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1.
Phys Rev Lett ; 123(2): 025004, 2019 Jul 12.
Artigo em Inglês | MEDLINE | ID: mdl-31386509

RESUMO

We demonstrate that in partially ionized plasmas, Coulomb scattering can be significantly perturbed by electron collisions with neutral gas particles, and that this effect can be incorporated in the Coulomb collision terms of the Boltzmann equation by a modification of the classical Coulomb logarithm. We show that Boltzmann transport calculations using this modified Coulomb logarithm are in excellent agreement, for a sensitive model problem and a wide range of conditions, with particle simulations describing the many-body Coulomb interactions from first principles.

2.
Phys Rev E ; 99(1-1): 013203, 2019 Jan.
Artigo em Inglês | MEDLINE | ID: mdl-30780312

RESUMO

The self-diffusion phenomenon in a two-dimensional dusty plasma at extremely strong (effective) magnetic fields is studied experimentally and by means of molecular dynamics simulations. In the experiment the high magnetic field is introduced by rotating the particle cloud and observing the particle trajectories in a corotating frame, which allows reaching effective magnetic fields up to 3000 T. The experimental results confirm the predictions of the simulations: (i) superdiffusive behavior is found at intermediate timescales and (ii) the dependence of the self-diffusion coefficient on the magnetic field is well reproduced.

3.
Phys Rev E ; 95(1-1): 013209, 2017 Jan.
Artigo em Inglês | MEDLINE | ID: mdl-28208314

RESUMO

A magnetic field was recently shown to enhance field-parallel heat conduction in a strongly correlated plasma whereas cross-field conduction is reduced. Here we show that in such plasmas, the magnetic field has the additional effect of inhibiting the isotropization process between field-parallel and cross-field temperature components, thus leading to the emergence of strong and long-lived temperature anisotropies when the plasma is locally perturbed. An extended heat equation is shown to describe this process accurately.

4.
Phys Rev Lett ; 119(4): 045001, 2017 Jul 28.
Artigo em Inglês | MEDLINE | ID: mdl-29341739

RESUMO

Dynamic characteristics of strongly coupled classical one-component Coulomb and Yukawa plasmas are obtained within the nonperturbative model-free moment approach without any data input from simulations so that the dynamic structure factor (DSF) satisfies the first three nonvanishing sum rules automatically. The DSF, dispersion, decay, sound speed, and other characteristics of the collective modes are determined using exclusively the static structure factor calculated from various theoretical approaches including the hypernetted chain approximation. A good quantitative agreement with molecular dynamics simulation data is achieved.

5.
Phys Rev E ; 94(3-1): 033203, 2016 Sep.
Artigo em Inglês | MEDLINE | ID: mdl-27739697

RESUMO

In a two-dimensional (2D) dusty plasma composed of superparamagnetic, charged dust grains and immersed in an external magnetic field B, the grains interact via both Yukawa and magnetic dipole-dipole potentials. Because the grains' magnetic dipole moments are induced by B, the dipole moments all lie along B. When B is tilted with respect to the normal to the dust layer, the interaction between the grains becomes anisotropic. In our previous paper [Hartmann et al., Phys. Rev. E 89, 043102 (2014)PLEEE81539-375510.1103/PhysRevE.89.043102], we studied the character of waves in such a system, confined strictly to two dimensions, without any spatial extension in the direction perpendicular to the layer. We analyzed how the dispersion of waves depends on the direction of propagation and the relative strengths of the magnetic dipole and Yukawa potentials. In this paper, we consider a more realistic quasi-2D system where the grains are confined by an external potential and can undergo small oscillations perpendicular to the layer. We analyze the effect of the strength of the confining potential on the in-plane correlations and on the wave propagation. In addition to the in-plane compressional and transverse waves, there now appears an out-of-plane transverse wave generated by the oscillation of the grains in the confining potential. The theoretical approach uses the quasi-localized charge approximation paralleled by molecular dynamics simulations.

6.
Rev Sci Instrum ; 87(6): 063102, 2016 Jun.
Artigo em Inglês | MEDLINE | ID: mdl-27370421

RESUMO

A "scanning" drift tube apparatus, capable of mapping of the spatiotemporal evolution of electron swarms, developing between two plane electrodes under the effect of a homogeneous electric field, is presented. The electron swarms are initiated by photoelectron pulses and the temporal distributions of the electron flux are recorded while the electrode gap length (at a fixed electric field strength) is varied. Operation of the system is tested and verified with argon gas; the measured data are used for the evaluation of the electron bulk drift velocity. The experimental results for the space-time maps of the electron swarms - presented here for the first time - also allow clear observation of deviations from hydrodynamic transport. The swarm maps are also reproduced by particle simulations.

7.
Phys Rev E ; 93(6): 063209, 2016 Jun.
Artigo em Inglês | MEDLINE | ID: mdl-27415379

RESUMO

The influence of an external homogeneous magnetic field on the quasilocalization of the particles-characterized quantitatively by cage correlation functions-in strongly coupled three-dimensional Yukawa systems is investigated via molecular dynamics computer simulations over a wide domain of the system parameters (coupling and screening strengths, and magnetic field). The caging time is found to be enhanced by the magnetic field B. The anisotropic migration of the particles in the presence of magnetic field is quantified via computing directional correlation functions, which indicate a more significant increase of localization in the direction perpendicular to B, while a moderate increase is also found along the B field lines. Associating the particles' escapes from the cages with jumps of a characteristic length, a connection is found with the diffusion process: the diffusion coefficients derived from the decay time of the directional correlation functions in both the directions perpendicular to and parallel with B are in very good agreement with respective diffusion coefficients values obtained from their usual computation based on the mean-squared displacement of the particles.

8.
Artigo em Inglês | MEDLINE | ID: mdl-26764836

RESUMO

In a classical ideal plasma, a magnetic field is known to reduce the heat conductivity perpendicular to the field, whereas it does not alter the one along the field. Here we show that, in strongly correlated plasmas that are observed at high pressure and/or low temperature, a magnetic field reduces the perpendicular heat transport much less and even enhances the parallel transport. These surprising observations are explained by the competition of kinetic, potential, and collisional contributions to the heat conductivity. Our results are based on first-principle molecular dynamics simulations of a one-component plasma.

9.
Artigo em Inglês | MEDLINE | ID: mdl-24730953

RESUMO

We investigate the effect of an external magnetic field on the velocity autocorrelation function and the "caging" of the particles in a two-dimensional strongly coupled Yukawa liquid, via numerical simulations. The influence of the coupling strength on the position of the dominant peak in the frequency spectrum of the velocity autocorrelation function confirms the onset of a joint effect of the magnetic field and strong correlations at high coupling. Our molecular dynamics simulations quantify the decorrelation of the particles' surroundings: the magnetic field is found to increase significantly the caging time, which reaches values well beyond the time scale of plasma oscillations. The observation of the increased caging time is in accordance with findings that the magnetic field decreases diffusion in similar systems.

10.
Phys Rev E Stat Nonlin Soft Matter Phys ; 85(6 Pt 2): 066401, 2012 Jun.
Artigo em Inglês | MEDLINE | ID: mdl-23005223

RESUMO

Because liquids cannot resist shear except over very short distances comparable to the atomic spacing, shear sound waves (i.e., transverse phonons) propagate only for very short wavelengths. A measure of this limit is the cutoff wave number k(c), which is sometimes called the critical wave number. Previously k(c) was determined in molecular dynamics (MD) simulations by obtaining the dispersion relation. Another approach is developed in this paper by identifying the wave number at the onset of a negative peak in the transverse current correlation function. This method is demonstrated using a three-dimensional MD simulation of a Yukawa fluid, which mimics dusty plasmas. In general, k(c) is an indicator of conditions where elastic and dissipative effects are approximately balanced. Additionally, the crossover frequency for the real and imaginary terms of the complex viscosity of a dusty plasma is obtained; this crossover frequency corresponds to the Maxwell relaxation time.


Assuntos
Modelos Químicos , Reologia/métodos , Soluções/química , Simulação por Computador , Resistência ao Cisalhamento
11.
Phys Rev Lett ; 109(22): 225001, 2012 Nov 30.
Artigo em Inglês | MEDLINE | ID: mdl-23368129

RESUMO

The dynamics of the ion structure in warm dense matter is determined by molecular dynamics simulations using an effective ion-ion potential. This potential is obtained from ab initio simulations and has a strong short-range repulsion added to a screened Coulomb potential. Models based on static or dynamic local field corrections are found to be insufficient to describe the data. An extended Mermin approach, a hydrodynamic model, and the method of moments with local constraints are capable of reproducing the numerical results but have rather limited predictive powers as they all need some numerical data as input. The method of moments is found to be the most promising.

12.
Phys Rev E Stat Nonlin Soft Matter Phys ; 83(4 Pt 2): 046403, 2011 Apr.
Artigo em Inglês | MEDLINE | ID: mdl-21599312

RESUMO

The generation of higher harmonics of the magnetoplasmon frequency which has recently been reported in strongly coupled two-dimensional Yukawa systems is investigated in detail and, in addition, extended to two-dimensional Coulomb systems. We observe higher harmonics over a much larger frequency range than before and compare the theoretical prediction with the simulations. The influence of the coupling, structure, and thermal energy on the excitation of these modes is examined in detail. We also report on the effect of friction on the mode spectra to make predictions about the experimental observability of this new effect.

13.
J Chem Phys ; 134(6): 064308, 2011 Feb 14.
Artigo em Inglês | MEDLINE | ID: mdl-21322681

RESUMO

We investigate the Ar(+)-Fe asymmetric charge transfer (ACT) reaction using a combination of plasma diagnostics methods and a kinetic model of the afterglow plasma, which allow monitoring of the temporal evolution of the densities of different species. The iron vapor is created inside a discharge cell by cathode sputtering; its density is measured by atomic absorption spectroscopy. The rate coefficient of the reaction is evaluated from the emission intensity decay of Fe(+)∗ lines pumped by the ACT process in the He-Ar-Fe and Ar-Fe afterglow plasmas. The measurements yield a rate coefficient k = 7.6( ± 3.0) × 10(-9) cm(3) s(-1) at T = 300 K.


Assuntos
Argônio/química , Ferro/química , Hélio/química , Íons/química , Cinética , Espectrofotometria Atômica , Vácuo
14.
Phys Rev Lett ; 107(27): 275001, 2011 Dec 30.
Artigo em Inglês | MEDLINE | ID: mdl-22243313

RESUMO

Unlike α- and γ-mode operation, electrons accelerated by strong drift and ambipolar electric fields in the plasma bulk and at the sheath edges are found to dominate the ionization in strongly electronegative discharges. These fields are caused by a low bulk conductivity and local maxima of the electron density at the sheath edges, respectively. This drift-ambipolar mode is investigated by kinetic particle simulations, experimental phase-resolved optical emission spectroscopy, and an analytical model in CF(4). Mode transitions induced by voltage and pressure variations are studied.

15.
Phys Rev E Stat Nonlin Soft Matter Phys ; 81(5 Pt 2): 056404, 2010 May.
Artigo em Inglês | MEDLINE | ID: mdl-20866341

RESUMO

The viscoelastic properties of strongly coupled Yukawa liquids are characterized by computing the complex shear viscosity η(ω) . This is done using three methods of molecular-dynamics simulation: equilibrium, nonequilibrium, and Langevin dynamics, all with a mutually repulsive Yukawa interparticle potential. A change from viscous to elastic response is observed with increasing frequency, as well as a decrease of the magnitude of the viscosity with increasing frequency. The Langevin simulation reveals that the dependence of the complex viscosity on the friction has a different character for hot and cool liquids. At ω=0 , we find that as friction increases, the viscosity diminishes at high temperature but increases at low temperature. In addition to finding its frequency dependence, we also derive the wave-number (length-scale) dependence of the shear viscosity.

16.
Phys Rev Lett ; 105(5): 055002, 2010 Jul 30.
Artigo em Inglês | MEDLINE | ID: mdl-20867926

RESUMO

The existence of plasma oscillations at multiples of the magnetoplasmon frequency in a strongly coupled two-dimensional magnetized Yukawa plasma is reported, based on extensive molecular dynamics simulations. These modes are the analogues of Bernstein modes which are renormalized by strong interparticle correlations. Their properties are theoretically explained by a dielectric function incorporating the combined effect of a magnetic field, strong correlations and finite temperature.

17.
Phys Rev E Stat Nonlin Soft Matter Phys ; 79(2 Pt 2): 026401, 2009 Feb.
Artigo em Inglês | MEDLINE | ID: mdl-19391849

RESUMO

The existence of coefficients for diffusion, viscosity, and thermal conductivity is examined for two-dimensional (2D) liquids. Equilibrium molecular dynamics simulations are performed using a Yukawa potential and the long-time behavior of autocorrelation functions is tested. Advances reported here as compared to previous 2D Yukawa liquid simulations include an assessment of the thermal conductivity, using a larger system size to allow meaningful examination of longer times, and development of improved analysis methods. We find that the transport coefficient exists for diffusion at high temperature and viscosity at low temperature, but not in the opposite limits. The thermal conductivity coefficient does not appear to exist at high temperature. Further advances in computing power could improve these assessments by allowing even larger system sizes and longer time series.

18.
Phys Rev Lett ; 103(24): 245002, 2009 Dec 11.
Artigo em Inglês | MEDLINE | ID: mdl-20366204

RESUMO

A classical dusty plasma experiment was performed using two different dust grain sizes to form a strongly coupled asymmetric bilayer (two closely spaced interacting monolayers) of two species of charged dust particles. The observation and analysis of the thermally excited particle oscillations revealed the collective mode structure and dispersion (wave propagation) in this system; in particular, the existence of the theoretically predicted k=0 energy (frequency) gap was verified. Equilibrium molecular-dynamics simulations were performed to emulate the experiment, assuming Yukawa-type interparticle interaction. The simulations and analytic calculations based both on lattice summation and on the quasilocalized charge approximation approach are in good agreement with the experimental findings and help in identifying and characterizing the observed phenomena.

19.
Phys Rev E Stat Nonlin Soft Matter Phys ; 78(2 Pt 2): 026408, 2008 Aug.
Artigo em Inglês | MEDLINE | ID: mdl-18850947

RESUMO

We present molecular-dynamics calculations of the shear viscosity of three-dimensional strongly coupled Yukawa liquids which are frequently used as a model system of complex plasmas. The results obtained using two independent nonequilibrium simulation methods are critically compared with each other and with earlier published data for a wide range of plasma coupling (Gamma) and screening (kappa) parameters. The non-Newtonian behavior of the liquid, manifested as a decrease of the shear viscosity with increasing shear rate (shear thinning), and the validity of the Stokes-Einstein relation at high coupling strength are also demonstrated.

20.
Phys Rev E Stat Nonlin Soft Matter Phys ; 78(2 Pt 2): 026409, 2008 Aug.
Artigo em Inglês | MEDLINE | ID: mdl-18850948

RESUMO

The emergence and vanishing of superdiffusion in quasi-two-dimensional Yukawa systems are investigated by molecular dynamics simulations. Using both the asymptotic behavior of the mean-squared displacement of the particles and the long-time tail of the velocity autocorrelation function as indicators of superdiffusion, we confirm the existence of a transition from normal diffusion to superdiffusion in systems changing from a three-dimensional to a two-dimensional character. A connection between superdiffusion and dimensionality is established by the behavior of the projected pair distribution function.

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