Model of Active Solids: Rigid Body Motion and Shape-Changing Mechanisms.

Active solids such as cell collectives, colloidal clusters, and active metamaterials exhibit diverse collective phenomena, ranging from rigid body motion to shape-changing mechanisms. The nonlinear dynamics of such active materials remains, however, poorly understood when they host zero-energy deformation modes and when noise is present. Here, we show that stress propagation in a model of active solids induces the spontaneous actuation of multiple soft floppy modes, even without exciting vibrational modes. By introducing an adiabatic approximation, we map the dynamics onto an effective Landau free energy, predicting mode selection and the onset of collective dynamics. These results open new ways to study and design living and robotic materials with multiple modes of locomotion and shape change.

Elasticity of self-organized frustrated disordered spring networks.

There have been some interesting recent advances in understanding the notion of mechanical disorder in structural glasses and the statistical mechanics of these systems' low-energy excitations. Here we contribute to these advances by studying a minimal model for structural glasses' elasticity in which the degree of mechanical disorder-as characterized by recently introduced dimensionless quantifiers-is readily tunable over a very large range. We comprehensively investigate a number of scaling laws observed for various macro, meso and microscopic elastic properties, and rationalize them using scaling arguments. Interestingly, we demonstrate that the model features the universal quartic glassy vibrational density of states as seen in many atomistic and molecular models of structural glasses formed by cooling a melt. The emergence of this universal glassy spectrum highlights the role of self-organization (toward mechanical equilibrium) in its formation, and elucidates why models featuring structural frustration alone do not feature the same universal glassy spectrum. Finally, we discuss relations to existing work in the context of strain stiffening of elastic networks and of low-energy excitations in structural glasses, in addition to future research directions.

Avalanche properties at the yielding transition: from externally deformed glasses to active systems.

We investigated the yielding phenomenon in the quasistatic limit using numerical simulations of soft particles. Two different deformation scenarios, simple shear (passive) and self-random force (active), and two interaction potentials were used. Our approach reveals that the exponents describing the avalanche distribution are universal within the margin of error, showing consistency between the passive and active systems. This indicates that any differences observed in the flow curves may have resulted from a dynamic effect on the avalanche propagation mechanism. The evolution time required to reach a steady state differs significantly between active and passive scenarios under similar conditions. However, we demonstrated that plastic avalanches under athermal quasistatic simulation dynamics display a similar scaling relationship between avalanche size and relaxation time, which cannot explain the different flow curves.

Elasticity and rheology of auxetic granular metamaterials.

The flowing, jamming, and avalanche behavior of granular materials is satisfyingly universal and vexingly hard to tune: A granular flow is typically intermittent and will irremediably jam if too confined. Here, we show that granular metamaterials made from particles with a negative Poisson's ratio yield more easily and flow more smoothly than ordinary granular materials. We first create a collection of auxetic grains based on a re-entrant mechanism and show that each grain exhibits a negative Poisson's ratio regardless of the direction of compression. Interestingly, we find that the elastic and yielding properties are governed by the high compressibility of granular metamaterials: At a given confinement, they exhibit lower shear modulus, lower yield stress, and more frequent, smaller avalanches than materials made from ordinary grains. We further demonstrate that granular metamaterials promote flow in more complex confined geometries, such as intruder and hopper geometries, even when the packing contains only a fraction of auxetic grains. Moreover, auxetic granular metamaterials exhibit enhanced impact absorption. Our findings blur the boundary between complex fluids and metamaterials and could help in scenarios that involve process, transport, and reconfiguration of granular materials.

Critical yielding rheology: from externally deformed glasses to active systems.

We use extensive computer simulations to study the yielding transition under two different loading schemes: standard simple shear dynamics and self-propelled dense active systems. In the active systems, a yielding transition toward an out-of-equilibrium flowing state known as the liquid phase is observed when self-propulsion is increased. The range of self-propulsions in which this pure liquid regime exists appears to vanish upon approaching the so-called 'jamming point' at which the solidity of soft-sphere packings is lost. Such an 'active yielding' transition shares similarities with the generic yielding transition for shear flows. A Herschel-Bulkley law is observed along the liquid regime in both loading scenarios, with a clear difference in the critical scaling exponents between the two, suggesting the existence of different universality classes for the yielding transition under different driving conditions. In addition, we present the direct measurements of growing length and time scales for both driving scenarios. A comparison with theoretical predictions from the recent literature reveals poor agreement with our numerical results.

Elastic weak turbulence: From the vibrating plate to the drum.

Weak wave turbulence has been observed on a thin elastic plates since the work by Düring et al. [Phys. Rev. Lett. 97, 025503 (2006)PRLTAO0031-900710.1103/PhysRevLett.97.025503]. Here we report theoretical, experimental, and numerical studies of wave turbulence in a forced thin elastic plate submitted to increasing tension. When increasing the tension (or decreasing the bending stiffness of the plate) the plate evolves progressively from a plate into an elastic membrane as in drums. We first consider a thin plate and increase the tension in experiments and numerical simulations. We observe that the system remains in a state of weak turbulence of weakly dispersive waves. This observation is in contrast with what has been observed in water waves when decreasing the water depth, which also changes the waves from dispersive to weakly dispersive. The weak turbulence observed in the deep water case evolves into a solitonic regime. Here no such transition is observed for the stretched plate. We then apply the weak turbulence theory to the membrane case and show with numerical simulations that indeed the weak turbulence framework remains valid for the membrane and no formation of singular structures (shocks) should be expected in contrast with acoustic wave turbulence.

Exact result in strong wave turbulence of thin elastic plates.

An exact result concerning the energy transfers between nonlinear waves of a thin elastic plate is derived. Following Kolmogorov's original ideas in hydrodynamical turbulence, but applied to the Föppl-von Kármán equation for thin plates, the corresponding Kármán-Howarth-Monin relation and an equivalent of the 4/5-Kolmogorov's law is derived. A third-order structure function involving increments of the amplitude, velocity, and the Airy stress function of a plate, is proven to be equal to -ɛℓ, where ℓ is a length scale in the inertial range at which the increments are evaluated and ɛ the energy dissipation rate. Numerical data confirm this law. In addition, a useful definition of the energy fluxes in Fourier space is introduced and proven numerically to be flat in the inertial range. The exact results derived in this Rapid Communication are valid for both weak and strong wave turbulence. They could be used as a theoretical benchmark of new wave-turbulence theories and to develop further analogies with hydrodynamical turbulence.

Erratum: Statistics and Properties of Low-Frequency Vibrational Modes in Structural Glasses [Phys. Rev. Lett. 117, 035501 (2016)].

This corrects the article DOI: 10.1103/PhysRevLett.117.035501.

Effect of particle collisions in dense suspension flows.

We study nonlocal effects associated with particle collisions in dense suspension flows, in the context of the Affine Solvent Model, known to capture various aspects of the jamming transition. We show that an individual collision changes significantly the velocity field on a characteristic volume Ω_{c}∼1/δz that diverges as jamming is approached, where δz is the deficit in coordination number required to jam the system. Such an event also affects the contact forces between particles on that same volume Ω_{c}, but this change is modest in relative terms, of order f_{coll}∼f[over ¯]^{0.8}, where f[over ¯] is the typical contact force scale. We then show that the requirement that coordination is stationary (such that a collision has a finite probability to open one contact elsewhere in the system) yields the scaling of the viscosity (or equivalently the viscous number) with coordination deficit δz. The same scaling result was derived [E. DeGiuli, G. Düring, E. Lerner, and M. Wyart, Phys. Rev. E 91, 062206 (2015)PLEEE81539-375510.1103/PhysRevE.91.062206] via different arguments making an additional assumption. The present approach gives a mechanistic justification as to why the correct finite size scaling volume behaves as 1/δz and can be used to recover a marginality condition known to characterize the distributions of contact forces and gaps in jammed packings.

Statistics and Properties of Low-Frequency Vibrational Modes in Structural Glasses.

Low-frequency vibrational modes play a central role in determining various basic properties of glasses, yet their statistical and mechanical properties are not fully understood. Using extensive numerical simulations of several model glasses in three dimensions, we show that in systems of linear size L sufficiently smaller than a crossover size L_{D}, the low-frequency tail of the density of states follows D(ω)∼ω^{4} up to the vicinity of the lowest Goldstone mode frequency. We find that the sample-to-sample statistics of the minimal vibrational frequency in systems of size L

Self-similar formation of an inverse cascade in vibrating elastic plates.

The dynamics of random weakly nonlinear waves is studied in the framework of vibrating thin elastic plates. Although it has been previously predicted that no stationary inverse cascade of constant wave action flux could exist in the framework of wave turbulence for elastic plates, we present substantial evidence of the existence of a time-dependent inverse cascade, opening up the possibility of self-organization for a larger class of systems. This inverse cascade transports the spectral density of the amplitude of the waves from short up to large scales, increasing the distribution of long waves despite the short-wave fluctuations. This dynamics appears to be self-similar and possesses a power-law behavior in the short-wavelength limit which significantly differs from the exponent obtained via a Kolmogorov dimensional analysis argument. Finally, we show explicitly a tendency to build a long-wave coherent structure in finite time.

Length scales and self-organization in dense suspension flows.

Dense non-Brownian suspension flows of hard particles display mystifying properties: As the jamming threshold is approached, the viscosity diverges, as well as a length scale that can be identified from velocity correlations. To unravel the microscopic mechanism governing dissipation and its connection to the observed correlation length, we develop an analogy between suspension flows and the rigidity transition occurring when floppy networks are pulled, a transition believed to be associated with the stress stiffening of certain gels. After deriving the critical properties near the rigidity transition, we show numerically that suspension flows lie close to it. We find that this proximity causes a decoupling between viscosity and the correlation length of velocities ξ, which scales as the length l(c) characterizing the response to a local perturbation, previously predicted to follow l(c)∼ 1/sqrt[z(c)-z] ∼ p(0.18), where p is the dimensionless particle pressure, z is the coordination of the contact network made by the particles, and z(c) is twice the spatial dimension. We confirm these predictions numerically and predict the existence of a larger length scale l(r)∼sqrt[p] with mild effects on velocity correlation and of a vanishing strain scale δγ ∼ 1/p that characterizes decorrelation in flow.

Effects of coordination and pressure on sound attenuation, boson peak and elasticity in amorphous solids.

Connectedness and applied stress strongly affect elasticity in solids. In various amorphous materials, mechanical stability can be lost either by reducing connectedness or by increasing pressure. We present an effective medium theory of elasticity that extends previous approaches by incorporating the effect of compression, of amplitude e, allowing one to describe quantitative features of sound propagation, transport, the boson peak, and elastic moduli near the elastic instability occurring at a compression ec. The theory disentangles several frequencies characterizing the vibrational spectrum: the onset frequency where strongly-scattered modes appear in the vibrational spectrum, the pressure-independent frequency ω* where the density of states displays a plateau, the boson peak frequency ωBP found to scale as , and the Ioffe-Regel frequency ωIR where scattering length and wavelength become equal. We predict that sound attenuation crosses over from ω(4) to ω(2) behaviour at ω0, consistent with observations in glasses. We predict that a frequency-dependent length scale ls(ω) and speed of sound ν(ω) characterize vibrational modes, and could be extracted from scattering data. One key result is the prediction of a flat diffusivity above ω0, in agreement with previously unexplained observations. We find that the shear modulus does not vanish at the elastic instability, but drops by a factor of 2. We check our predictions in packings of soft particles and study the case of covalent networks and silica, for which we predict ωIR ≈ ωBP. Overall, our approach unifies sound attenuation, transport and length scales entering elasticity in a single framework where disorder is not the main parameter controlling the boson peak, in agreement with observations. This framework leads to a phase diagram where various glasses can be placed, connecting microscopic structure to vibrational properties.

Breakdown of continuum elasticity in amorphous solids.

We show numerically that the response of simple amorphous solids (elastic networks and particle packings) to a local force dipole is characterized by a lengthscale lc that diverges as unjamming is approached as lc ∼ (z - 2d)(-1/2), where z ≥ 2d is the mean coordination, and d is the spatial dimension, at odds with previous numerical claims. We also show how the magnitude of the lengthscale lc is amplified by the presence of internal stresses in the disordered solid. Our data suggests a divergence of lc ∼ (pc - p)(-1/4) with proximity to a critical internal stress pc at which soft elastic modes become unstable.

Why glass elasticity affects the thermodynamics and fragility of supercooled liquids.

Supercooled liquids are characterized by their fragility: The slowing down of the dynamics under cooling is more sudden and the jump of specific heat at the glass transition is generally larger in fragile liquids than in strong ones. Despite the importance of this quantity in classifying liquids, explaining what aspects of the microscopic structure controls fragility remains a challenge. Surprisingly, experiments indicate that the linear elasticity of the glass--a purely local property of the free energy landscape--is a good predictor of fragility. In particular, materials presenting a large excess of soft elastic modes, the so-called boson peak, are strong. This is also the case for network liquids near the rigidity percolation, known to affect elasticity. Here we introduce a model of the glass transition based on the assumption that particles can organize locally into distinct configurations that are coupled spatially via elasticity. The model captures the mentioned observations connecting elasticity and fragility. We find that materials presenting an abundance of soft elastic modes have little elastic frustration: Energy is insensitive to most directions in phase space, leading to a small jump of specific heat. In this framework strong liquids turn out to lie the closest to a critical point associated with a rigidity or jamming transition, and their thermodynamic properties are related to the problem of number partitioning and to Hopfield nets in the limit of small memory.

A unified framework for non-brownian suspension flows and soft amorphous solids.

While the rheology of non-brownian suspensions in the dilute regime is well understood, their behavior in the dense limit remains mystifying. As the packing fraction of particles increases, particle motion becomes more collective, leading to a growing length scale and scaling properties in the rheology as the material approaches the jamming transition. There is no accepted microscopic description of this phenomenon. However, in recent years it has been understood that the elasticity of simple amorphous solids is governed by a critical point, the unjamming transition where the pressure vanishes, and where elastic properties display scaling and a diverging length scale. The correspondence between these two transitions is at present unclear. Here we show that for a simple model of dense flow, which we argue captures the essential physics near the jamming threshold, a formal analogy can be made between the rheology of the flow and the elasticity of simple networks. This analogy leads to a new conceptual framework to relate microscopic structure to rheology. It enables us to define and compute numerically normal modes and a density of states. We find striking similarities between the density of states in flow, and that of amorphous solids near unjamming: both display a plateau above some frequency scale ω(∗) ∼ |z(c) - z|, where z is the coordination of the network of particle in contact, z(c) = 2D where D is the spatial dimension. However, a spectacular difference appears: the density of states in flow displays a single mode at another frequency scale ω(min) ≪ ω(∗) governing the divergence of the viscosity.

Symmetry induced four-wave capillary wave turbulence.

We report theoretical and experimental results on 4-wave capillary wave turbulence. A system consisting of two immiscible and incompressible fluids of the same density can be written in a Hamiltonian way for the conjugated pair (eta, Psi). Adding the symmetry z --> -z, the set of capillary waves display a Kolmogorov-Zakharov spectrum k(-4) in wave vector space and f(-8/3) in the frequency domain. The wave system is studied experimentally with two immiscible fluids of almost equal densities (water and silicon oil) where the capillary surface waves are excited by a low-frequency random forcing. The probability density function of the local wave amplitude shows a quasi-Gaussian behavior and the power spectral density is shows a power-law behavior in frequency with a slope of -2.75. Theoretical and experimental results are in fairly good agreement with each other.

Irreversibility and self-organization in hydrodynamic echo experiments.

We discuss the reversible-irreversible transition in low-Reynolds hydrodynamic systems driven by external cycling actuation. We introduce a set of models with no auto-organization, and show that a sharp crossover is obtained between a Lyapunov regime in which any noise source, such as thermal noise, is amplified exponentially, and a diffusive regime where this no longer holds. In the latter regime, groups of particles are seen to move cooperatively, yet no spatial organization occurs.

Weak turbulence for a vibrating plate: can one hear a Kolmogorov spectrum?

We study the long-time evolution of waves of a thin elastic plate in the limit of small deformation so that modes of oscillations interact weakly. According to the theory of weak turbulence (successfully applied in the past to plasma, optics, and hydrodynamic waves), this nonlinear wave system evolves at long times with a slow transfer of energy from one mode to another. We derive a kinetic equation for the spectral transfer in terms of the second order moment. We show that such a theory describes the approach to an equilibrium wave spectrum and represents also an energy cascade, often called the Kolmogorov-Zakharov spectrum. We perform numerical simulations that confirm this scenario.