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1.
Int J Mol Sci ; 19(2)2018 Feb 13.
Artigo em Inglês | MEDLINE | ID: mdl-29438349

RESUMO

Ionic liquids have recently been used as means of modulating the charge carrier properties of cuprates. The mechanism behind it, however, is still a matter of debate. In this paper we report experiments on ionic liquid gated ultrathin La2-xSrxCuO4 films. Our results show that the electrostatic part of gating has limited influence in the conductance of the cuprate in the gate voltage range of 0 to - 2 V. A non-electrostatic mechanism takes over for gate voltages below - 2 V. This mechanism most likely changes the oxygen concentration of the film. The results presented are in line with previous X-ray based studies on ionic liquid gating induced oxygenation of the cuprate materials YBa2Cu3O7-x and La2-xSrxCuO4.


Assuntos
Líquidos Iônicos/química , Cobre/química , Condutividade Elétrica , Lantânio/química , Óxidos/química , Oxigênio/química , Eletricidade Estática , Estrôncio/química
2.
Science ; 349(6253): 1202-5, 2015 Sep 11.
Artigo em Inglês | MEDLINE | ID: mdl-26359398

RESUMO

An array of superconducting islands placed on a normal metal film offers a tunable realization of nanopatterned superconductivity. This system enables investigation of the nature of competing vortex states and phase transitions between them. A square array creates the eggcrate potential in which magnetic field-induced vortices are frozen into a vortex insulator. We observed a vortex insulator-vortex metal transition driven by the applied electric current and determined critical exponents that coincided with those for thermodynamic liquid-gas transition. Our findings offer a comprehensive description of dynamic critical behavior and establish a deep connection between equilibrium and nonequilibrium phase transitions.

3.
Sci Rep ; 3: 2383, 2013.
Artigo em Inglês | MEDLINE | ID: mdl-23924946

RESUMO

Despite intensive research a physical explanation of high Tc superconductors remains elusive. One reason for this is that these materials have generally a very complex structure making useless theoretical models for a homogeneous system. Little is known on the control of the critical temperature by the space disposition of defects because of lack of suitable experimental probes. X-ray diffraction and neutron scattering experiments used to investigate y oxygen dopants in YBa2Cu3O6+y lack of spatial resolution. Here we report the spatial imaging of dopants distribution inhomogeneity in YBa2Cu3O6.67 using scanning nano X-ray diffraction. By changing the X-ray beam size from 1 micron to 300 nm of diameter, the lattice inhomogeneity increases. The ordered oxygen puddles size distribution vary between 6-8 nm using 1 × 1 µm(2) beam, while it is between 5-12 nm with a fat tail using the 300 × 300 nm(2) beam. The increased inhomogeneity at the nanoscale points toward a network of superconducting puddles made of ordered oxygen interstitials.


Assuntos
Cobre/química , Oxigênio/química , Condutividade Elétrica , Teste de Materiais
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