Transverse Doppler effect due to Gaussian beams.

We report on the observation of a transverse Doppler shift in the optical domain. It occurs when a receiving system travels perpendicularly to the propagation direction of a Gaussian beam. Shifts of a few tens of Hz have been evidence for a detector moving in the mm/s range. The shift increases as the detector is far from the beam axis. The observations fully agree with theoretical calculations on the propagation of Gaussian beams. It can be observed for any kind of waves, including radio and acoustic waves. Practical consequences are then discussed, especially for techniques using Doppler measurements in microsystems.

Rotational Doppler shift from a rotating rod.

This Letter reports on a rotational Doppler effect obtained from a rotating rod illuminated by a fundamental Gaussian laser beam. More specifically, we decompose the transmitted light behind the rotating rod into Laguerre-Gaussian modes and investigate the associated frequency shifts. The main contributing modes correspond to modes having the same rotational symmetry as the rotating object. Furthermore, their shifts equal the topological charge of the beam times the rotational frequency of the object. Potential applications in pattern recognition and rotation identification are then considered.

Resonant vibration of a thin polymer film under optical excitation.

We report on the mechanical excitation of a 220 µm thick thermoplastic film in its amorphous state by the radiation pressure of light. By modulating a low power visible laser (from 100 to 600 mW) at low frequencies (below 100 Hz), we observe a deformation of the film interfaces. The phenomenon, that is independent of the laser wavelength, is amplified at a resonant frequency and reaches 0.68 µm. The deformation is reversible and varies linearly with the optical power. Using the damped oscillator model, we show that the resonant frequency depends on the surface tension of the film. The associated free energy is then compared with the energy lost, taking into account the contribution of the damping corresponding to the imaginary part of the Young's modulus.

Nanometer optical trap based on stimulated emission in evanescence of a totally reflected Arago spot : Nanometer optical trap for fluorescent nanoparticles.

Optical tweezers have paved the way towards the manipulation of particles and living cells at the micrometer range. Its extension towards the nanometer world may create unprecedented potentialities in many areas of science. Following a letter (O. Emile, J. Emile, H. Tabuteau, EPL 129, 58001 (2020)) that reported the observation of the trapping of a single 200nm diameter fluorescent particle in a nanometric volume, we detail here our experimental findings. In particular, the trapping mechanism is shown to be based on the radiation pressure of light in one direction and on the stimulated emission of the particle in the evanescent wave of a nanometer Arago spot on a glass/liquid interface on the other directions. The trapping volume is a 200nm height cylinder whose radius varies with the spreading of the evanescent wave near the spot and can reach 50nm. The calculation of the force and the parameters limiting the lifetime are detailed. Applications to laser trapping of atoms and molecules are also discussed.

Experimental analysis of submicrometer optical intensity distributions after an opaque disk.

Generation of subwavelength beam sizes is a fascinating challenge with several implications. The observation of a 120 nm laser spot in the visible part of the spectrum is reported here. It has a size variation of less than 10% in a distance of $ 50\;\unicode{x00B5}{\rm m} $50µm along the axis of propagation. This so-called Arago spot results from the diffraction of the light from a laser diode by the edges of an absorbing disk. Applications are discussed and hollow beams carrying orbital angular momentum with a 400 nm diameter dark spot in the center are evidenced. This paves the way toward atom lithography via atom guiding or new spectroscopy on forbidden transitions.

Rotation of a floating hydrophobic disk: influence of line tension.

The rotation of a sub-millimeter size disk over a water bath is reported. The origin of the rotation arises from the transfer of angular momentum from a plane wave diffracted by an asymmetrical picture printed on the disk. Because of its hydrophobic character, the viscous friction contribution to the rotational motion of the object floating on the air/liquid interface is weak. From the driving optical torque and the steady-state rotation, we measure the contribution of the line tension in the femto-Newton range.

Naked eye picometer resolution in a Michelson interferometer using conjugated twisted beams.

Michelson interferometry is one of the most widely used techniques for accuracy measurements. Its main characteristic feature is to infer a displacement in one of the arms of the interferometer from a phase measurement. Two different twisted beams, also called vortex beams, with opposite twisted rotations in each arm of the interferometer interfere in a daisy flower-like pattern. The number of petals is twice the topological charge. Their position depends on the relative phase of the beams. Naked eye detection of 44 pm displacements is achieved. The sensitivity of such an interferometer together with possible further improvements, and applications are then discussed.

Influence of the interface on the optical activity of confined glucose films.

We report on the time evolution of the optical activity of a thinning liquid film containing glucose, and confined between two glass slides. This dynamics strongly depends on the presence of surfactant molecules. With sodium dodecyl sulfate (SDS), we evidence favorable interactions of sugar molecules with the sulfate group. As previously observed for a freely suspended soap film in the air (see Emile et al., 2013), this corresponds to an anchoring of glucose molecules at the interface. For glucose alone, we also highlight a molecular rearrangement that is not instantaneous and occurs after several minutes. This interfacial organization leads to an unusual giant optical activity that is different with or without SDS. Molecular simulations confirm the anchoring of the glucose molecules at the glass/liquid interface, and show a different molecular orientation in each case.

Rotation of millimeter-sized objects using ordinary light.

The ability to optically rotate bodies offers new degrees of control of micro-objects with applications in various domains, including microelectromechanical systems (MEMS), biomanipulations, or optofluidics. Here we demonstrate the optically-induced rotation of simple asymmetric two-dimensional objects using plane waves originating either from ordinary laser sources or from black body radiation. The objects are floating on an air/water interface. We observe a steady-state rotation depending on the light intensity and on the asymmetry of the object. We interpret this rotation in terms of light diffraction by the edges of the object. Such systems could be easily implemented in optofluidic devices to induce liquid flow without the need for special light sources.

Laser-induced vibration of a thin soap film.

We report on the vibration of a thin soap film based on the optical radiation pressure force. The modulated low power laser induces a counter gravity flow in a vertical free-standing draining film. The thickness of the soap film is then higher in the upper region than in the lower region of the film. Moreover, the lifetime of the film is dramatically increased by a factor of 2. Since the laser beam only acts mechanically on the film interfaces, such a film can be employed in an optofluidic diaphragm pump, the interfaces behaving like a vibrating membrane and the liquid in-between being the fluid to be pumped. Such a pump could then be used in delicate micro-equipment, in chips where temperature variations are detrimental and even in biological systems.

Electromagnetically induced torque on a large ring in the microwave range.

We report on the exchange of orbital angular momentum between an electromagnetic wave and a 30 cm diameter ring. Using a turnstile antenna in the GHz range, we induce a torque on a suspended copper strip of the order of 10(-8) N m. Rotations of a few degrees and accelerations up to 4×10(-4) °/s2 are observed. A linear dependence of the acceleration as a function of the applied power is found. There are many applications in the detection of angular momentum in electromagnetics, in acoustics, and also in the magnetization of nanostructures.

Giant optical activity of sugar in thin soap films.

We report on enhanced experimental optical activity measurements of thin soap films in the presence of sugar. This unusual optical activity is linked to the intramolecular chiral conformation of the glucose molecules at the air/liquid interface. Choosing sodium dodecylsulfate (SDS) as a model surfactant and glucose as model sugar, favorable interactions between the anionic group -OSO3(-)- and the glucose molecules are highlighted. This induces an interfacial anchoring of glucose molecules leading to a perturbing influence of the asymmetric chiral environment.

Recent advances in Many Body Dissipative Particles Dynamics simulations of liquid-vapor interfaces.

Many Body Dissipative Particles Dynamics (MDPD) simulation is a novel promising mesoscopic method to model the liquid-vapor interfaces. Based upon works of Paganobarraga and Frenkel (J. Chem. Phys. 15, 5015 (2001)) and Trofimov (J. Chem. Phys. 117, 9383 (2002)) and of Warren (Phys. Rev. E 68, 066702 (2003)) this method has been critically reviewed during this last decade. We propose here to give an overview of the Many Body Dissipative Particles Dynamic simulation within the framework of the liquid-vapor interfaces. We recall the theoretical background of MDPD and we present some recent results of systems of interest such as water liquid-vapor interfaces and salt effect on water surface tension. Additionally we discuss the ability of MDPD to capture the mechanisms at the mesoscopic scale through the formation of micelles and the coalescence of a nanodroplet water on water surface.

Foam films in the presence of functionalized gold nanoparticles.

Dry aqueous foams made of anionic surfactant (SDS) and spherical gold nanoparticles are studied by small angle X-ray scattering and by optical techniques. To obtain stable foams, the surfactant concentration is well above the critical micelle concentration. The specular reflectivity signal obtained on a very thin film (thickness 20 nm) shows that functionalized nanoparticles (17 nm typical size) are trapped within the film in the form of a single monolayer. In order to isolate the film behavior, investigations are made on a single film confined in a tube. The film thinning according to the ratio of functionalized nanoparticle and SDS micelles (1:1, 1:10, 1:100) is mainly governed by the structural arrangement of SDS micelles. In thick films, nanoparticles tend to form aggregates that disappear during drainage. In particular self-organization of nanoparticles (with different surface charge) inside the film is not detected.

Low-power laser deformation of an air-liquid interface.

We report on the deformation of an air-water surface with a totally reflected low-power laser beam, inducing a convex mirror effect on the beam propagation. This bending is stronger close to the critical angle and depends on the polarization of the laser light. A model, leading to a simple dependence between the Goos-Hänchen shift and the radius of curvature of the interface, supports these observations. Bendings with radius of curvature as low as 0.10 m are demonstrated.

A systematic and quantitative study of the link between foam slipping and interfacial viscoelasticity.

Aqueous foams are often used under various flow regimes, and one of the biggest challenges is to create predictive models of their complex rheological properties. Previous theoretical and experimental studies have qualitatively characterized the wall slip of foams. We focus on this phenomenon in a 1D geometry, studying the friction force to move a train of foam films in a narrow channel. We perform, and correlate, 1D experiments and interfacial measurements of surface elasticity. We adapt existing models to correctly analyze and interpret 1D data, allowing for comparison with 3D foam slip results. Different mixtures of surfactants allow us to quantify the influence of interfacial properties. In particular, we show for 1D experiments that already with a low elasticity, of order 1 mN m(-1), we leave the regime where the interface can be considered as fluid, to enter a regime where dissipation depends only marginally on surface elasticity.

Structure of liquid films of an ordered foam confined in a narrow channel.

A bamboo foam is the simplest case of an ordered foam confined in a narrow channel. It is made of a regular film distribution, arranged perpendicularly to the channel. Our work consists of studying the structural properties of several films taken in a drained foam. X-ray experiments highlighted the equality of the equilibrium thickness for each film within a foam. The same thickness was found as by measurements of disjoining pressure isotherms, proving as well that films of a bamboo foam behave like isolated ones. The refinement of X-ray data by a simple model of specular reflectivity showed a significant variation of the electronic distribution of the surfactant layer for a common black film forwarding from one equilibrium state to another. A discussion on the organization of the surfactant molecules to the gas/liquid interface and film is proposed.