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1.
Sci Rep ; 11(1): 4090, 2021 Feb 18.
Artigo em Inglês | MEDLINE | ID: mdl-33603100

RESUMO

The superconducting systems emerging from topological insulators upon metal ion intercalation or application of high pressure are ideal for investigation of possible topological superconductivity. In this context, Sr-intercalated Bi[Formula: see text]Se[Formula: see text] is specially interesting because it displays pressure induced re-entrant superconductivity where the high pressure phase shows almost two times higher [Formula: see text] than the ambient superconducting phase ( [Formula: see text] K). Interestingly, unlike the ambient phase, the pressure-induced superconducting phase shows strong indication of unconventional superconductivity. However, since the pressure-induced phase remains inaccessible to spectroscopic techniques, the detailed study of the phase remained an unattained goal. Here we show that the high-pressure phase can be realized under a mesoscopic point contact, where transport spectroscopy can be used to probe the spectroscopic properties of the pressure-induced phase. We find that the point contact junctions on the high-pressure phase show unusual response to magnetic field supporting the possibility of unconventional superconductivity.

2.
J Phys Condens Matter ; 31(8): 085701, 2019 Feb 27.
Artigo em Inglês | MEDLINE | ID: mdl-30524072

RESUMO

The type II Dirac semimetal PdTe[Formula: see text] is unique in the family of topological parent materials because it displays a superconducting ground state below 1.7 K. Despite wide speculation on the possibility of an unconventional topological superconducting phase, tunneling and heat capacity measurements revealed that the superconducting phase of PdTe[Formula: see text] follows predictions of the microscopic theory of Bardeen, Cooper and Schrieffer for conventional superconductors. The superconducting phase in PdTe[Formula: see text] is further interesting because it also displays properties that are characteristic of type-I superconductors and are generally unexpected for binary compounds. Here, from scanning tunneling spectroscopic measurements we show that the surface of PdTe[Formula: see text] displays intrinsic electronic inhomogeneities in the normal state which leads to a mixed type I and type II superconducting behaviour along with a spatial distribution of critical fields in the superconducting state. Understanding of the origin of such inhomogeneities may be important for understanding the topological properties of PdTe[Formula: see text] in the normal state.

3.
J Phys Condens Matter ; 30(35): 355001, 2018 Sep 05.
Artigo em Inglês | MEDLINE | ID: mdl-30015627

RESUMO

The surface states of topological insulators (TI) are protected by time reversal symmetry and they display intrinsic spin helicity where the momentum of the charge carriers decides their spin states. As a consequence, a current injected through the surface states becomes spin polarized and this transport spin-polarization leads to a proportionate suppression of Andreev reflection in superconductor/TI junctions. Here we show that upon doping Bi2Se3 with Mn, the transport spin-polarization is seen to be monotonically suppressed. The parent compound Bi2Se3 is found to exhibit a transport spin-polarization of about 63% whereas crystals with 10% Mn doping show transport spin-polarization of about 48%. This suppression is accompanied by an increasing ferromagnetic order of the crystals with Mn doping. Scanning tunneling spectroscopy shows that the topological protection of the surface states reduces due to Mn doping. The net measured transport spin-polarization is due to a competition of this effect with the increased magnetization on Mn doping. The present results provide important insights for the choice of magnetic topological insulators for spintronic applications.

4.
J Phys Condens Matter ; 30(25): 255002, 2018 Jun 27.
Artigo em Inglês | MEDLINE | ID: mdl-29708502

RESUMO

For certain complex superconducting systems, the superconducting properties get enhanced under mesoscopic point contacts made of elemental non-superconducting metals. However, understanding of the mechanism through which such contact induced local enhancement of superconductivity happens has been limited due to the complex nature of such compounds. In this paper we present a large enhancement of superconducting transition temperature T c and superconducting energy gap Δ in a simple elemental superconductor Zr. While bulk Zr shows a critical temperature around 0.6 K, superconductivity survives at Ag/Zr and Pt/Zr point contacts up to 3 K with a corresponding five-fold enhancement of Δ. Further, the first-principles calculations on a model system provide useful insights. We show that the enhancement in superconducting properties can be attributed to a modification in the electron-phonon coupling accompanied by an enhancement of the density of states which involves the appearance of a new electron band at the Ag/Zr interfaces.

5.
Nat Commun ; 8: 13974, 2017 01 10.
Artigo em Inglês | MEDLINE | ID: mdl-28071685

RESUMO

A Weyl semimetal is a topologically non-trivial phase of matter that hosts mass-less Weyl fermions, the particles that remained elusive for more than 80 years since their theoretical discovery. The Weyl semimetals exhibit unique transport properties and remarkably high surface spin polarization. Here we show that a mesoscopic superconducting phase with critical temperature Tc=7 K can be realized by forming metallic point contacts with silver (Ag) on single crystals of TaAs, while neither Ag nor TaAs are superconductors. Andreev reflection spectroscopy of such point contacts reveals a superconducting gap of 1.2 meV that coexists with a high transport spin polarization of 60% indicating a highly spin-polarized supercurrent flowing through the point contacts on TaAs. Therefore, apart from the discovery of a novel mesoscopic superconducting phase, our results also show that the point contacts on Weyl semimetals are potentially important for applications in spintronics.

6.
J Phys Condens Matter ; 28(19): 195701, 2016 May 18.
Artigo em Inglês | MEDLINE | ID: mdl-27089948

RESUMO

From temperature and magnetic field dependent point-contact spectroscopy on the ferromagnetic superconductor Sr0.5Ce0.5FBiS2 (bulk superconducting [Formula: see text] K) we observe (a) a pseudogap in the normal state that sustains to a remarkably high temperature of 40 K and (b) two-fold enhancement of T c upto 5 K in the point-contact geometry. In addition, Andreev reflection spectroscopy reveals a superconducting gap of 6 meV for certain point-contacts suggesting that the mean field T c of this system could be approximately 40 K, the onset temperature of pseudo-gap. Our results suggest that quantum fluctuations originating from other competing orders in Sr0.5Ce0.5FBiS2 forbid a global phase coherence at high temperatures thereby suppressing T c. Apart from the known ordering to a ferromagnetic state, our first-principles calculations reveal nesting of a multi-band Fermi surface and a significant electron-phonon coupling that could result in charge density wave-like instabilities.

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