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1.
Phys Rev Lett ; 122(4): 040501, 2019 Feb 01.
Artigo em Inglês | MEDLINE | ID: mdl-30768296

RESUMO

We use a novel unitary map toolbox-discrete-time quantum walks originally designed for quantum computing-to implement ultrafast computer simulations of extremely slow dynamics in a nonlinear and disordered medium. Previous reports on wave packet spreading in Gross-Pitaevskii lattices observed subdiffusion with the second moment m_{2}∼t^{1/3} (with time in units of a characteristic scale t_{0}) up to the largest computed times of the order of 10^{8}. A fundamental and controversially debated question-whether this process can continue ad infinitum, or has to slow down-stands unresolved. Current experimental devices are not capable to even reach 1/10^{4} of the reported computational horizons. With our toolbox, we outperform previous computational results and observe that the universal subdiffusion persists over an additional four decades reaching "astronomic" times 2×10^{12}. Such a dramatic extension of previous computational horizons suggests that subdiffusion is universal, and that the toolbox can be efficiently used to assess other hard computational many-body problems.

2.
ACS Nano ; 5(5): 3896-904, 2011 May 24.
Artigo em Inglês | MEDLINE | ID: mdl-21491948

RESUMO

Graphene-based materials have been suggested for applications ranging from nanoelectronics to nanobiotechnology. However, the realization of graphene-based technologies will require large quantities of free-standing two-dimensional (2D) carbon materials with tunable physical and chemical properties. Bottom-up approaches via molecular self-assembly have great potential to fulfill this demand. Here, we report on the fabrication and characterization of graphene made by electron-radiation induced cross-linking of aromatic self-assembled monolayers (SAMs) and their subsequent annealing. In this process, the SAM is converted into a nanocrystalline graphene sheet with well-defined thickness and arbitrary dimensions. Electric transport data demonstrate that this transformation is accompanied by an insulator to metal transition that can be utilized to control electrical properties such as conductivity, electron mobility, and ambipolar electric field effect of the fabricated graphene sheets. The suggested route opens broad prospects toward the engineering of free-standing 2D carbon materials with tunable properties on various solid substrates and on holey substrates as suspended membranes.


Assuntos
Grafite/química , Nanoestruturas/química , Nanoestruturas/ultraestrutura , Transporte de Elétrons , Substâncias Macromoleculares/química , Teste de Materiais , Conformação Molecular , Tamanho da Partícula , Propriedades de Superfície
3.
Nature ; 452(7187): 613-5, 2008 Apr 03.
Artigo em Inglês | MEDLINE | ID: mdl-18385735

RESUMO

Synchronized oscillators are ubiquitous in nature, and synchronization plays a key part in various classical and quantum phenomena. Several experiments have shown that in thin superconducting films, disorder enforces the droplet-like electronic texture--superconducting islands immersed into a normal matrix--and that tuning disorder drives the system from superconducting to insulating behaviour. In the vicinity of the transition, a distinct state forms: a Cooper-pair insulator, with thermally activated conductivity. It results from synchronization of the phase of the superconducting order parameter at the islands across the whole system. Here we show that at a certain finite temperature, a Cooper--air insulator undergoes a transition to a superinsulating state with infinite resistance. We present experimental evidence of this transition in titanium nitride films and show that the superinsulating state is dual to the superconducting state: it is destroyed by a sufficiently strong critical magnetic field, and breaks down at some critical voltage that is analogous to the critical current in superconductors.

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