Accuracy assessment and climatology of MODIS aerosol optical properties over North Africa.

In this study, the aerosol optical depth (AOD) from the Moderate Resolution Imaging Spectroradiometer (MODIS) Collection 6.1 (C6.1) product was compared with ground-based measurements at five sites of the Aerosol Robotic Network (AERONET) in North Africa. The MODIS AOD showed a good correlation coefficient of ~0.78, a very small mean bias error of 0.009, and a root mean square error of 0.126 with AERONET. The Dark Target/Deep Blue (DT/DB) algorithm showed better performance at low aerosol loading while underestimating AOD at higher aerosol loading, mainly for coarse-dominated aerosol types. This work also showed the benefits of using MODIS retrievals as a reliable data source for aerosols and providing a long-term aerosol type classification. The primary aerosol type is dust emitted from the Sahara Desert, and the dusty atmosphere becomes gradually mixed with pollution aerosols approaching the coastal region. The annual mean MODIS AOD at 550 nm and Ångström exponent at 412-650 nm (AE) ranged from 0.17 to 0.45 and from 0.13 to 1.25, respectively, in Algeria between 2001 and 2019. Lower AOD (< 0.22) and higher AE (> 1) were found in the northern region, while the highest AOD (0.35 to 0.45) and the lowest AE (< 0.25) were observed over the Tanezrouft desert in southern Algeria. The seasonal mean AOD was highest in summer, while the lowest was in winter due to very high easterly and northeasterly Harmattan surface wind over Zone of Chotts and the Tidikelt Depression, respectively. The negative AOD trends observed over Algeria could be partially connected to the decline (increase) in surface (850 hPa) winds over potential dust source areas in southern Algeria.

Long-term variations in aerosol optical properties, types, and radiative forcing in the Sichuan Basin, Southwest China.

Long-term variations in aerosol optical properties, types, and radiative forcing over the Sichuan Basin (SCB) and surrounding regions in Southwest China were investigated based on two-decade data (2001-2020) from the Moderate Resolution Imaging Spectroradiometer, Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation, and the Santa Barbara DISORT Atmospheric Radiative Transfer model. The results showed that the aerosol optical depth (AOD550nm) in the SCB, a major polluted region in Southwest China, experienced an increasing tendency at a rate of +0.052 yr-1 during 2001-2006; thereafter, it decreased speedy up from -0.020 to -0.058 yr-1 over recent years, whereas the interannual variation in Ångström exponent (AE470-660nm) presented a persistently increasing trend during 2001-2020, with a rate of +0.014 yr-1. An improved atmospheric environment but an enhanced fine particle contribution to regional aerosols in the SCB was observed. Over the polluted SCB region, the dominant aerosol types were biomass burning/urban industrial and mixed-type aerosols with the proportions of 80.7%-87.5% in regional aerosols, with a higher frequency of clean aerosols in recent years, reflecting an effect of controlling anthropogenic emission in the SCB owing to governmental regulation. By contrast, few changes were observed in the aerosol types and amounts in the eastern Tibetan Plateau (ETP), where clean continental aerosols dominate with high proportion of 93.7% in the clean atmospheric environment. A significant decline in polluted anthropogenic aerosols was observed below 3 km over the SCB, resulting in the regional aerosol extinction coefficients at 532 nm (EC532nm) were declined by -0.22 km-1 from 2013 to 2020. Notably, the decreases in aerosol radiative forcing within the atmosphere were found in the SCB and the adjacent northern Yunnan-Guizhou Plateau (NYGP) and ETP, with -41.6%, -33.7%, and -13.6%, respectively during 2013-2020. This indicates that such an attenuated aerosol heating rate in the atmosphere, caused by aerosol variation, could alter the atmospheric thermal structure over the SCB and surrounding areas for regional changes of environment and climate in recent years.