A new setup for measurements of absolute saturation vapor pressures using a dynamical method: Experimental concept and validation.

We describe a new experimental system for direct measurements of the absolute saturation vapor pressures of liquid or solid samples. The setup allows the isolation of the sample under steady conditions in an ultra-high vacuum chamber, where the measurement of the sample's vapor pressure as a function of its temperature can be performed in a range around room temperature and in a pressure range defined only by the applied absolute pressure sensor. We characterize the setup and illustrate its capability to measure saturation vapor pressures as well as enthalpies of evaporation around room temperature with explicit measurements on four liquid compounds (diethyl phthalate, 1-decanol, 1-heptanol, and 1-hexanol) for which accurate vapor pressures have previously been reported.

Narrow-linewidth Fano microcavities with resonant subwavelength grating mirror.

We report on the theoretical and experimental investigations of optical microcavities consisting in the plane-plane arrangement of a broadband high-reflectivity mirror and a suspended one-dimensional grating mirror possessing a high-quality factor Fano resonance. By varying the length of these cavities from the millimeter to the few-micron range, we observe at short lengths the reduction of the spectral linewidth predicted to occur for such a Fano cavity as compared to a conventional broadband mirror cavity with the same length and internal losses. Such narrow linewidth and small modevolume microcavities with high-mechanical quality ultrathin mirrors will be attractive for a wide range of applications within optomechanics and sensing.

Polarization-independent optical spatial differentiation with a doubly-resonant one-dimensional guided-mode grating.

We report on the design and experimental characterization of a suspended silicon nitride subwavelength grating possessing a polarization-independent guided-mode resonance at oblique incidence. At this resonant wavelength we observe that the transverse intensity profile of the transmitted beam is consistent with a first-order spatial differentiation of the incident beam profile in the direction of the grating periodicity, regardless of the incident light polarization. These observations are corroborated by full numerical simulations. The simple one-dimensional and symmetric design, combined with the thinness and excellent mechanical properties of these essentially loss-free dieletric films, is attractive for applications in optical processing, sensing and optomechanics.

Collimation and finite-size effects in suspended resonant guided-mode gratings.

The optical transmission of resonant guided-mode gratings patterned on suspended silicon nitride thin films and illuminated at normal incidence with a Gaussian beam is investigated both experimentally and theoretically. Effects due to the beam focusing and its finite size are accounted for by a phenomenological coupled-mode model whose predictions are found to be in very good agreement with the experimentally measured spectra for various grating structures and beam sizes, and which allow for a detailed analysis of the respective magnitude of these effects. These results are highly relevant for the design and optimization of such suspended structured films that are widely used for photonics, sensing, and optomechanics applications.

Optical spatial differentiation with suspended subwavelength gratings.

We investigate first- and second-order spatial differentiation of an optical beam transverse profile using guided-mode resonances in thin, suspended subwavelength gratings. Highly reflective one-dimensional gratings are patterned on freestanding 200 nm-thick silicon nitride membranes using Electron Beam Lithography and plasma etching. The optical transmission of these gratings, designed for illumination with either TM or TE polarized light, are experimentally measured under normal and oblique incidence and found to be in excellent agreement with the predictions of an analytical coupled-mode model as well as Rigorous Coupled Wave Analysis numerical simulations. Intensity profiles consistent with high quality first- and second-order spatial differentiation of a Gaussian beam are observed in transmission at oblique and normal incidence, respectively. Such easy-to-fabricate, ultrathin and loss-free optical components may be attractive for beam shaping and optical information processing and computing.

Cavity Quantum Electrodynamics with Frequency-Dependent Reflectors.

We present a general framework for cavity quantum electrodynamics with strongly frequency-dependent mirrors. The method is applicable to a variety of reflectors exhibiting sharp internal resonances as can be realized, for example, with photonic-crystal mirrors or with two-dimensional atomic arrays around subradiant points. Our approach is based on a modification of the standard input-output formalism to explicitly include the dynamics of the mirror's internal resonance. We show how to directly extract the interaction parameters from the comparison with classical transfer matrix theory and how to treat the non-Markovian dynamics of the cavity field mode introduced by the mirror's internal resonance. As an application within optomechanics, we illustrate how a non-Markovian Fano-resonance cavity with a flexible photonic-crystal mirror can provide both sideband resolution as well as strong heating suppression in optomechanical cooling. This approach, amenable to a wide range of systems, opens up possibilities for using hybrid frequency-dependent reflectors in cavity quantum electrodynamics for engineering novel forms of light-matter interactions.

Microcavities with suspended subwavelength structured mirrors.

We investigate the optical properties of microcavities with suspended subwavelength structured mirrors, such as high-contrast gratings or two-dimensional photonic crystals slabs, and focus in particular on the regime in which the microcavity free-spectral range is larger than the width of a Fano resonance of the highly reflecting structured mirror. In this unusual regime, the transmission spectrum of the microcavity essentially consists in a single mode, whose linewidth can be significantly narrower than both the Fano resonance linewidth and the linewidth of an equally short cavity without structured mirror. This generic interference effect-occuring in any Fabry-Perot resonator with a strongly wavelength-dependent mirror-can be exploited for realizing small modevolume and high quality factor microcavities and, if high mechanical quality suspended structured thin films are used, for optomechanics and optical sensing applications.

Optomechanical characterization of silicon nitride membrane arrays.

We report on the optical and mechanical characterization of arrays of parallel micromechanical membranes. Pairs of high-tensile stress, 100 nm thick silicon nitride membranes are assembled parallel to each other with separations ranging from 8.5 to 200 µm. Their optical properties are accurately determined using transmission measurements under broadband and monochromatic illuminations, and the lowest vibrational mode frequencies and mechanical quality factors are determined interferometrically. The results and techniques demonstrated are promising for investigations of collective phenomena in optomechanical arrays.

Reconfigurable long-range phonon dynamics in optomechanical arrays.

We investigate periodic optomechanical arrays as reconfigurable platforms for engineering the coupling between multiple mechanical and electromagnetic modes and for exploring many-body phonon dynamics. Exploiting structural resonances in the coupling between light fields and collective motional modes of the array, we show that tunable effective long-range interactions between mechanical modes can be achieved. This paves the way towards the implementation of controlled phononic walks and heat transfer on densely connected graphs as well as the coherent transfer of excitations between distant elements of optomechanical arrays.

Strong coupling and long-range collective interactions in optomechanical arrays.

We investigate the collective optomechanics of an ensemble of scatterers inside a Fabry-Pérot resonator and identify an optimized configuration where the ensemble is transmissive, in contrast to the usual reflective optomechanics approach. In this configuration, the optomechanical coupling of a specific collective mechanical mode can be several orders of magnitude larger than the single-element case, and long-range interactions can be generated between the different elements since light permeates throughout the array. This new regime should realistically allow for achieving strong single-photon optomechanical coupling with massive resonators, realizing hybrid quantum interfaces, and exploiting collective long-range interactions in arrays of atoms or mechanical oscillators.

Pinning an ion with an intracavity optical lattice.

We report one-dimensional pinning of a single ion by an optical lattice. A standing-wave cavity produces the lattice potential along the rf-field-free axis of a linear Paul trap. The ion's localization is detected by measuring its fluorescence when excited by standing-wave fields with the same period, but different spatial phases. The experiments agree with an analytical model of the localization process, which we test against numerical simulations. For the best localization achieved, the ion's average coupling to the cavity field is enhanced from 50% to 81(3)% of its maximum possible value, and we infer that the ion is bound in a lattice well with over 97% probability.

Increasing entanglement between Gaussian states by coherent photon subtraction.

We experimentally demonstrate that the entanglement between Gaussian entangled states can be increased by non-Gaussian operations. Coherent subtraction of single photons from Gaussian quadrature-entangled light pulses, created by a nondegenerate parametric amplifier, produces delocalized states with negative Wigner functions and complex structures more entangled than the initial states in terms of negativity. The experimental results are in very good agreement with the theoretical predictions.

Femtosecond Ti:sapphire cryogenic amplifier with high gain and MHz repetition rate.

We demonstrate high gain amplification of 160-femtosecond pulses in a compact double-pass cryogenic Ti:sapphire amplifier. The setup involves a negative GVD mirrors recompression stage, and operates with a repetition rate between 0.2 and 4 MHz with a continuous pump laser. Amplification factors as high as 17 and 320 nJ Fourier-limited pulses are obtained at a 800 kHz repetition rate.