Color-switching hydrogels as integrated microfluidic pressure sensors.

Precisely measuring pressure in microfluidic flows is essential for flow control, fluid characterization, and monitoring, but faces specific challenges such as achieving sufficient resolution, non-invasiveness, or ease of use. Here, we demonstrate a fully integrated multiplexed optofluidic pressure sensor, entirely decoupled from the flow path, that enables local pressure measurements along any microfluidic channel without altering its flow geometry. The sensor itself relies on the compression of a soft mechano-actuated hydrogel, changing color in response to a pressure change. The hydrogel is separated from the fluid circulating in the channel by a thin membrane, allowing for the unrestricted use of different types of fluids. Imaging the gel through the transparent PDMS with a color camera provides a direct, easy, and contact-free determination of the fluid pressure at the sensing location for pressures as small as 20mbar with a resolution of around 10mbar. The sensitivity and accessible pressure range can be tuned via the mechanical properties of the sensing unit. The photonic gel can also be used to acquire 2D pressure or deformation maps, taking advantage of the fast response time and fine spatial resolution.

A mechanism of strain hardening and Bauschinger effect: shear-history-dependent microstructure of elasto-plastic suspensions.

Dispersing solid hard particles in an elasto-plastic material leads to important shear-history dependence of the behavior, namely strain hardening and Bauschinger effect. Strain hardening is observed as the progressive strengthening of a material during its plastic deformation and is usually associated with ductility, a property often sought after in composite materials to postpone fractures and failure. In addition, anisotropic mechanical properties are developed, the material resistance being larger in the direction of the imposed flow, which is referred to as the Bauschinger effect. We show that this is related here to shear-history-dependent particle-pair distribution functions. Roughness and interparticle contacts likely play a major role, as replacing hard particles by non-deformable bubbles modifies the suspension microstructure and suppresses strain hardening. Beyond suspensions, our study provides new insight in the understanding and control of strain hardening and Bauschinger effect in composite materials.

Coupling of elasticity to capillarity in soft aerated materials.

We study the elastic properties of soft solids containing air bubbles. Contrary to standard porous materials, the softness of the matrix allows for a coupling of the matrix elasticity to surface tension forces acting on the bubble surface. Thanks to appropriate experiments on model systems, we demonstrate how the elastic response of the soft porous solid is governed by two dimensionless parameters: the gas volume fraction and a capillary number comparing the elasticity of the matrix with the stiffness of the bubbles. Furthermore, we show that our experimental results are accurately predicted by computations of the shear modulus through a micro-mechanical approach.