced Sagnac interferometer, an unprecedented background reduction of 17 dB over a broad bandwidth of 60 THz (2000 cm(-1)) is achieved and its application to femtosecond stimulated Raman scattering loss spectroscopy is demonstrated. Apart from raising the signal-to-background ratio in the measurement of the Raman intensity spectrum, this interferometric method grants access to the spectral phase of the resonant χ(3) contribution. The spectral phase becomes apparent as a dispersive lineshape and is reproduced numerically with a simple oscillator model.

Compensation of spatial inhomogeneities in a cavity soliton laser using a spatial light modulator.

Dissipative solitons are self-localized states which can exist anywhere in a system with translational symmetry, but in real systems this translational symmetry is usually broken due to parasitic inhomogeneities leading to spatial disorder, pinning the soliton positions. We discuss the effects of semiconductor growth induced spatial disorder on the operation of a cavity soliton laser based on a vertical-cavity surface-emitting laser (VCSEL). We show that a refractive index variation induced by an external, suitably spatially modulated laser beam can be used to counteract the inherent disorder. In particular, it is demonstrated experimentally that the threshold of one cavity soliton can be lowered without influencing other cavity solitons making two solitons simultaneously bistable which were not without control. This proof of principle paves the way to achieve full control of large numbers of cavity solitons at the same time.

A route to sub-diffraction-limited CARS Microscopy.

We theoretically investigate a scheme to obtain sub-diffraction-limited resolution in coherent anti-Stokes Raman scattering (CARS) microscopy. We find using density matrix calculations that the rise of vibrational (Raman) coherence can be strongly suppressed, and thereby the emission of CARS signals can be significantly reduced, when pre-populating the corresponding vibrational state through an incoherent process. The effectiveness of pre-populating the vibrational state of interest is investigated by considering the excitation of a neighbouring vibrational (control) state through an intense, mid-infrared control laser. We observe that, similar to the processes employed in stimulated emission depletion microscopy, the CARS signal exhibits saturation behaviour if the transition rate between the vibrational and the control state is large. Our approach opens up the possibility of achieving chemically selectivity sub-diffraction-limited spatially resolved imaging.

Gradient induced motion control of drifting solitary structures in a nonlinear optical single feedback experiment.

We realize an absolute position control of drifting dissipative optical solitons by injecting an incoherent amplitude parameter gradient onto the nonlinear optical system. This allows for two-dimensional, arbitrary control patterns. The control of the soliton drift velocity is studied applying a periodic, hexagonally shaped modulation. The guiding of dissipative solitons by one- and two-dimensional parameter modulations is demonstrated. Furthermore, one-dimensional, line-shaped parameter modulations are designed to act as barriers for dissipative solitons, allowing implementations of position selectors for solitons. The interaction of dissipative optical solitons with barriers is studied for different barrier parameters.

Dynamic and static position control of optical feedback solitons.

We report on the experimental implementation of an external control for optical feedback solitons using incoherent spatial intensity distributions in a liquid crystal light valve (LCLV) optical single feedback system. The external control provides excellent experimental possibilities for static and dynamic control of the lateral positions of the optical feedback solitons which will be demonstrated. Particularly, the influence of different gradients onto the drift motion of spatial solitons is experimentally investigated in detail. In agreement with theoretical predictions, the drift velocity of the soliton increases according to the steepness of the gradient. Additionally, a completely incoherent addressing scheme including creation and erasure of feedback solitons is demonstrated for the LCLV setup.