Laser-induced particle emission as a precursor to laser damage.

Mass spectrometry was used to investigate particle emission, specifically contaminant species, as a possible precursor to laser damage. Experiments were carried out in a clean ultrahigh vacuum chamber with background pressure of 4 x 10(-8) Pa. Both pulsed (8-ns) and cw Nd:YAG lasers operating at 1.06 microm were used to irradiate a variety of samples, which included uncoated Si, fused silica coated with films of Al(2)O(3), or ZrO(2), and bare Si?111?. In the pulsed laser experiments, both 1-on-1 and N-on-1 irradiations were investigated. Emitted particles were mass analyzed with a quadruple mass spectrometer. Single pulse damage thresholds found in this study were consistent with those reported in the literature. Important differences are exhibited in pulse radiation data depending on whether the laser fluence is above or below the damage threshold as well as on the type of sample irradiated. In cw laser experiments, fluence was sufficient to cause damage only in the SiO(2)/ZrO(2) multilayered coating due to absorption by the Si substrate. Continuous wave irradiation also resulted in desorption signals at lower intensities than was possible with pulsed radiation.

Nondestructive depth profiling of ZnS and MgO films by spectroscopic ellipsometry.

Spectroscopic ellipsometric (SE) measurements followed by linear-regression analysis of the SE data obtained on ZnS and MgO films on vitreous silica substrates reveal the distribution of voids (or low-density regions) in these transparent thin films.

Surface charging in laser damage to dielectric surfaces and thin films.

We investigated the relationship between laser damage and surface charging of the damaged area on dielectric thin film coatings of HfO(2) and M(g)F(2) and on bare polished surfaces of fused silica and M(g)F(2). A noncontacting Kelvin probe was developed which was sensitive to surface charge and surface potential changes and had a patial resolution of 1 mm. With this probe, surface charge density changes due to laser irradiation could be mapped over relatively large areas with great accuracy in a nonintrusive manner. All the samples tested showed the accumulation of negative charge in areas more than 10 times larger in diameter than the laser beam spot or damage area. This initial charge density was observed to decay on a time scale of 1 h to a lower fixed value associated with permanent damage to the surface.

Laser-induced damage in optical materials: sixteenth ASTM symposium.

The Sixteenth Annual Symposium on Optical Materials for High Power Lasers (Boulder Damage Symposium) was held at the National Bureau of Standards in Boulder, CO, 15-17 Oct. 1984. The Symposium was held under the auspices of ASTM Committee F-1, Subcommittee on Laser Standards, with the joint sponsorship of NBS, the Defense Advanced Research Project Agency, the Department of Energy, the Office of Naval Research, and the Air Force Office of Scientific Research. Approximately 180 scientists attended the Symposium, including representatives from England, France, The Netherlands, Scotland, and West Germany. The Symposium was divided into sessions concerning Materials and Measurements, Mirrors and Surfaces, Thin Films, and Fundamental Mechanisms. As in previous years, the emphasis of the papers presented at the Symposium was directed toward new frontiers and new developments. Particular emphasis was given to materials for high-power apparatus. The wavelength range of prime interest was from 10.6,microm to the UV region. Highlights included surface characterization, thin-film-substrate boundaries, and advances in fundamental laser-matter threshold interactions and mechanisms. Harold E. Bennett of the U.S. Naval Weapons Center, Arthur H. Guenther of the U.S. Air Force Weapons Laboratory, David Milam of the Lawrence Livermore National Laboratory, and Brian E. Newnam of the Los Alamos National Laboratory were cochairmen of the Symposium.

1.06-microm laser damage of thin film optical coatings: a round-robin experiment involving various pulse lengths and beam diameters.

A number of commercially available optical coatings, both antireflective and high reflective, have been tested for their laser-induced damage threshold, involving a total of eight different laboratories. The results obtained and the experimental methods used at these laboratories were discussed among the participants in this round robin at a minisymposium held at Balzers, Liechtenstein, 9-10 Dec. 1982. A final report of the round robin and a summary of the conclusions drawn at that symposium are presented.

Three-photon absorption in direct-gap crystals.

Third-order time-dependent perturbation theory, utilizing parabolic and nonparabolic energy bands and calculated (from band structure) higher bands as intermediate levels, and a Keldysh first-order model are used to calculate three-photon-absorption coefficients of several direct-gap crystals. Third-order perturbation results for CdS at 1.06 microm agree well with the experimental data.

Laser induced damage in optical materials: twelfth ASTM symposium.

The twelfth annual Symposium on Optical Materials for High Power Lasers (Boulder Damage Symposium) was held at the National Bureau of Standards in Boulder, Colorado, 30 Sept.-l Oct., 1980. The symposium was held under the auspices of ASTM Committee F-l, Subcommittee on Laser Standards, with the joint sponsorship of NBS, the Defense Advanced Research Projects Agency, the Department of Energy, the Office of Naval Research, and the Air Force Office of Scientific research. Over 150 scientists attended the symposium, including representatives of the United Kingdom, France, Japan, and West Germany. The symposium was divided into sessions concerning materials and measurements, mirrors and surfaces, thin films, and finally fundamental mechanisms. As in previous years, the emphasis of the papers presented at the symposium was directed toward new frontiers and new developments. Particular emphasis was given to materials for high power systems. The wavelength range of prime interest was from 10.6 microm to the UV region. Highlights included surface characterization, thin film-substrate boundaries, and advances in fundamental laser-matter threshold interactions and mechanisms. The scaling of damage thresholds with pulse duration, focal area, and wavelength was discussed in detail. Harold E. Bennett of the Naval Weapons Center, Alexander J. Glass of the Lawrence Livermore National Laboratory, Arthur H. Guenther of the Air Force Weapons Laboratory, and Brian E. Newnam of the Los Alamos National Laboratory were cochairmen of the symposium. The thirteenth annual symposium is scheduled for 17-18 Nov. 1981 at the National Bureau of Standards, Boulder, Colorado.

Laser induced damage in optical materials: eleventh ASTM symposium.

The eleventh Symposium on Optical Materials for High-Power Lasers (Boulder Damage Symposium) was held at the National Bureau of Standards in Boulder, Colorado, 30-31 October 1979. The symposium was held under the auspices of ASTM Committee F-1, Subcommittee on Laser Standards, with the joint sponsorship of NBS, the Defense Advanced Research Projects Agency, the Department of Energy, and the Office of Naval Research. About 150 scientists attended the symposium, including representatives of the United Kingdom, France, Canada, Japan, West Germany, and Denmark. The symposium was divided into sessions concerning transparent optical materials and the measurement of their properties, mirrors and surfaces, thin film characteristics, thin film damage, considerations for high-power systems, and finally theory and breakdown. As in previous years, the emphasis of the papers presented at the symposium was directed toward new frontiers and new developments. Particular emphasis was given to materials for high-power apparatus. The wavelength range of prime interest was from 10.6 microm to the UV region. Highlights included surface characterization, thin film-substrate boundaries, and advances in fundamental laser-matter threshold interactions and mechanisms. The scaling of damage thresholds with pulse duration, focal area, and wavelength was discussed in detail. Harold E. Bennett of the Naval Weapons Center, Alexander J. Glass of the Lawrence Livermore Laboratory, Arthur H. Guenther of the Air Force Weapons Laboratory, and Brian E. Newnam of the Los Alamos Scientific Laboratory were cochairpersons. The twelfth annual symposium is scheduled for 30 September-1 October 1980 at the National Bureau of Standards, Boulder, Colorado.

Low power laser trigger switching of a solid insulated spark gap.

The feasibility of reliably triggering solid dielectric insulated spark gaps by low power ( approximately 6 MW) lasers has been demonstrated. Breakdown of 10-mil Lexan dielectric sheets stressed to 70 kV was initiated by a focused 6 MW, Nd in YAG laser emitting 40 mJ in a pulse 6 ns wide at the half-peak intensity height. Delays achieved were in the tens of ns. Slight increases in laser power or electrical stress should produce shorter delays (<10 ns) and subnanosecond jitter.

Low jitter, low inductance solid dielectric switches.

It has been shown that the use of graded solid dielectric sandwiches in laser-triggered spark gaps (LTS) can lead to highly desirable multichannel operations while maintaining the low delay and jitter performance characteristics of LTS. As many as ten separate breakdown channels were observed when small circular or hexagonal aluminum inserts were inserted between two Mylar dielectric sheets stressed at 4.1 kV/mil. A reduction in rise time was noted for these multichannel switching events.

Laser induced damage in optical materials: tenth ASTM symposium.

The tenth annual Symposium on Optical Materials for High Power Lasers (Boulder Damage Symposium) was held at the National Bureau of Standards in Boulder, Colorado, 12-14 September 1978. The symposium was held under the auspices of ASTM Committee F-1, Subcommittee on Laser Standards, with the joint sponsorship of NBS, the Defense Advanced Research Project Agency, the Department of Energy, and the Office of Naval Research. About 175 scientists attended, including representatives of the United Kingdom, France, Canada, Japan, West Germany, and the Soviet Union. The symposium was divided into sessions concerning the measurement of absorption characteristics, bulk material properties, mirrors and surfaces, thin film damage, coating materials and design, and breakdown phenomena. As in previous years, the emphasis of the papers presented was directed toward new frontiers and new developments. Particular emphasis was given to materials for use from 10.6 microm to the UV region. Highlights included surface characterization, thin film-substrate boundaries, and advances in fundamental laser-matter threshold interactions and mechanisms. The scaling of damage thresholds with pulse duration, focal area, and wavelength was also discussed. In commemoration of the tenth symposium in this series, a number of comprehensive review papers were presented to assess the state of the art in various facets of laser induced damage in optical materials. Alexander J. Glass of Lawrence Livermore Laboratory and Arthur H. Guenther of the Air Force Weapons Laboratory were co-chairpersons. The eleventh annual symposium is scheduled for 30-31 October 1979 at the National Bureau of Standards, Boulder, Colorado.