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1.
J Phys Chem Lett ; 14(36): 8060-8068, 2023 Sep 14.
Artigo em Inglês | MEDLINE | ID: mdl-37655950

RESUMO

Despite decades of intensive experimental and theoretical efforts, the physics of cuprate high-temperature superconductors in general, and, in particular, their normal state, is still under debate. Here, we report our investigation of low-energy charge excitations in the normal state. We find that the peculiarities of the electronic band structure at low energies have a profound impact on the nature of the intraband collective modes. It gives rise to a new kind of mode with huge intensity and non-Lorentzian spectral function in addition to well-known collective excitations like conventional plasmons and spin fluctuation. We predict two such modes with maximal spectral weight in the nodal and antinodal directions. Additionally, we found a long-living quasi-one-dimensional plasmon becoming an intense soft mode over an extended momentum range along the antinodal direction. These modes might explain some of the resonant inelastic X-ray scattering spectroscopy data.

2.
Phys Rev Lett ; 123(20): 207202, 2019 Nov 15.
Artigo em Inglês | MEDLINE | ID: mdl-31809068

RESUMO

A wide variety of complex phases in quantum materials are driven by electron-electron interactions, which are enhanced through density of states peaks. A well-known example occurs at van Hove singularities where the Fermi surface undergoes a topological transition. Here we show that higher order singularities, where multiple disconnected leaves of Fermi surface touch all at once, naturally occur at points of high symmetry in the Brillouin zone. Such multicritical singularities can lead to stronger divergences in the density of states than canonical van Hove singularities, and critically boost the formation of complex quantum phases via interactions. As a concrete example of the power of these Fermi surface topological transitions, we demonstrate how they can be used in the analysis of experimental data on Sr_{3}Ru_{2}O_{7}. Understanding the related mechanisms opens up new avenues in material design of complex quantum phases.

3.
Phys Rev Lett ; 113(17): 177001, 2014 Oct 24.
Artigo em Inglês | MEDLINE | ID: mdl-25379930

RESUMO

Bulk TiSe2 is an intrinsically layered transition metal dichalcogenide hosting both superconducting and charge-density-wave ordering. Motivated by the recent progress in preparing two-dimensional transition metal dichalcogenides, we study these frustrated orderings in a single trilayer of TiSe2. Using a renormalization group approach, we find that electronic correlations can give rise to charge-density-wave order and two kinds of superconductivity. One possible superconducting state corresponds to unconventional s(+-) pairing. The other is particularly exciting as it is chiral, breaking time-reversal symmetry. Its stability depends on the precise strength and screening of the electron-electron interactions in two-dimensional TiSe2.

4.
Phys Rev Lett ; 112(3): 037202, 2014 Jan 24.
Artigo em Inglês | MEDLINE | ID: mdl-24484163

RESUMO

We discuss the form of the damping of magnetic excitations in a metal near a ferromagnetic instability. The paramagnon theory predicts that the damping term should have the form γ(q,Ω)∝Ω/Γ(q), with Γ(q)∝q (the Landau damping). However, the experiments on uranium metallic compounds UGe2 and UCoGe showed that Γ(q) is essentially independent of q. A nonzero γ(q=0,Ω) is impossible in systems with one type of carrier (either localized or itinerant) because it would violate the spin conservation. It has been conjectured recently that a near-constant Γ(q) in UGe2 and UCoGe may be due to the presence of both localized and itinerant electrons in these materials, with ferromagnetism involving predominantly localized spins. We present the microscopic analysis of the damping of near-critical localized excitations due to interaction with itinerant carriers. We show explicitly how the presence of two types of electrons breaks the cancellation between the contributions to Γ(0) from the self-energy and vertex correction insertions into the spin polarization bubble. We compare our theory with the available experimental data.

5.
Nat Mater ; 3(12): 853-6, 2004 Dec.
Artigo em Inglês | MEDLINE | ID: mdl-15558036

RESUMO

Transition metal oxides with a perovskite-type structure constitute a large group of compounds with interesting properties. Among them are materials such as the prototypical ferroelectric system BaTiO(3), colossal magnetoresistance manganites and the high-T(c) superconductors. Hundreds of these compounds are magnetic, and hundreds of others are ferroelectric, but these properties very seldom coexist. Compounds with an interdependence of magnetism and ferroelectricity could be very useful: they would open up a plethora of new applications, such as switching of magnetic memory elements by electric fields. Here, we report on a possible way to avoid this incompatibility, and show that in charge-ordered and orbitally ordered perovskites it is possible to make use of the coupling between magnetic and charge ordering to obtain ferroelectric magnets. In particular, in manganites that are less than half doped there is a type of charge ordering that is intermediate between site-centred and bond-centred. Such a state breaks inversion symmetry and is predicted to be magnetic and ferroelectric.


Assuntos
Cristalização/métodos , Eletroquímica , Magnetismo/instrumentação , Compostos de Manganês/química , Manufaturas , Modelos Químicos , Modelos Moleculares , Simulação por Computador , Eletricidade , Eletrônica , Armazenamento e Recuperação da Informação , Conformação Molecular
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