Production of orbital angular momentum states of optical vortex beams using a vortex half-wave retarder with double-pass configuration.

Higher orders of orbital angular momentum states (OAMs) of light have been produced with a double-pass configuration through a zero-order vortex half-wave retarder (VHWR). This double-pass technique can reduce the number of VHWR plates used, thus reducing costs. The OAM states of the vortex beams are identified by the near-field Talbot effect. Polarization dependence of the vortex states can also be demonstrated with this VHWR using Talbot effect. Without using the Talbot patterns, this effect of the polarization on the vortex beam can not be recognized. A theoretical validation has also been provided to complement the experimental results. Our study gives an improved understanding of this approach to use a VHWR plate.

High-precision grating period measurement.

We introduce a method for measuring a periodic structure, particularly a grating period. The method is based on the high-precision laser Talbot effect. The combination of a rubidium-locked external cavity diode laser and the Talbot interferometer provides an excellent and simple tool for this purpose. Some experimental results are provided to demonstrate the approach.

High-contrast optical vortex detection using the Talbot effect.

We apply the near-field Talbot effect to distinguish, characterize, and detect optical vortices. We perform experiments with single-, double-, multiple-slit, and grating diffraction. High-contrast image detection is achieved with the Talbot effect of a grating, even for higher than l=±1 orbital angular momentum states. Furthermore, we manipulate the vortex beam with different vortex states and use the Talbot effect for detecting. The experimental results are supported by theoretical simulations and demonstrate that the Talbot effect provides an excellent tool for optical vortex detection.

Realization of the single photon Talbot effect with a spatial light modulator.

We demonstrate the quantum Talbot effect using a beam of single photons produced by parametric down conversion. In contrast to the previous works, we use a programmable spatial light modulator to behave as a diffraction grating. Thus, the investigation of the Talbot diffraction patterns under the variation of grating structure can be easily performed. The influence of spectral bandwidth of the down-converted photons on the diffraction pattern is also investigated. A theoretical model based on the wave nature of photons is presented to explain the Talbot diffraction patterns under varying conditions. The measured diffraction patterns are in good agreement with the theoretical prediction. We are convinced that our study improves the understanding of the quantum Talbot effect.

Realization of optical carpets in the Talbot and Talbot-Lau configurations.

Talbot and Talbot-Lau effects are frequently used in lensless imaging applications with light, ultrasound, x-rays, atoms and molecules--generally in situations where refractive optical elements are non-existent or not suitable. We here show an experimental visualization of the intriguing wave patterns that are associated with near-field interferometry behind a single periodic diffraction grating under plane wave illumination and which are often referred to as Talbot carpets or quantum carpets. We also show the patterns behind two separated diffraction gratings under nearly-monochromatic but spatially incoherent illumination that illustrate the nature of Talbot-Lau carpets.

Wave and particle in molecular interference lithography.

The wave-particle duality of massive objects is a cornerstone of quantum physics and a key property of many modern tools such as electron microscopy, neutron diffraction or atom interferometry. Here we report on the first experimental demonstration of quantum interference lithography with complex molecules. Molecular matter-wave interference patterns are deposited onto a reconstructed Si(111) 7x7 surface and imaged using scanning tunneling microscopy. Thereby both the particle and the quantum wave character of the molecules can be visualized in one and the same image. This new approach to nanolithography therefore also represents a sensitive new detection scheme for quantum interference experiments.

Gas phase sorting of fullerenes, polypeptides and carbon nanotubes.

We discuss the Stark deflectometry of micro-modulated molecular beams for the enrichment of biomolecular isomers as well as single-wall carbon nanotubes, and we demonstrate the working principle of this idea with fullerenes. The sorting is based on the species-dependent susceptibility-to-mass ratio χ/m. The device is compatible with a high molecular throughput, and the spatial micro-modulation of the beam permits one to obtain a fine spatial resolution and a high sorting sensitivity.

Thermal and electrical properties of porphyrin derivatives and their relevance for molecule interferometry.

The authors present new measurements of thermal and electrical properties for two porphyrin derivatives. They determine their sublimation enthalpy from the temperature dependence of the effusive beam intensity. The authors study H2TPP and Fe(TPP)Cl in matter-wave interferometry. Both molecules have nearly equal de Broglie wavelengths but different internal characteristics: only Fe(TPP)Cl exhibits an electric dipole moment of about 2.7 D and the authors discuss its influence on the molecular interference pattern. The authors add an external electric force field to the interferometer and use it to measure the scalar polarizability. They compare their experimental values alpha(H2TPP)=105+/-4+/-6 A3 and alpha(Fe(TPP)Cl)=102+/-9+/-6 A3 to ab initio calculations and they discuss the influence of thermal excitations on the polarizability.