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1.
J Environ Radioact ; 233: 106611, 2021 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-33857821

RESUMO

The sediments deposited in Lake Kevojärvi (69°45N, 27°00'E) in northernmost Finland were investigated for radioactivity. Freeze cores recovered from the 35-m deep basin has preserved a distinct succession of annual laminations deposited between 1909 and 2015. The basic varve structure is composed of a detrital snowmelt layer and an organic-rich post-snowmelt layer lying on top of the snowmelt layer. The past nuclear events have been preserved in the lake sediment. In order to study these, sediment freeze with annual sediment laminations were recovered from the lake bottom and measured for gamma emitting radionuclides. A total of 53 sediment subsamples, each incorporating sediment from one to two varves i.e. sediment deposited during one to two years, were taken for gamma spectroscopy measurements using low-background HPGe detector system. The measurements showed large variations in 137Cs and 241Am concentrations between different laminae marking different nuclear events in history. This highly resolved profile revealed a detailed record of anthropogenic radioactive fallout from atmospheric nuclear weapons testing during 1950s and 1960s and the Chernobyl accident in 1986. The measured 137Cs concentrations varied between 0.6 and 229 Bq/kg dry weight (dw) while the measured 241Am concentrations varied between 0.6 and 6.4 Bq/kg dw. The 137Cs showed downward migration in the sediment column since 137Cs was also found in varves dating before 1945. The first clear increase in 137Cs concentration was observed in 1956 varve and the 137Cs concentrations were found to peak in the 1964, 1970 and 1986 varves. The 241Am was first observed in 1957 varve and the concentrations peaked in 1960-1962, 1964 and 1970 varves. This demonstrated that 241Am can be a complementary chronostratigraphic marker to 137Cs in sediment. A time delay of one to two years was observed between the years of intensive atmospheric nuclear weapons testing and the increased 137Cs and 241Am concentrations in the sediment varves. In the 210Pb concentrations long-time periods of low (~1930-1950 and ~1990-2000) and high concentrations (~1950-1980) were observed. The reason for large variation was the amount of sediment input. The Constant rate of supply (CRS) model results showed good agreement with the varve counting. The model results showed that the 210Pb deposition has been constant over the last 80 years and no effect of climate change to the 210Pb deposition was observed.


Assuntos
Monitoramento de Radiação , Poluentes Radioativos da Água , Radioisótopos de Césio/análise , Finlândia , Sedimentos Geológicos , Lagos , Poluentes Radioativos da Água/análise
2.
Science ; 340(6139): 1421-7, 2013 Jun 21.
Artigo em Inglês | MEDLINE | ID: mdl-23661643

RESUMO

Understanding the evolution of Arctic polar climate from the protracted warmth of the middle Pliocene into the earliest glacial cycles in the Northern Hemisphere has been hindered by the lack of continuous, highly resolved Arctic time series. Evidence from Lake El'gygytgyn, in northeast (NE) Arctic Russia, shows that 3.6 to 3.4 million years ago, summer temperatures were ~8°C warmer than today, when the partial pressure of CO2 was ~400 parts per million. Multiproxy evidence suggests extreme warmth and polar amplification during the middle Pliocene, sudden stepped cooling events during the Pliocene-Pleistocene transition, and warmer than present Arctic summers until ~2.2 million years ago, after the onset of Northern Hemispheric glaciation. Our data are consistent with sea-level records and other proxies indicating that Arctic cooling was insufficient to support large-scale ice sheets until the early Pleistocene.

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