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1.
Nature ; 626(7998): 294-299, 2024 Feb.
Artigo em Inglês | MEDLINE | ID: mdl-38326595

RESUMO

An essential ingredient for the production of Majorana fermions for use in quantum computing is topological superconductivity1,2. As bulk topological superconductors remain elusive, the most promising approaches exploit proximity-induced superconductivity3, making systems fragile and difficult to realize4-7. Due to their intrinsic topology8, Weyl semimetals are also potential candidates1,2, but have always been connected with bulk superconductivity, leaving the possibility of intrinsic superconductivity of their topological surface states, the Fermi arcs, practically without attention, even from the theory side. Here, by means of angle-resolved photoemission spectroscopy and ab initio calculations, we identify topological Fermi arcs on two opposing surfaces of the non-centrosymmetric Weyl material trigonal PtBi2 (ref. 9). We show these states become superconducting at temperatures around 10 K. Remarkably, the corresponding coherence peaks appear as the strongest and sharpest excitations ever detected by photoemission from solids. Our findings indicate that superconductivity in PtBi2 can occur exclusively at the surface, rendering it a possible platform to host Majorana modes in intrinsically topological superconductor-normal metal-superconductor Josephson junctions.

2.
Adv Sci (Weinh) ; 10(10): e2203239, 2023 Apr.
Artigo em Inglês | MEDLINE | ID: mdl-36802132

RESUMO

The recent realizations of the quantum anomalous Hall effect (QAHE) in MnBi2 Te4 and MnBi4 Te7 benchmark the (MnBi2 Te4 )(Bi2 Te3 )n family as a promising hotbed for further QAHE improvements. The family owes its potential to its ferromagnetically (FM) ordered MnBi2 Te4 septuple layers (SLs). However, the QAHE realization is complicated in MnBi2 Te4 and MnBi4 Te7 due to the substantial antiferromagnetic (AFM) coupling between the SLs. An FM state, advantageous for the QAHE, can be stabilized by interlacing the SLs with an increasing number n of Bi2 Te3 quintuple layers (QLs). However, the mechanisms driving the FM state and the number of necessary QLs are not understood, and the surface magnetism remains obscure. Here, robust FM properties in MnBi6 Te10 (n = 2) with Tc ≈ 12 K are demonstrated and their origin is established in the Mn/Bi intermixing phenomenon by a combined experimental and theoretical study. The measurements reveal a magnetically intact surface with a large magnetic moment, and with FM properties similar to the bulk. This investigation thus consolidates the MnBi6 Te10 system as perspective for the QAHE at elevated temperatures.

3.
Nano Lett ; 23(4): 1229-1235, 2023 Feb 22.
Artigo em Inglês | MEDLINE | ID: mdl-36720048

RESUMO

Symmetry breaking in topological matter has become in recent years a key concept in condensed matter physics to unveil novel electronic states. In this work, we predict that broken inversion symmetry and strong spin-orbit coupling in trigonal PtBi2 lead to a type-I Weyl semimetal band structure. Transport measurements show an unusually robust low dimensional superconductivity in thin exfoliated flakes up to 126 nm in thickness (with Tc ∼ 275-400 mK), which constitutes the first report and study of unambiguous superconductivity in a type-I Weyl semimetal. Remarkably, a Berezinskii-Kosterlitz-Thouless transition with TBKT ∼ 310 mK is revealed in up to 60 nm thick flakes, which is nearly an order of magnitude thicker than the rare examples of two-dimensional superconductors exhibiting such a transition. This makes PtBi2 an ideal platform to study low dimensional and unconventional superconductivity in topological semimetals.

4.
Phys Rev Lett ; 127(5): 056601, 2021 Jul 30.
Artigo em Inglês | MEDLINE | ID: mdl-34397225

RESUMO

We show that Weyl Fermi arcs are generically accompanied by a divergence of the surface Berry curvature scaling as 1/k^{2}, where k is the distance to a hot line in the surface Brillouin zone that connects the projection of Weyl nodes with opposite chirality, but which is distinct from the Fermi arc itself. Such surface Berry curvature appears whenever the bulk Weyl dispersion has a velocity tilt toward the surface of interest. This divergence is reflected in a variety of Berry curvature mediated effects that are readily accessible experimentally and, in particular, leads to a surface Berry curvature dipole that grows linearly with the thickness of a slab of a Weyl semimetal material in the limit of the long lifetime of surface states. This implies the emergence of a gigantic contribution to the nonlinear Hall effect in such devices.

5.
Nat Mater ; 19(2): 163-169, 2020 Feb.
Artigo em Inglês | MEDLINE | ID: mdl-31819211

RESUMO

A kagome lattice of 3d transition metal ions is a versatile platform for correlated topological phases hosting symmetry-protected electronic excitations and magnetic ground states. However, the paradigmatic states of the idealized two-dimensional kagome lattice-Dirac fermions and flat bands-have not been simultaneously observed. Here, we use angle-resolved photoemission spectroscopy and de Haas-van Alphen quantum oscillations to reveal coexisting surface and bulk Dirac fermions as well as flat bands in the antiferromagnetic kagome metal FeSn, which has spatially decoupled kagome planes. Our band structure calculations and matrix element simulations demonstrate that the bulk Dirac bands arise from in-plane localized Fe-3d orbitals, and evidence that the coexisting Dirac surface state realizes a rare example of fully spin-polarized two-dimensional Dirac fermions due to spin-layer locking in FeSn. The prospect to harness these prototypical excitations in a kagome lattice is a frontier of great promise at the confluence of topology, magnetism and strongly correlated physics.

6.
Nano Lett ; 20(1): 300-305, 2020 Jan 08.
Artigo em Inglês | MEDLINE | ID: mdl-31774686

RESUMO

Weyl semimetals exhibit interesting electronic properties due to their topological band structure. In particular, large anomalous Hall and anomalous Nernst signals are often reported, which allow for a detailed and quantitative study of subtle features. We pattern single crystals of the magnetic Weyl semimetal Co3Sn2S2 into nanoribbon devices using focused ion beam cutting and optical lithography. This approach enables a very precise study of the galvano- and thermomagnetic transport properties. Indeed, we found interesting features in the temperature dependency of the anomalous Hall and Nernst effects. We present an analysis of the data based on the Mott relation and identify in the Nernst response signatures of magnetic fluctuations enhancing the anomalous Nernst conductivity at the magnetic phase transition.

7.
J Phys Condens Matter ; 31(24): 245602, 2019 Jun 19.
Artigo em Inglês | MEDLINE | ID: mdl-30844779

RESUMO

We analyze the electronic properties of interacting crystal field split three band systems. Using a rotationally invariant slave boson approach we analyze the behavior of the electronic mass renormalization as a function of the intralevel repulsion U, the Hund's coupling J, the crystal field splitting, and the number of electrons per site n. We first focus on the case in which two of the bands are identical and the levels of the third one are shifted by [Formula: see text] with respect to the former. We find an increasing quasiparticle mass differentiation between the bands, for system away from half-filling (n = 3), as the Hubbard interaction U is increased. This leads to orbital selective Mott transitions where either the higher energy band (for 4 > n > 3) or the lower energy degenerate bands (2 < n < 3) become insulating for U larger than a critical interaction [Formula: see text]. Away from the half-filled case [Formula: see text] there is a wide range of parameters for [Formula: see text] where the system presents a Hund's metal phase with the physics dominated by the local high spin multiplets. Finally, we study the fate of the n = 2 Hund's metal as the energy splitting between orbitals is increased for different possible crystal distortions. We find a strong sensitivity of the Hund's metal regime to crystal fields due to the opposing effects of J and the crystal field splittings on the charge distribution between the bands.

8.
Phys Rev Lett ; 121(24): 246403, 2018 Dec 14.
Artigo em Inglês | MEDLINE | ID: mdl-30608737

RESUMO

Transitions between topologically distinct electronic states have been predicted in different classes of materials and observed in some. A major goal is the identification of measurable properties that directly expose the topological nature of such transitions. Here, we focus on the giant Rashba material bismuth tellurium iodine which exhibits a pressure-driven phase transition between topological and trivial insulators in three dimensions. We demonstrate that this transition, which proceeds through an intermediate Weyl semimetallic state, is accompanied by a giant enhancement of the Berry curvature dipole which can be probed in transport and optoelectronic experiments. From first-principles calculations, we show that the Berry dipole-a vector along the polar axis of this material-has opposite orientations in the trivial and topological insulating phases and peaks at the insulator-to-Weyl critical points, at which the nonlinear Hall conductivity can increase by over 2 orders of magnitude.

9.
J Phys Condens Matter ; 25(24): 245701, 2013 Jun 19.
Artigo em Inglês | MEDLINE | ID: mdl-23719090

RESUMO

We report magnetoresistance measurements in Nb films having a periodic thickness modulation. The cylinder shaped thicker regions of the sample, which form a square lattice, act as repulsive centers for the superconducting vortices. For low driving currents along one of the axes of the square lattice, the resistivity ρ increases monotonously with increasing magnetic field B and the ρ-B characteristics are approximately piecewise linear. The linear ρ versus B segments change their slope at matching fields where the number of vortices is an integer or a half integer times the number of protruding cylinders in the sample. Numerical simulations allow us to associate the different segments of linear magnetoresistance to different vortex-flow regimes, some of which are dominated by the propagation of discommensurations (kinks).

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