Optomagnetism with a plasmonic skyrmion.

Research at the frontier between optics and magnetism is revealing a wealth of innovative phenomena and avenues of exploration. Optical waves are demonstrating the capacity to induce ultrafast magnetism, while optical analogs of magnetic states, such as magnetic skyrmions, offer the prospect of novel, to the best of our knowledge, spin-optical states. In this Letter, we strengthen the synergy between light and magnetism by exploring the ability of plasmonic Neel skyrmions to create an optomagnetic field, i.e., an opto-induced stationary magnetic field, within a thin gold film. We show that, when generated using a focused radially polarized vortex beam (RPVB), a plasmonic Neel skyrmion emerges as an optimum for inducing optomagnetism in a thin gold film. Optical skyrmions offer new degrees of freedom for enhancing and controlling optomagnetism in plasmonic nanostructures, with direct application in all-optical magnetization switching, magnetic recording, and the excitation of spin waves.

Optical Spin Waves.

Chirality is inherent to a broad range of systems, including solid-state and wave physics. The precession (chiral motion) of the magnetic moments in magnetic materials, forming spin waves, has various properties and many applications in magnetism and spintronics. We show that an optical analogue of spin waves can be generated in arrays of plasmonic nanohelices. Such optical waves arise from the interaction between twisted helix eigenmodes carrying spin and orbital angular momenta. We demonstrate that these optical spin waves are reflected at the interface between successive domains of enantiomeric nanohelices, forming a heterochiral lattice regardless of the wave propagation direction within the lattice. Optical spin waves may be applied in techniques involving photon spin, ranging from data processing and storage to quantum optics.

Six-probe scintillator dosimeter for treatment verification in HDR-brachytherapy.

BACKGROUND: In vivo dosimetry (IVD) is gaining interest for treatment delivery verification in HDR-brachytherapy. Time resolved methods, including source tracking, have the ability both to detect treatment errors in real time and to minimize experimental uncertainties. Multiprobe IVD architectures holds promise for simultaneous dose determinations at the targeted tumor and surrounding healthy tissues while enhancing measurement accuracy. However, most of the multiprobe dosimeters developed so far either suffer from compactness issues or rely on complex data post-treatment. PURPOSE: We introduce a novel concept of a compact multiprobe scintillator detector and demonstrate its applicability in HDR-brachytherapy. Our fabricated seven-fiber probing system is sufficiently narrow to be inserted in a brachytherapy needle or in a catheter. METHODS: Our multiprobe detection system results from the parallel implementation of six miniaturized inorganic Gd2 O2 S:Tb scintillator detectors at the end of a bundle of seven fibers, one fiber is kept bare to assess the stem effect. The resulting system, which is narrower than 320 microns, is tested with a MicroSelectron 9.14 Ci Ir-192 HDR afterloader, in a water phantom. The detection signals from all six probes are simultaneously read with a sCMOS camera (at a rate of 0.06 s). The camera is coupled to a chromatic filter to cancel Cerenkov signal induced within the fibers upon exposure. By implementing an aperiodic array of six scintillating cells along the bundle axis, we first determine the range of inter-probe spacings leading to optimal source tracking accuracy (first tracking method). Then, three different source tracking algorithms involving all the scintillating probes are tested and compared. In each of these four methods, dwell positions are assessed from dose measurements and compared to the treatment plan. Dwell time is also determined and compared to the treatment plan. RESULTS: The optimum inter-probe spacing for an accurate source tracking ranges from 15 to 35 mm. The optimum detection algorithm consists of adding the readout signals from all detector probes. In that case, the error to the planned dwell positions is of 0.01 ± 0.14 mm and 0.02 ± 0.29 mm at spacings between the source and detector axes of 5.5 and 40 mm, respectively. Using this approach, the average deviations to the expected dwell time are of - 0.006 ± 0.009 $-0.006\,\pm \,0.009$ s and - 0.008 ± 0.058 $-0.008\, \pm 0.058$ s, at spacings between source and probe axes of 5.5 and 20 mm, respectively. CONCLUSIONS: Our six-probe Gd2 O2 S:Tb dosimeter coupled to a sCMOS camera can perform time-resolved treatment verification in HDR brachytherapy. This detection system of high spatial and temporal resolutions (0.25 mm and 0.06 s, respectively) provides a precise information on the treatment delivery via a dwell time and position verification of unmatched accuracy.

Multipixel x ray detection integrated at the end of a narrow multicore fiber.

We introduce and demonstrate the concept of a multipixel detector integrated at the tip of an individual multicore fiber. A pixel consists here of an aluminum-coated polymer microtip incorporating a scintillating powder. Upon irradiation, the luminescence released by the scintillators is efficiently transferred into the fiber cores owing to the specifically elongated metal-coated tips that ensure efficient luminescence matching to the fiber modes. With each pixel being selectively coupled to one of the cores of the multicore optical fiber, the resulting fiber-integrated x ray detection process is totally free from inter-pixel cross talk. Our approach holds promise for fiber-integrated probes and cameras for remote x and gamma ray analysis and imaging in hard-to-reach environments.

Bloch Surface Waves in Open Fabry-Perot Microcavities.

Thanks to the increasing availability of technologies for thin film deposition, all-dielectric structures are becoming more and more attractive for integrated photonics. As light-matter interactions are involved, Bloch Surface Waves (BSWs) may represent a viable alternative to plasmonic platforms, allowing easy wavelength and polarization manipulation and reduced absorption losses. However, plasmon-based devices operating at an optical and near-infrared frequency have been demonstrated to reach extraordinary field confinement capabilities, with localized mode volumes of down to a few nanometers. Although such levels of energy localization are substantially unattainable with dielectrics, it is possible to operate subwavelength field confinement by employing high-refractive index materials with proper patterning such as, e.g., photonic crystals and metasurfaces. Here, we propose a computational study on the transverse localization of BSWs by means of quasi-flat Fabry-Perot microcavities, which have the advantage of being fully exposed toward the outer environment. These structures are constituted by defected periodic corrugations of a dielectric multilayer top surface. The dispersion and spatial distribution of BSWs' cavity mode are presented. In addition, the hybridization of BSWs with an A exciton in a 2D flake of tungsten disulfide (WS2) is also addressed. We show evidence of strong coupling involving not only propagating BSWs but also localized BSWs, namely, band-edge and cavity modes.

Directional Bloch surface wave coupling enabled by magnetic spin-momentum locking of light.

We study the magnetic spin-locking of optical surface waves. Through an angular spectrum approach and numerical simulations, we predict that a spinning magnetic dipole develops a directional coupling of light to transverse electric (TE) polarized Bloch surface waves (BSWs). A high-index nanoparticle as a magnetic dipole and nano-coupler is placed on top of a one-dimensional photonic crystal to couple light into BSWs. Upon circularly polarized illumination, it mimics the spinning magnetic dipole. We find that the helicity of the light impinging on the nano-coupler controls the directionality of emerging BSWs. Furthermore, identical silicon strip waveguides are configured on the two sides of the nano-coupler to confine and guide the BSWs. We achieve a directional nano-routing of BSWs with circularly polarized illumination. Such a directional coupling phenomenon is proved to be solely mediated by the optical magnetic field. This offers opportunities for directional switching and polarization sorting by controlling optical flows in ultra-compact architectures and enables the investigation of the magnetic polarization properties of light.

Characterization of a miniaturized scintillator detector for time-resolved treatment monitoring in HDR-brachytherapy.

Purpose.HDR brachytherapy combines steep dose gradients in space and time, thereby requiring detectors of high spatial and temporal resolution to perform accurate treatment monitoring. We demonstrate a miniaturized fiber-integrated scintillator detector (MSD) of unmatched compactness which fulfills these conditions.Methods.The MSD consists of a 0.28 mm large and 0.43 mm long detection cell (Gd2O2S:Tb) coupled to a 110 micron outer diameter silica optical fiber. The fiber probe is tested in a phantom using a MicroSelectron 9.1 Ci Ir-192 HDR afterloader. The detection signal is acquired at a rate of 0.08 s with a standard sCMOS camera coupled to a chromatic filter (to cancel spurious Cerenkov signal). The dwell position and time monitoring are analyzed over prostate treatment sequences with dwell times spanning from 0.1 to 11 s. The dose rate at the probe position is both evaluated from a direct measurement and by reconstruction from the measured dwell position using the AAPM TG-43 formalism.Results.A total number of 1384 dwell positions are analyzed. In average, the measured dwell positions differ by 0.023 ± 0.077 mm from planned values over a 6-54 mm source-probe distance range. The standard deviation of the measured dwell positions is below 0.8 mm. 94% of the 966 dwell positions occurring at a source-probe inter-catheter spacing below 20 mm are successfully identified, with a 100% detection rate for dwell times exceeding 0.5 s. The average deviation to the planned dwell times is of 0.005 ± 0.060 s. The instant dose retrieval from dwell position monitoring leads to a relative mismatch to planned values of 0.14% ± 0.7%.Conclusion.A miniaturized Gd2O2S:Tb detector coupled to a standard sCMOS camera can be used for time-resolved treatment monitoring in HDR Brachytherapy.

Optomagnets in nonmagnetic plasmonic nanostructures: erratum.

This erratum amends two errors in Opt. Lett.46, 613 (2021)OPLEDP0146-959210.1364/OL.411108.

Miniaturized scintillator dosimeter for small field radiation therapy.

The concept of a miniaturized inorganic scintillator detector is demonstrated in the analysis of the small static photon fields used in external radiation therapy. Such a detector is constituted by a 0.25 mm diameter and 0.48 mm long inorganic scintillating cell (1.6 × 10-5cm3detection volume) efficiently coupled to a narrow 125µm diameter silica optical fiber using a tiny photonic interface (an optical antenna). The response of our miniaturized scintillator detector (MSD) under 6 MV bremsstrahlung beam of various sizes (from 1 × 1 cm2to 4 × 4 cm2) is compared to that of two high resolution reference probes, namely, a micro-diamond detector and a dedicated silicon diode. The spurious Cerenkov signal transmitted through our bare detector is rejected with a basic spectral filtering. The MSD shows a linear response regarding the dose, a repeatability within 0.1% and a radial directional dependence of 0.36% (standard deviations). Beam profiling at 5 cm depth with the MSD and the micro-diamond detector shows a mismatch in the measurement of the full widths at 80% and 50% of the maximum which does not exceed 0.25 mm. The same difference range is found between the micro-diamond detector and a silicon diode. The deviation of the percentage depth dose between the MSD and micro-diamond detector remains below 2.3% within the first fifteen centimeters of the decay region for field sizes of 1 × 1 cm2, 2 × 2 cm2and 3 × 3 cm2(0.76% between the silicon diode and the micro-diamond in the same field range). The 2D dose mapping of a 0.6 × 0.6 cm2photon field evidences the strong 3D character of the radiation-matter interaction in small photon field regime. From a beam-probe convolution theory, we predict that our probe overestimates the beam width by 0.06%, making our detector a right compromise between high resolution, compactness, flexibility and ease of use. The MSD overcomes problem of volume averaging, stem effects, and despite its water non-equivalence it is expected to minimize electron fluence perturbation due to its extreme compactness. Such a detector thus has the potential to become a valuable dose verification tool in small field radiation therapy, and by extension in Brachytherapy, FLASH-radiotherapy and microbeam radiation therapy.

Plasmonic Helical Nanoantenna As a Converter between Longitudinal Fields and Circularly Polarized Waves.

A wide variety of optical applications and techniques require control of light polarization. So far, the manipulation of light polarization relies on components capable of interchanging two polarization states of the transverse field of a propagating wave (e.g., linear to circular polarizations, and vice versa). Here, we demonstrate that an individual helical nanoantenna is capable of locally converting longitudinally oriented confined near-fields into a circularly polarized freely propagating wave, and vice versa. To this end, the nanoantenna is coupled to cylindrical surface plasmons bound to the top interface of a thin gold layer. Helices of constant and varying pitch lengths are experimentally investigated. The reciprocal conversion of an incoming circularly wave into diverging cylindrical surface plasmons is demonstrated as well. Interconnecting circularly polarized optical waves (carrying spin angular momentum) and longitudinal near-fields provides a new degree of freedom in light polarization control.

Optomagnets in nonmagnetic plasmonic nanostructures.

Using a simplified hydrodynamic model of the free electron gas of a metal, we theoretically investigate optically induced DC current loops in a plasmonic nanostructure. Such current loops originate from an optical rectification process relying on three electromotive forces, one of which arises from an optical spin-orbit interaction. The resulting static magnetic field is found to be maximum and dramatically confined at the corners of the plasmonic nanostructure, which reveals the ability of metallic discontinuities to concentrate and tailor static magnetic fields on the nanoscale. Plasmonics can thus generate and tune static magnetic fields and strong magnetic forces on the nanoscale, potentially impacting small scale magnetic tweezing and sensing as well as the generation of magneto-optical effects and spin waves.

Vortex Beam Generation by Spin-Orbit Interaction with Bloch Surface Waves.

Axis-symmetric grooves milled in metallic slabs have been demonstrated to promote the transfer of Orbital Angular Momentum (OAM) from far- to near-field and vice versa, thanks to spin-orbit coupling effects involving Surface Plasmons (SP). However, the high absorption losses and the polarization constraints, which are intrinsic in plasmonic structures, limit their effectiveness for applications in the visible spectrum, particularly if emitters located in close proximity to the metallic surface are concerned. Here, an alternative mechanism for vortex beam generation is presented, wherein a free-space radiation possessing OAM is obtained by diffraction of Bloch Surface Waves (BSWs) on a dielectric multilayer. A circularly polarized laser beam is tightly focused on the multilayer surface by means of an immersion optics, such that TE-polarized BSWs are launched radially from the focused spot. While propagating on the multilayer surface, BSWs exhibit a spiral-like wavefront due to the Spin-Orbit Interaction (SOI). A spiral grating surrounding the illumination area provides for the BSW diffraction out-of-plane and imparts an additional azimuthal geometric phase distribution defined by the topological charge of the spiral structure. At infinity, the constructive interference results into free-space beams with defined combinations of polarization and OAM satisfying the conservation of the Total Angular Momentum, based on the incident polarization handedness and the spiral grating topological charge. As an extension of this concept, chiral diffractive structures for BSWs can be used in combination with surface cavities hosting light sources therein.

Miniaturized fiber dosimeter of medical ionizing radiations on a narrow optical fiber.

Fiber dosimeters have recently drawn much interest for measuring in vivo and in real time the dose of medical radiations. This paper presents the first miniaturized fiber dosimeter integrated at the end of a narrow 125 µm outer diameter optical fiber. Miniaturization is rendered possible by exploiting the concept of a leaky wave optical antenna for interfacing the scintillators and the fiber and by taking advantage of the low propagation loss of narrow silica fibers and high detection yield of single-pixel photon counters. Upon irradiation at 6 MV in air, our fiber probe leads to a linear detection response with a signal-to-noise ratio as high as 195. Although implemented with inorganic scintillators and fiber, our miniaturized fiber probe induces minimum screening effects on ionizing radiations over a negligible area (0.153 mm2). Our nano-optically driven approach may thus result in ultra-compact fiber dosimeters of negligible footprint in the radiotherapeutic processes, even with non-water equivalent fibers and scintillators. This opens new opportunities for a large panel of therapies relying on ionizing radiations (photons or charged particles).

Chiroptical transmission through a plasmonic helical traveling-wave nanoantenna, towards on-tip chiroptical probes.

Resonant plasmonic helices have been widely utilized for locally enhancing and tailoring optical chirality. Here we investigate their nonresonant operation through the recently introduced concept of a plasmonic helical "traveling-wave" nanoantenna. Relying on the coupling of a nonresonant plasmonic helix and a nano-aperture, the helical traveling-wave nanoantenna transmits circularly polarized light with the same handedness as the helix and blocks the other, with a measured dissymmetry factor larger than 1.92 (maximum value of 2). This chiroptical transmission is spatially localized, spectrally broadband, and background-free. Finally, we demonstrate the possibility to engineer such a plasmonic helical nanoantenna at the apex of a sharp tip typically used in scanning near-field microscopies, thus opening the route for moveable, broadband, and background-free chiroptical probes.

Subwavelength polarization optics via individual and coupled helical traveling-wave nanoantennas.

Light polarization control is a key factor in modern photonics. Recent advances in surface plasmon manipulation have introduced the prospect of more compact and more efficient devices for this purpose. However, the current plasmonic-based polarization optics remain much larger than the wavelength of light, which limits the design degrees of freedom. Here, we present a plasmonic traveling-wave nanoantenna using a gold-coated helical carbon nanowire end-fired with a dipolar aperture nanoantenna. Our nonresonant helical nanoantenna enables tunable polarization control by swirling surface plasmons on the subwavelength scale and taking advantage of the optical spin-orbit interaction. Four closely packed helical traveling-wave nanoantennas (HTNs) are demonstrated to locally convert an incoming light beam into four beams of tunable polarizations and intensities, with the ability to impart different polarization states to the output beams in a controllable way. Moreover, by near-field coupling four HTNs of opposite handedness, we demonstrate a subwavelength waveplate-like structure providing a degree of freedom in polarization control that is unachievable with ordinary polarization optics and current metamaterials.

Bloch surface waves at the telecommunication wavelength with lithium niobate as the top layer for integrated optics.

Lithium niobate (LN)-based devices are widely used in integrated and nonlinear optics. This material is robust and resistive to high temperatures, which makes the LN-based devices stable, but challenging to fabricate. In this work, we report on the design, manufacturing, and characterization of engineered dielectric media with thin-film LN (TFLN) on top for the coupling and propagation of electromagnetic surface waves at telecommunication wavelengths. The designed one-dimensional photonic crystal (1DPhC) sustains Bloch surface waves (BSWs) at the multilayer-air interface at 1550 nm wavelength with a propagation detected over a distance of 3 mm. The working wavelength and improved BSW propagation parameters open the way for exploration of nonlinear properties of BSW-based devices. It is also expected that these novel devices potentially would be able to modify BSW propagation and coupling by external thermal-electrical stimuli due to the improved quality of the TFLN top layer of 1DPhC.

Directing Nanoscale Optical Flows by Coupling Photon Spin to Plasmon Extrinsic Angular Momentum.

As any physical particle or object, light undergoing a circular trajectory features a constant extrinsic angular momentum. Within strong curvatures, this angular momentum can match the spin momentum of a photon, thus providing the opportunity of a strong spin-orbit interaction. Using this effect, we demonstrate tunable symmetry breaking in the coupling of light into a curved nanoscale plasmonic waveguide. The helicity of the impinging optical wave controls the power distribution between the two counter-propagating subwavelength guided modes including unidirectional waveguiding. We found experimentally that up to 95% of the incoupled light can be selectively directed into one of the two propagation directions of a nanoscale waveguide. This approach offers new degrees of freedom in the manipulation of subdiffraction optical modes and thus appealing new prospects for the development of advanced, deeply subwavelength optical functionalities.

Magnetic spin-orbit interaction of light.

We study the directional excitation of optical surface waves controlled by the magnetic field of light. We theoretically predict that a spinning magnetic dipole develops a tunable unidirectional coupling of light to transverse electric (TE) polarized Bloch surface waves (BSWs). Experimentally, we show that the helicity of light projected onto a subwavelength groove milled into the top layer of a 1D photonic crystal (PC) controls the power distribution between two TE-polarized BSWs excited on both sides of the groove. Such a phenomenon is shown to be solely mediated by the helicity of the magnetic optical field, thus revealing a magnetic spin-orbit interaction of light. Remarkably, this magnetic optical effect is clearly observed via a near-field coupler governed by an electric dipole moment: it is of the same order of magnitude as the electric optical effects involved in the coupling. This opens up new degrees of freedom for the manipulation of light and offers desirable and novel opportunities for the development of integrated optical functionalities.

Ultracompact x-ray dosimeter based on scintillators coupled to a nano-optical antenna.

We show that nano-optical antennas are capable of controlling the luminescence induced by the absorption of x rays into matter. The x-ray-excited luminescence from a tiny scintillation cluster coupled to a horn nano-optical antenna is highly directed and determined by the antenna's geometrical parameters. Directionality is sufficiently high to efficiently outcouple the x-ray-excited luminescence to a narrow single-mode optical fiber, thus enabling ultracompact fiber-integrated x-ray sensors. Our nano-optically driven approach offers the possibility of x-ray profiling and dosimetry in ultra-confined environments, opening up new avenues in the fields of x-ray imaging, as well as medical and industrial endoscopy. With this study, to the best of our knowledge, nano-optical antennas make a first key contribution to the development of x-ray sensing protocols and architectures.

Polarization controlled directional propagation of Bloch surface wave.

Bloch surface waves (BSWs) are recently developing alternative to surface plasmon polaritons (SPPs). Due to dramatically enhanced propagation distance and strong field confinement these surface states can be successfully used in on-chip all-optical integrated devices of increased complexity. In this work we propose a highly miniaturized grating based BSW coupler which is gathering launching and directional switching functionalities in a single element. This device allows to control with polarization the propagation direction of Bloch surface waves at subwavelength scale, thus impacting a large panel of domains such as optical circuitry, function design, quantum optics, etc.