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RSC Adv ; 11(39): 24137-24143, 2021 Jul 06.
Artigo em Inglês | MEDLINE | ID: mdl-35479049

RESUMO

Hybrid organic-inorganic lead halide perovskite nanoparticles are promising candidates for optoelectronic applications. This investigation describes the structural and optical properties of MA x Cs1-x PbBr3 mixed cation colloidal nanoparticles spanning the complete compositional range of Cs substitution. A monotonic progression in the cubic lattice parameter (a) with changes in the Cs+ content confirmed the formation of mixed cation materials. More importantly, time-resolved photoluminescence (TRPL) revealed the optimized 13 mol% Cs nanoparticle composition exhibits the longest charge carrier lifetime and enhancement in radiative pathways. This sample also showed the highest photoluminescence quantum yield (PLQY) of ∼88% and displays ∼100% improvement in the PLQY of pure MAPbBr3 and CsPbBr3. Prototype LEDs fabricated from MA0.87Cs0.13PbBr3 were demonstrated.

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